0000000000007534
AUTHOR
V. I. Mishin
Frequency tripling for resonance ionization spectroscopy (RIS) of Cd
To explore the nucleosynthesis of heavy elements in the rapid neutron-capture process, investigations on short- lived, very neutron-rich Cd isotopes are planned that require pure samples. These will be produced at the CERN-ISOLDE on-line mass separator in combination with a chemically se- lective laser ion source. The excitation scheme for resonance ionization of Cd was tested in Mainz with a copper-vapor- pumped dye laser system. Due to the high ionization potential of Cd, frequency tripling was required for the first excita- tion step.1D 228: 8n m/. Laser light with an average power of 2m Wwas obtained after frequency tripling and was suc- cessfully used for RIS test measurements on cadmi…
On-line yields obtained with the ISOLDE RILIS
The ISOLDE resonance ionization laser ion source (RILIS) allows to ionize efficiently and selectively many metallic elements. In recent yield surveys and on-line experiments with the ISOLDE RILIS we observed 23–34 Mg, 26–34 Al, 98–132 Cd, 149 Tb, 155–177 Yb, 179–200 Tl, 183–215 Pb and 188–218 Bi. The obtained yields are presented together with measured release parameters which allow to extrapolate the release efficiency towards more exotic (short-lived) nuclides of the same elements. 2002 Elsevier Science B.V. All rights reserved.
New information on β-delayed neutron emission from Be-12, Be-14
17 pages, 3 tables, 5 figures, 1 appendix.-- PACS nrs.: 23.40.Hc; 27.20.+n.
Atomic spectroscopy studies of short-lived isotopes and nuclear isomer separation with the ISOLDE RILIS
The Resonance Ionization Laser Ion Source (RILIS) at the ISOLDE on-line isotope separator is based on the selective excitation of atomic transitions by tunable laser radiation. Ion beams of isotopes of 20 elements have been produced using the RILIS setup. Together with the mass separator and a particle detection system it represents a tool for high-sensitive laser spectroscopy of short-lived isotopes. By applying narrow-bandwidth lasers for the RILIS one can study isotope shifts (IS) and hyperfine structure (HFS) of atomic optical transitions. Such measurements are capable of providing data on nuclear charge radii, spins and magnetic moments of exotic nuclides far from stability. Although t…
Light exotic isotopes: recent beam developments and physics applications at ISOLDE
This paper is divided in three parts: (i) the measurement of yields and decay losses of Li and Be isotopes released from a thin foil tantalum target at the CERN/ISOLDE PS-Booster; (ii) results from beta-decay experiments on Be-12 and Be-14, an improved half-life of 21.49(3) ms has been obtained for Be-12; (iii) the beta-decay of C-9. An outline of the analysis procedure to determine the branching at high excitation energies is given. The ground-state branch has been determined to 54.1(15)%.
Study of short-lived tin isotopes with a laser ion source
A chemically selective laser ion source based on resonance ionization of atoms in a hot cavity has been applied for the study of short-lived silver isotopes at CERN/ ISOLDE. Silver atoms were ionized by two resonant excitations and final laser ionization into the continuum. Decay properties of the neutron-rich isotopes121–127Ag were studied with a neutron long-counter and aβ-detector.
Production of radioactive Ag ion beams with a chemically selective laser ion source
Abstract We have developed a chemically selective laser ion source at the CERN-ISOLDE facility in order to study neutron-rich Ag nuclides. A pulsed laser system with high repetition rate has been used based on high-power coppe-vapour pump lasers and dye lasers. With this source significant reductions of the isobaric background has been achieved.
Selective laser ionization of very neutron-rich cadmium isotopes: Decay properties of131Cd83and132Cd84
A chemically selective laser ion source has been applied in a decay study of the very neutron-rich isotopes ${}^{131}\mathrm{Cd}$ and ${}^{132}\mathrm{Cd}$ at CERN/ISOLDE. For the ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of the $N=83$ nuclide ${}^{131}\mathrm{Cd}$ a surprisingly short half-life of $(68\ifmmode\pm\else\textpm\fi{}3)$ ms and a weak delayed-neutron branch of ${P}_{n}=(3.5\ifmmode\pm\else\textpm\fi{}1.0)%$ were observed. For the $N=84$ nuclide ${}^{132}\mathrm{Cd}$ a half-life of $(97\ifmmode\pm\else\textpm\fi{}10)$ ms and a ${P}_{n}$ value of $(60\ifmmode\pm\else\textpm\fi{}15)%$ were obtained. Schematic features of both decay schemes are developed. We find that our new d…
$\beta$ - decay of the M$_{T}$=-1 nucleus $^{58}$Zn studied by selective laser ionization
$\beta$ - decay of $^{58}$Zn has been studied for the first time. A new laser ion-source concept has been used to produce mass-separated sources for $\beta$ and $\gamma$ - spectroscopy. The half-life of $^{58}$Zn was determined to be 86(18) ms. Comparisons are made with previous data from charge-exchange reactions. Our Gamow-Teller strength to the 1$^{+}$ state at 1051 keV excitation in $^{58}$Cu agrees well with the value extracted from a recent ($^{3}$He, t) study. Extensive shell-model calculations are presented.
