A new differentially pumped plunger device to measure excited-state lifetimes in proton emitting nuclei

Abstract A new plunger device has been designed and built to measure the lifetimes of unbound states in exotic nuclei beyond the proton drip-line. The device has been designed to work in both vacuum and dilute-gas environments made possible through the introduction of a low-voltage stepping motor. DPUNS will be used in conjunction with the gas-filled separator RITU and the vacuum separator MARA at the accelerator laboratory of the University of Jyvaskyla, Finland, to measure the lifetimes of excited states with low population cross-sections. This is achieved by eliminating the need for a carbon foil to isolate the helium gas of RITU from the beam line thus reducing the background from beam-…

Evolution of collectivity inHg180andHg182

Lifetimes of yrast states in $^{180}\mathrm{Hg}$ up to the ${8}^{+}$ state and of the ${9}^{\ensuremath{-}}$ state have been extracted from recoil-decay tagged $\ensuremath{\gamma}$-ray spectra by using the recoil distance Doppler-shift method. In addition, lifetimes of yrast states up to the ${10}^{+}$ state in $^{182}\mathrm{Hg}$ have been extracted from recoil-gated $\ensuremath{\gamma}\ensuremath{\gamma}$-coincidence spectra. The present study addresses the evolution of collectivity of two competing shapes in neutron-deficient Hg nuclei as a function of $A$ and the configuration mixing at low spin.

Local suppression of collectivity in theN=80isotones at theZ=58subshell closure

) transition strengths [1] and thenumber of nucleons in the valence shell. The global behaviorof these quantities between the major shells as a function ofthe nucleon number is well understood in the frameworks ofboth collective and microscopic models. One could expect thatthese general trends in the collective properties between themajorshellsaremodulated bythesubshellstructure.However,it is usually thought that the pairing correlations with anenergy scale of about 2 MeV, smear out and dissolve thesubshell structure as long as the separation energies betweenthe subshells are only about a few hundred keV.The recently observed evolution of the isovectorquadrupole-collective valence-shell exc…

Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes

Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po196,198,200,202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po200,202, the transitional and diagonal matrix elements of the 2+1 state are determined. In Po196,198 multistep Coulomb excitation is observed, populating the 4+1,0+2, and 2+2 states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from Po196 onwards. Three model descriptions are used to compare to the data. Calculati…

α -decay spectroscopy of the N=130 isotones Ra218 and Th220 : Mitigation of α -particle energy summing with implanted nuclei

© 2019 American Physical Society. An analysis technique has been developed in order to mitigate energy summing due to sequential short-lived α decays from nuclei implanted into a silicon detector. Using this technique, α-decay spectroscopy of the N=130 isotones Ra218 (Z=88) and Th220 (Z=90) has been performed. The energies of the α particles emitted in the Ra218→Rn214 and Th220→Ra216 ground-state-to-ground-state decays have been measured to be 8381(4) keV and 8818(13) keV, respectively. The half-lives of the ground states of Ra218 and Th220 have been measured to be 25.99(10) μs and 10.4(4) μs, respectively. The half-lives of the ground states of the α-decay daughters, Rn214 and Ra216, have …

Shape dynamics in neutron-rich Kr isotopes: Coulomb excitation of 92Kr, 94Kr and 96Kr

We report on the study of excited states in 92,94,96Kr populated via projectile Coulomb excitation at safe energies. The radioactive ion beams at energies of 2.85 MeV/u were delivered by the REX-ISOLDE facility at CERN and impinged on self-supporting 194,196Pt targets. The emitted γ -rays were detected by the Miniball detector-array. A detailed description of the experimental techniques used for extracting diagonal and transitional matrix elements and of the theoretical framework is given. The present experiment reveals the moderate evolution of the collective structure in the considered neutron-rich Kr isotopic chain, which is supported by the interacting boson model combined with the self…

