Optical polarization of neutron-rich sodium isotopes and β-NMR measurements of quadrupole moments
The nuclear quadrupole moments of neutron-rich sodium isotopes are being investigated with the help of in-beam polarization by optical pumping in combination with $\beta$-NMR techniques. First measurements have yielded the quadrupole splittings of NMR signals in the lattice of LiNbO$_{3}$ for the isotopes $^{26}$Na, $^{27}$Na and $^{28}$Na. Interaction constants and ratios of the electric quadrupole moments are derived. In view of future experiments, $\beta$-decay asymmetries for the sequence of isotopes up to the $N$=20 neutron shell closure, $^{26-31}$Na, have been measured.
Atomic beam magnetic resonance apparatus for systematic measurement of hyperfine structure anomalies (Bohr-Weisskopf effect)
Abstract An atomic beam magnetic resonance (ABMR) apparatus has been constructed at Orsay, and has been installed at the CERN PS Booster ISOLDE mass separator facility for “on-line” work with radioactive isotopes in a program to measure hyperfine structure anomalies (the Bohr-Weisskopf effect) over long isotopic chains. The hfs anomalies result from the effect of the spatial distribution of the nuclear magnetization on the atomic hfs interaction. Constructional details of the system are described: emphasis is placed on the measurement of nuclear g-factors by a triple resonance, laser state selected, ABMR method. A precision better than 10−4 for gI values has been obtained in stable atomic b…
Measurement of the Spin and Magnetic Moment ofMg31: Evidence for a Strongly Deformed Intruder Ground State
Unambiguous values of the spin and magnetic moment of $^{31}\mathrm{M}\mathrm{g}$ are obtained by combining the results of a hyperfine-structure measurement and a $\ensuremath{\beta}$-NMR measurement, both performed with an optically polarized ion beam. With a measured nuclear $g$ factor and spin $I=1/2$, the magnetic moment $\ensuremath{\mu}(^{31}\mathrm{M}\mathrm{g})=\ensuremath{-}0.88355(15){\ensuremath{\mu}}_{N}$ is deduced. A revised level scheme of $^{31}\mathrm{M}\mathrm{g}$ ($Z=12$, $N=19$) with ground state spin/parity ${I}^{\ensuremath{\pi}}=1/{2}^{+}$ is presented, revealing the coexistence of 1p-1h and 2p-2h intruder states below 500 keV. Advanced shell-model calculations and th…
Nuclear moments of strongly deformed strontium isotopes
Nuclear spins, moments and mean square charge radii of78–100Sr have been obtained by fast ion-beam collinear laserspectroscopy. The experiments performed at ISOLDE have been extended to include99Sr, measured by a non-optical detection scheme with a two-step optical pumping sequence. The results for the strongly deformed isotopes are discussed in the frame of the particle-plus-deformed core model.
Nuclear moments of neon isotopes in the range fromNe17at the proton drip line to neutron-richNe25
Nuclear moments of odd-A neon isotopes in the range 17 ≤ A ≤ 25 have been determined from optical hyperfine structures measured by collinear fast-beam laser spectroscopy. The magnetic dipole moments of 17 Ne, 23 Ne and 25 Ne, as well as the electric quadrupole moment of 23 Ne are either reported for the first time or improved considerably. The measurements also decide for a 1/2 + ground state of 25 Ne. The behavior of the magnetic moments of the proton drip-line nucleus 17 Ne and its mirror partner 17 N suggests isospin symmetry. Thus, no clear indication of an anomalous nuclear structure is found for 17 Ne. The magnetic moments of the investigated nuclei are discussed in a shell-model appr…
Spin, moments, and mean square nuclear charge radius ofSr77
The neutron deficient $^{77}\mathrm{Sr}$ nucleus was studied by fast ion beam collinear laser spectroscopy with a detection scheme based on optical pumping, state selective neutralization, and atom counting. From the measured hyperfine splitting and isotope shift of the Sr II transition 5s $^{2}$${\mathit{S}}_{1/2}$\ensuremath{\rightarrow}5p $^{2}$${\mathit{P}}_{3/2}$ the nuclear spin I=5/2, the nuclear moments \ensuremath{\mu}=-0.348(4)${\mathrm{\ensuremath{\mu}}}_{\mathit{N}}$, ${\mathit{Q}}_{\mathit{s}}$=1.40(11) b, and the change in mean square charge radius \ensuremath{\delta}〈${\mathit{r}}^{2}$${\mathrm{〉}}^{88,77}$=0.248(12) ${\mathrm{fm}}^{2}$ were deduced. These ground-state proper…
Laser spectroscopy measurement of isotope shifts and nuclear moments of short-lived neon isotopes
Within the scope of a laser spectroscopy study of nuclear structure in the sd shell we are measuring nuclear moments and isotope shifts of neon isotopes. An ultra-sensitive variant of collinear laser spectroscopy [1, 2] is applied to a neutralized fast beam from ISOLDE (CERN). The non-optical detection is based on optical pumping, state selective collisional ionization and β-activity counting. This method gives access in particular to the short-lived isotopes in the extended chain of 17–26,28Ne.