Selective laser ionization of radioactive Ni-isotopes
Abstract A chemically selective laser ion source based on resonance ionization of atoms in a hot cavity has been applied in the study of Ni-isotopes at the CERN-ISOLDE on-line isotope separator. Laser ionization enhanced the yields of long-lived Ni-isotopes almost four orders of magnitude when compared to the yields obtained with the surface ionization mode of the source. As a result, high yields of long-lived Ni-isotopes were obtained. Separation efficiencies of 0.3 and 0.8% were obtained for Ni produced in uranium-carbide, produced from uranium-di-pthalocyanine, and Ta-foil targets, respectively. Ni was found to be released very slowly from the present target and ion source combination.
Decay of Neutron-Rich Mn Nuclides and Deformation of Heavy Fe Isotopes
The use of chemically selective laser ionization combined with beta-delayed neutron counting at CERN/ISOLDE has permitted identification and half-life measurements for 623-ms Mn-61 up through 14-ms Mn-69. The measured half-lives are found to be significantly longer near N=40 than the values calculated with a QRPA shell model using ground-state deformations from the FRDM and ETFSI models. Gamma-ray singles and coincidence spectroscopy has been performed for Mn-64 and Mn-66 decays to levels of Fe-64 and Fe-66, revealing a significant drop in the energy of the first 2+ state in these nuclides that suggests an unanticipated increase in collectivity near N=40.
Beta decay of the new isotope101Sn
The very neutron-deficient isotope 101Sn was produced in a 50Cr(58Ni, 2p5n) reaction and its decay properties were determined for the first time. By using chemically selective ion sources of an on-line mass separator, the energy spectrum and the half-life (3 ± 1 s) of beta-delayed protons of 101Sn were measured. These results are compared to theoretical predictions.
Ground-state spin of 59Mn
Beta decay of $^{59}$Mn has been studied at PSB-ISOLDE, CERN. The intense and pure Mn beam was produced using the Resonance Ionization Laser Ion Source (RILIS). Based on the measured $\beta$-decay rates the ground-state spin and parity are proposed to be $J^{\pi}$ = 5/2$^{-}$. This result is consistent with the systematic trend of the odd-A Mn nuclei and extends the systematics one step further towards the neutron drip line.
Charge radius change in the heavy tin isotopes until A = 132 from laser spectroscopy
Laser spectroscopy measurements have been carried out on the very neutron-rich tin isotopes with the COMPLIS experimental setup. Using the 5s 25p 23P 0 → 5s 25p6s 3P 1 optical transition, hyperfine spectra of 126-132Sn and 125m, 127m, 129m-131mSn where recorded for the first time. The variation of the mean-square charge radius ( δ〈r 2〉) between these nuclei and nuclear moments of the isomers and the odd isotopes were thus measured. An odd-even staggering which inverts at A = 130 is clearly observed. This indicates a small appearance of a plateau on the δ〈r 2〉 which has to be confirmed by measuring the isotope shift beyond A = 132.
Measurement of the Magnetic Moment of the One-Neutron Halo NucleusB11e
The magnetic moment of ${}^{11}\mathrm{Be}$ ( ${T}_{1/2}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}13.8\phantom{\rule{0ex}{0ex}}\mathrm{s}$) was measured by detecting nuclear magnetic resonance signals in a beryllium crystal lattice. The experimental technique applied to a ${}^{11}{\mathrm{Be}}^{+}$ ion beam from a laser ion source includes in-beam optical polarization, implantation into a metallic single crystal, and observation of rf resonances in the asymmetric angular distribution of the $\ensuremath{\beta}$ decay ( $\ensuremath{\beta}$-NMR). The nuclear magnetic moment $\ensuremath{\mu}{(}^{11}\mathrm{Be})\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}\ensuremath{-}1.6816(8…
β-decay studies of135–137Snusing selective resonance laser ionization techniques
The decays of the very neutron rich Sn isotopes Sn135-137 were studied at CERN/ISOLDE using isotopic and isobaric selectivity achieved by the use of a resonance ionization laser ion source and mass spectroscopy, respectively. Neutron decay rates, gamma-ray singles, and gamma-gamma coincidence data were collected as a function of time. The half-life (T-1/2) and delayed neutron emission probability (P-n) values of 135 Sn were measured to be 530(20) ms and 21(3)%, respectively. For Sn-136, a T-1/2 of 250(30) ms was determined along with a P-n value of 30(5)%. For Sn-137, a T-1/2 of 190(60) ms and a P-n value of 58(15)% were deduced. Identification of low-energy transitions in Sb-135 was made p…