Coulomb Excitation of Proton-rich N=80 Isotones at HIE-ISOLDE

Abstract A projectile Coulomb-excitation experiment was performed at the radioactive ion beam facility HIE-ISOLDE at CERN. The radioactive 140Nd and 142Sm ions were post accelerated to the energy of 4.62 MeV/A and impinged on a 1.45 mg/cm2-thin 208Pb target. The γ rays depopulating the Coulomb-excited states were recorded by the HPGe-array MINIBALL. The scattered charged particles were detected by a double-sided silicon strip detector in forward direction. Experimental γ-ray intensities were used for the determination of electromagnetic transition matrix elements. Preliminary results for the reduced transition strength of the B ( M 1 ; 2 3 + → 2 1 + ) = 0.35 ( 19 ) μ N 2 of 140Nd and a firs…

Collective 2$^{+1}$ excitations in$^{206}$Po and$^{208,210}$Rn

In the present study, $B(E2; 2^{+}_{1}\rightarrow 0^{+}_{1})$ values have been measured in the 208,210Rn and 206Po nuclei through Coulomb excitation of re-accelerated radioactive beams in inverse kinematics at CERN-ISOLDE. These nuclei have been proposed to lie in, or at the boundary of the region where the seniority scheme should persist. However, contributions from collective excitations are likely to be present when moving away from the N=126 closed shell. Such an effect is confirmed by the observed increased collectivity of the $2^{+}_{1}\rightarrow 0^{+}_{1}$ transitions. Experimental results have been interpreted with the aid of theoretical studies carried out within the BCS-based QRP…

A new plunger device to measure lifetimes of unbound states in tagged exotic nuclei

A new plunger device has been designed and is being built at the University of Manchester to measure lifetimes of unbound states in exotic nuclei approaching the proton drip-line. The device is designed to work in both vacuum and gas environments and will be used in conjunction with the gas filled separator RITU and the vacuum-mode separator MARA at the University of Jyvaskyla, Finland. This will enable the accurate measurement of excited state lifetimes identified via isomer and charged-particle tagging. The plunger will be used to address many key facets of nuclear structure physics with particular emphasis on the effect of deformation on proton emission rates.

Excited states in Ra217 populated in the α decay of Th221

Fine structure in the α decay of Th90221, populating excited states in Ra88217, was studied using αγ-coincidence spectroscopy. Two α-decay branches from Th221 have been newly observed, with Eα(keV)[bα(%)]=7951(8)[0.14(3)] and 8247(3)[1.51(12)], together with three previously known branches. Also, two new states in Ra217 were identified at E = 177 and 227 keV. The ground-state configurations of the odd-A, N = 131 transitional isotones above Pb208 are interpreted from their α-decay fine structure systematics and considered in terms of predictions using spherical shell and reflection-asymmetric models.

Coulomb excitation of re-accelerated 208Rn and 206Po beams

In the present study, B( E2; 2(+)-> 0(+) ) values have been measured in the Rn-208 and Po-206 nuclei through Coulomb excitation of re-accelerated radioactive beams in inverse kinematics at CERN-ISOLDE. The resulting B(E2; 2(+)-> 0(+)) in 208Rn is similar to 0.08 e(2)b(2). These nuclei lie in, or at the boundary of the region where seniority scheme should persist. However, contributions from collective excitations may be present when moving away from the N = 126 shell closure. To date, surprisingly little is known of the transition probabilities between the low-spin states in this region.

Evidence for a Smooth Onset of Deformation in the Neutron-Rich Kr Isotopes

The neutron-rich nuclei Kr94,96 were studied via projectile Coulomb excitation at the REX-ISOLDE facility at CERN. Level energies of the first excited 2 + states and their absolute E2 transition strengths to the ground state are determined and discussed in the context of the E(21+) and B(E2;21+→01+) systematics of the krypton chain. Contrary to previously published results no sudden onset of deformation is observed. This experimental result is supported by a new proton-neutron interacting boson model calculation based on the constrained Hartree-Fock-Bogoliubov approach using the microscopic Gogny-D1M energy density functional. © 2012 American Physical Society.