On the odd-even staggering of mean-square charge radii in the light krypton and strontium region
Recently isotope shifts of $^{72,74-96}$Kr and $^{77-100}$Sr have been measured at the ISOLDE/ CERN mass separator facility by collinear laser spectroscopy. The deduced changes in mean square charge radii reveal sharp transitions in nuclear shape from spherical near the magic neutron number N=50 towards strongly deformed for both the neutron deficient and neutron rich isotopes far from stability. The mean square charge radii of the neutron deficient isotopes exhibit a sign change of the odd-even staggering (OES), i.e. below the neutron number N=46 the radius is systematically larger for the odd-N nuclei than for their even-N neighbours. This is in contrast to the situation of normal OES whi…
Laser spectroscopy investigation of the nuclear moments and radii of lutetium isotopes
Collinear laser spectroscopy experiments in the LuI transition $5d6s\!^{2} \; ^{2}\!D_{3/2} \rightarrow 5d6s6p \; ^{2}\!D_{3/2}$ were performed on all lutetium isotopes in the range of $^{161-179}$Lu. The nuclear spins, magnetic moments and quadrupole moments were determined from the hyperfine structures observed for 19 ground states and 11 isomers. Variations in the mean square charge radii as a function of neutron number were obtained from the isotope shifts. These data considerably extend the systematics of the properties of nuclei in the upper rare-earth region. A particular feature is the appearance of high-spin and low-spin ground states and isomeric states in the vicinity of the stab…
Spin and Magnetic Moment ofMg33: Evidence for a Negative-Parity Intruder Ground State
We report on the first determination of the nuclear ground-state spin of $^{33}\mathrm{Mg}$, $I=3/2$, and its magnetic moment, $\ensuremath{\mu}=\ensuremath{-}0.7456(5)\text{ }{\ensuremath{\mu}}_{N}$, by combining laser spectroscopy with nuclear magnetic resonance techniques. These values are inconsistent with an earlier suggested 1 particle-1 hole configuration and provide evidence for a 2 particle-2 hole intruder ground state with negative parity. The results are in agreement with an odd-neutron occupation of the $3/2\text{ }[321]$ Nilsson orbital at a large prolate deformation. The discussion emphasizes the need of further theoretical and experimental investigation of the island of inver…
Isotope shifts and nuclear-charge radii in singly ionizedCa40–48
The isotope shifts in the resonance lines 4${\mathit{s}}_{1/2}$\ensuremath{\rightarrow}4${\mathit{p}}_{1/2,3/2}$ in Ca ii have been measured for the isotopes $^{40\mathrm{\ensuremath{-}}48}\mathrm{Ca}$ by fast-ion-beam collinear laser spectroscopy. Atomic many-body perturbation theory was then used to calculate the electronic factor for the field shift, giving F=-285(3) MHz/${\mathrm{fm}}^{2}$. The estimate of the uncertainty in F is based on the agreement at the level of 1% for the 4s and 4p hyperfine structures obtained using the same wave functions which include core polarization and pair correlation to all orders. The theoretical value is in excellent agreement with the result F=-283(6)…
Systematics of nuclear ground state properties inSr78–100by laser spectroscopy
Hyperfine structures and isotope shifts of strontium isotopes with A=78 to A=98 and A=100 were measured by collinear fast beam laser spectroscopy. Nuclear spins, moments and changes in mean square charge radii are extracted from the data. The spins and moments of most of the odd isotopes are explained in the framework of the single particle model. The changes in mean square charge radii are compared with predictions of the droplet model and of Hartree-Fock-plus-BCS calculations. For the isotopes in the transitional regions below and above the N=50 shell closure, the inclusion of quadrupole zero point motion in the Droplet model describes part of the observed shell effect. An additional chan…
The electronic field shift factor of the 4s2S1/2?4p2PJ transitions in CaII