Testing refined shell-model interactions in thesdshell: Coulomb excitation ofNa26

Background: Shell-model calculations crucially depend on the residual interaction used to approximate the nucleon-nucleon interaction. Recent improvements to the empirical universal $sd$ interaction (USD) describing nuclei within the $sd$ shell yielded two new interactions---USDA and USDB---causing changes in the theoretical description of these nuclei.Purpose: Transition matrix elements between excited states provide an excellent probe to examine the underlying shell structure. These observables provide a stringent test for the newly derived interactions. The nucleus $^{26}\mathrm{Na}$ with 7 valence neutrons and 3 valence protons outside the doubly-magic ${}^{16}\mathrm{O}$ core is used a…

Erratum: Evidence for a Smooth Onset of Deformation in the Neutron-Rich Kr Isotopes [Phys. Rev. Lett.108, 062701 (2012)]

A NEW PLUNGER DEVICE FOR INVESTIGATING THE EFFECTS OF DEFORMATION ON PROTON EMISSION RATES VIA LIFETIME MEASUREMENTS

A new plunger device has been designed and built to measure the lifetimes of unbound states in exotic nuclei beyond the proton drip-line. The device is designed to work in both vacuum and dilute-gas environments made possible through the introduction of a lowvoltage piezoelectric motors. The differential plunger for unbound nuclear states, DPUNS, will be used in conjunction with the gas-filled separator RITU and the vacuum separator MARA at the accelerator laboratory of the University of Jyvaskyla, Finland, to measure the lifetimes of excited states with low population cross-sections. This is achieved by eliminating the need for a carbon foil to isolate the helium gas of RITU from the beam …

Role of Chiral Two-Body Currents in Li6 Magnetic Properties in Light of a New Precision Measurement with the Relative Self-Absorption Technique

A direct measurement of the decay width of the excited ${0}_{1}^{+}$ state of $^{6}\mathrm{Li}$ using the relative self-absorption technique is reported. Our value of ${\mathrm{\ensuremath{\Gamma}}}_{\ensuremath{\gamma},{0}_{1}^{+}\ensuremath{\rightarrow}{1}_{1}^{+}}=8.17(14{)}_{\mathrm{stat}.}(11{)}_{\mathrm{syst}.}\text{ }\text{ }\mathrm{eV}$ provides sufficiently low experimental uncertainties to test modern theories of nuclear forces. The corresponding transition rate is compared to the results of ab initio calculations based on chiral effective field theory that take into account contributions to the magnetic dipole operator beyond leading order. This enables a precision test of the im…

Restoring the valence-shell stabilization in Nd 140

A projectile Coulomb-excitation experiment was performed at the radioactive-ion beam facility HIE-ISOLDE at CERN to obtain E2 and M1 transition matrix elements of Nd-140 using the multistep Coulomb-excitation code GOSIA. The absolute M1 strengths, B(M1; 2(2)(-) -> 2(1)(+)) = 0.033(8)mu(2)(N), B(M1 ; 2(3)(+) -> 2(1)(+)) = 0.26(-0.10)(+0.11)mu(2)(N), and B(M1; 2(4)+ -> 2(1)(+)) <0.04 mu(2)(N) identify the 2(3)(+) state as the main fragment of the one-quadrupole-phonon proton-neutron mixed-symmetry state of Nd-140. The degree of F-spin mixing in Nd-140 was quantified with the determination of the mixing matrix element VF-mix <7(-7)(-13) keV. Peer reviewed

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around Z=82 and the neutron midshell at N=104. Purpose: Evidence for shape coexistence has been inferred from α-decay measurements, laser spectroscopy, and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of Rn202 and Rn…

Search for Isovector Valence-Shell Excitations in 140 Nd and 142 Sm via Coulomb excitation reactions of radioactive ion beams

Projectile Coulomb excitation experiments were performed at HIE-ISOLDE at CERN with the radioactive ion beams of 140Nd and 142Sm. Ions with an energy of 4:62 MeV/A were impinging on a 1.45 mg/cm2 thick 208Pb target. The γ-rays depopulating the Coulomb-excited states were recorded by the HPGe-array MINIBALL and scattered particles were detected by a double-sided silicon strip detector. Experimental intensities were used for the determination of electromagnetic transition matrix elements. A preliminary result of the B(M1; 2+3 → 2+1) of 140Nd and an upper limit for the case of 142Sm are revealing the main fragments of the proton-neutron mixed-symmetry 2+1;ms states.

Transition probability studies in175Au

Transition probabilities have been measured between the low-lying yrast states in 175Au by employing the recoil distance Doppler-shift method combined with the selective recoil-decay tagging technique. Reduced transition probabilities and magnitudes of transition quadrupole moments have been extracted from measured lifetimes allowing dramatic changes in nuclear structure within a low excitation-energy range to probed. The transition quadrupole moment data are discussed in terms of available systematics as a function of atomic number and aligned angular momentum.

Corrigendum to: “Shape dynamics in neutron-rich Kr isotopes: Coulomb excitation of 92Kr, 94Kr and 96Kr” [Nucl. Phys. A 899 (2013) 1–28]

Determination of the B(E3, 0+ → 3−)-excitation strength in octupole-correlated nuclei near A ≈224 by the means of Coulomb excitation at REX-ISOLDE

The IS475 collaboration conducted Coulomb-excitation experiments with postaccelerated radioactive 220Rn and 224Ra beams at the REX-ISOLDE facility. The beam particles (Ebeam ≈ 2.83 MeV/u) were Coulomb excited using 60Ni, 114Cd, and 120Sn scattering targets. De-excitation γ-rays were detected employing the Miniball array and scattered particles were detected in a silicon detector. Exploiting the Coulomb-excitation code GOSIA for each nucleus several matrix elements could be obtained from the measured γ-ray yields. The extracted 3−||Ê3||0+ matrix element allows for the conclusion that, while 220Rn represents an octupole vibrational system, 224Ra has already substantial octupole correlations i…

Lifetime measurements probing triple shape coexistence in ^{175}Au

Lifetimes of the low-lying excited states in the very neutron-deficient nucleus ${}^{175}$Au have been measured by the recoil-distance Doppler-shift method using $\ensuremath{\gamma}$-ray spectra obtained with the recoil-decay tagging technique. Transition quadrupole moments and reduced transition probabilities extracted for this odd-$Z$ nucleus indicate the existence of three different shapes and the competition between collective and noncollective structures.

The Miniball spectrometer

The Miniball germanium detector array has been operational at the REX (Radioactive ion beam EXperiment) post accelerator at the Isotope Separator On-Line facility ISOLDE at CERN since 2001. During the last decade, a series of successful Coulomb excitation and transfer reaction studies have been performed with this array, utilizing the unique and high-quality radioactive ion beams which are available at ISOLDE. In this article, an overview is given of the technical details of the full Miniball setup, including a description of the γ-ray and particle detectors, beam monitoring devices and methods to deal with beam contamination. The specific timing properties of the REX-ISOLDE facility are hi…

Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements inHg184,186and two-state mixing calculations

The neutron-deficient mercury isotopes, $^{184,186}$Hg, were studied with the Recoil Distance Doppler Shift (RDDS) method using the Gammasphere array and the Koln Plunger device. The Differential Decay Curve Method (DDCM) was employed to determine the lifetimes of the yrast states in $^{184,186}$Hg. An improvement on previously measured values of yrast states up to $8^{+}$ is presented as well as first values for the $9_{3}$ state in $^{184}$Hg and $10^{+}$ state in $^{186}$Hg. $B(E2)$ values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia (VMI) model, allowing for extraction of spin-dependent mixing strengths and amplitudes.