The isotope shifts (IS) of the resonance lines 4s2S1/2−4p2PJin CaII (seven isotopes) have been measured by fast ion beam collinear laser spectroscopy (FIBCLS) with non-optical detection of the resonant laser-ion interaction. The electronic field shift factorF was derived from the experimental IS via a King plot procedure using the mean square nuclear charge radii from muon spectroscopy andelectron scattering. TheJ-independent resultF=−283(6) Mhz/fm2 was obtained. TheF-value resulting from extensive many body perturbation theory (MBPT) calculations, recently performed by Martensson-Pendrill et al., is in excellent agreement with the experimental value, confirming the reliability of the MBPT …
Nuclear ground-state spins and magnetic moments ofMg27,Mg29, andMg31
The ground-state spins and magnetic moments of neutron-rich {sup 27}Mg, {sup 29}Mg, and {sup 31}Mg were measured for the first time with laser and {beta}-NMR spectroscopy at ISOLDE/CERN. The hyperfine structure of {sup 27}Mg--observed in fluorescence--confirms previous assignments of the spin I=1/2 and reveals the magnetic moment {mu}{sub I}({sup 27}Mg)=-0.4107(15){mu}{sub N}. The hyperfine structure and nuclear magnetic resonance of optically polarized {sup 29}Mg--observed in the asymmetry of its {beta} decay after implantation in a cubic crystal--give I=3/2 and {mu}{sub I}({sup 29}Mg)=+0.9780(6){mu}{sub N}. For {sup 31}Mg they yield together I=1/2 and {mu}{sub I}({sup 31}Mg)=-0.88355(15){…
The mean square nuclear charge radius of
We report on a collinear laser spectroscopy measurement of the nuclear charge radius of (I = 3/2), yielding . Within the experimental accuracy, the N = 20 neutron shell closure has no influence on the charge radii of the calcium isotopes.
Nuclear ground state spins of short-lived strontium isotopes
Nuclear ground state spins of the odd-mass strontium isotopes between A=79 and 97 were determined by measurements of the hyperfine structure in the ionic transition 5s2S1/2−5p2P3/2. The spins of93Sr and97Sr are revised to I=5/2 and I=1/2, respectively, while assignments for the remaining isotopes are confirmed.
Laser-spectroscopy measurements of 72–96Kr spins, moments and charge radii
Abstract The spins, moments and radii of krypton isotopes have been investigated by collinear fast-beam laser spectroscopy in combination with ultra-sensitive collisional ionization detection. The sequence of isotopes under study ranges from the neutron-deficient N = Z = 36 isotope 72 Kr to the neutron-rich 96 Kr ( N = 60). The mean-square charge radii in the neighbourhood of the N = 50 neutron-shell closure exhibit a pronounced shell effect which has recently been explained in the framework of relativistic mean-field theory. The results for the neutron-deficient nuclei are related to the shape coexistence of strongly prolate and near-spherical states which is known from nuclear spectroscop…
Defect reactions of implanted Li in ZnSe observed by β-NMR
Abstract Using β-radiation detected nuclear magnetic resonance (β-NMR), we investigated the microscopic behavior of implanted 8 Li in nominally undoped ZnSe crystals. From the temperature-dependent amplitudes of high-resolution NMR spectra we conclude a gradual interstitial-to-substitutional site change between 200 and 350 K . This is in accordance with earlier emission channeling results. We argue that this conversion proceeds via Lii++VZn2−→LiZn− and involves implantation related Zn vacancies.
Nuclear moments and charge radii of argon isotopes between the neutron-shell closures and
We report the measurement of optical isotope shifts for 40−44 Ar relative to 38 Ar from which changes in the mean square nuclear charge radii across the 1f7/2 neutron shell are deduced. In addition, the hyperfine structure of 41 Ar and 43 Ar yields the spins, magnetic dipole and electric quadrupole moments, in particular the spin I = 5/2 for 43 Ar. The investigations were carried out by fast-beam collinear laser spectroscopy using highly sensitive detection based on optical pumping and state-selective collisional ionization. Mean square charge radii are now known from 32 Ar to 46 Ar, covering sd-shell as well as f7/2-shell nuclei. They are discussed in the framework of spherical SGII Skyrme…
The quadrupole moment of the neutron-halo nucleus 11Li
The quadrupole moment ratio of 9Li and 11Li was measured by a combination of in-beam laser induced nuclear polarization and β-NMR in LiNbO3. The result |Q(11Li)/Q(9Li)| = 1.14(16) is consistent with cluster models describing 11Li as composed of a 9Li core and a far extended halo of two loosely bound neutrons.
Moments and Radii of 78–100Sr
The chain of Sr isotopes ranges from the neutron-shell closure at N = 50 into both the N = 38 and N = 60 deformation regions which represent the main topic of this workshop. For a detailed understanding of the nature of these nuclei, laser spectroscopy can provide the ground state spins and moments, as well as the the changes in the mean square charge radii as a function of the neutron number N. Recent experiments at Karlsruhe [1] and at Daresbury [2] essentially cover the neutron-deficient and stable Sr isotopes between N = 40 and N = 50. In order to complement these results, and to extend the measurements into the region of neutron-rich isotopes, we have performed an experiment at the ISO…
Very high sensitivity in collinear laser spectroscopy: resonance detection by particle counting techniques
Abstract Fast-beam collinear laser spectroscopy with resonance detection by counting of fluorescence photons provides a versatile tool for precise determinations of nuclear ground-state properties. The intrinsic high sensitivity of this method can be further increased by almost three orders of magnitude if measuring schemes based on ion or atom counting are introduced. The optical pumping from one atomic state to another at an appreciably different excitation energy is detected via state-selective collisional charge exchange processes and charge-state separated atom or ion counting. Applications of these techniques on alkaline earth, noble gas, mercury and thallium beams is examined.
Charge radii of neon isotopes across the sd neutron shell
We report on the changes in mean square charge radii of unstable neon nuclei relative to the stable Ne-20, based on the measurement of optical isotope shifts. The studies were carried out using collinear laser spectroscopy on a fast beam of neutral neon atoms. High sensitivity on short-lived isotopes was achieved thanks to nonoptical detection based on optical pumping and state-selective collisional ionization, which was complemented by an accurate determination of the beam kinetic energy. The new results provide information on the structural changes in the sequence of neon isotopes all across the neutron sd shell, ranging from the proton drip line nucleus and halo candidate Ne-17 up to the…
Nuclear Charge Radii ofMg21−32
Charge radii of all magnesium isotopes in the sd shell have been measured, revealing evolution of the nuclear shape throughout two prominent regions of assumed deformation centered on (24)Mg and (32)Mg. A striking correspondence is found between the nuclear charge radius and the neutron shell structure. The importance of cluster configurations towards N=8 and collectivity near N=20 is discussed in the framework of the fermionic molecular dynamics model. These essential results have been made possible by the first application of laser-induced nuclear orientation for isotope shift measurements.
Decay pathways of stored metal-cluster anions after collisional activation
Size-selected gold clusters, Open image in new window (n ≤ 21), and tungsten clusters, Open image in new window , and Open image in new window (n = 4 – 8 and 12), stored in a Penning trap have been collisionally activated. Neutral monomer and dimer evaporation are observed in the case of gold. While no fragment products have been observed for tungsten clusters, there is evidence of electron emission from the anions.
Nuclear ground state properties of 99Sr by collinear laser spectroscopy with non-optical detection
Abstract Collinear fast-beam laser spectroscopy, with improved sensitivity for ions with hyperfine split transitions, is performed to measure the hyperfine structure and the isotope shift of the well deformed short-lived 99Sr. The new method consists in ground state depopulation by a two-step optical pumping sequence prior to state selective neutralization and fast-atom counting. A definitive nuclear spin value I = 3 2 , the change in mean square charge radius δ〈r2〉98,99 and the nuclear moments are derived. These results are compared to nuclear spectroscopy information and are interpreted in the frame of the particle plus deformed core model.
Spin and magnetic moment of23Mg
A negative magnetic moment of 23Mg has been determined by collinear laser spectroscopy at CERN-ISOLDE. The absolute value is in agreement with previous measurements by nuclear magnetic resonance while the sign points at high-seniority configurations. The result is consistent with shell-model predictions for nuclei with valence nucleons in the sd shell. ispartof: Journal of Physics G, Nuclear and Particle Physics vol:44 issue:7 status: published
Hyperfine structure constants of the CaII states 4s 2 S 1/2 and 4p 2 P 1/2, 3/2 and the nuclear quadrupole moment of43Ca
The hyperfine structure splittings of the 4s 2 S 1/2 → 4p 2 P 1/2, 3/2 transitions in43CaII have been measured by fast ion beam collinear laser spectroscopy. The resonant laser interaction was observed using non-optical detection based on optical ground state depopulation pumping, state selective neutralization and charge state separated particle counting. The extracted magnetic dipole hyperfine structure constants for43CaA(2 S 1/2)=−805(2) MHz,A(2 P 1/2)=−145.5(1.0) MHz andA(2 P 3/2)=−31.9(0.2) MHz are in excellent agreement with relativistic many body perturbation theory predictions available for this alkali-like ion. The combined results are used to evaluate the semi-empirical analysis m…