Investigation into the Effects of Deformation on Proton Emission Rates via Lifetime Measurements

Studies of pear-shaped nuclei using accelerated radioactive beams

There is strong circumstantial evidence that certain heavy, unstable atomic nuclei are ‘octupole deformed’, that is, distorted into a pear shape. This contrasts with the more prevalent rugby-ball shape of nuclei with reflection-symmetric, quadrupole deformations. The elusive octupole deformed nuclei are of importance for nuclear structure theory, and also in searches for physics beyond the standard model; any measurable electric-dipole moment (a signature of the latter) is expected to be amplified in such nuclei. Here we determine electric octupole transition strengths (a direct measure of octupole correlations) for short-lived isotopes of radon and radium. Coulomb excitation experiments we…

Lifetimes of odd-spin yrast states inHg182

Lifetimes of excited states in $^{182}\mathrm{Hg}$ were extracted from recoil-gated $\ensuremath{\gamma}$-ray spectra and recoil-gated $\ensuremath{\gamma}\ensuremath{\gamma}$-coincidence matrices using the recoil distance Doppler-shift method. States were populated using the $^{96}\mathrm{Mo}$($^{88}\mathrm{Sr}$,$2n$)$^{182}\mathrm{Hg}$ fusion-evaporation reaction. Measured lifetimes allowed transition probabilities, transition quadrupole moments, quadrupole deformation parameters, and transition dipole moments to be deduced for the band formed by the odd-spin yrast states. The experimental results confirm the low degree of octupole collectivity in this mass region.

Shapes and Collectivity in Neutron Deficient Even-Mass 188–198Pb Isotopes

Collectivity in ${}^{\mathrm{196,198}}$Pb isotopes probed in Coulomb-excitation experiments at REX-ISOLDE

The neutron-deficient ${}^{\mathrm{196,198}}$Pb isotopes have been studied in Coulomb-excitation experiments employing the Miniball γ-ray spectrometer and radioactive ion beams from the REX-ISOLDE post-accelerator at CERN. The reduced transition probabilities of the first excited 2+ states in 196Pb and 198Pb nuclei have been measured for the first time. Values of $B(E2)={18.2}_{-4.1}^{+4.8}$ W.u. and $B(E2)={13.1}_{-3.5}^{+4.9}$ W.u., were obtained, respectively. The experiment sheds light on the development of collectivity when moving from the regime governed by the generalised seniority scheme to a region, where intruding structures, associated with different deformed shapes, start to com…

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes: Coulomb excitation of Hg-182, Hg-184, Hg-186 and Hg-188

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate…

Combined in-beam electron andγ-ray spectroscopy ofHg184,186

By exploiting the SAGE spectrometer a simultaneous measurement of conversion electrons and {gamma} rays emitted in the de-excitation of excited levels in the neutron-deficient nuclei {sup 184,186}Hg was performed. The light Hg isotopes under investigation were produced using the 4n channels of the fusion-evaporation reactions of {sup 40}Ar and {sup 148,150}Sm. The measured K- and L-conversion electron ratios confirmed the stretched E2 nature of several transitions of the yrast bands in {sup 184,186}Hg. Additional information on the E0 component of the 2{sub 2}{sup +}{yields}2{sub 1}{sup +} transition in {sup 186}Hg was obtained.

Evolution of Octupole Deformation in Radium Nuclei from Coulomb Excitation of Radioactive Ra222 and Ra228 Beams

There is sparse direct experimental evidence that atomic nuclei can exhibit stable "pear" shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole (E3) matrix elements have been determined for transitions in ^{222,228}Ra nuclei using the method of sub-barrier, multistep Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of E3 matrix elements for different nuclear transitions is explained by describing ^{222}Ra as pear shaped with stable octupole deformation, while ^{228}Ra behaves like an octupole vibrator.

Do nuclei go pear-shaped? Coulomb excitation of 220Rn and 224Ra at REX-ISOLDE (CERN)

Artículo escrito por muchos autores, sólo se referencian el primero, los autores que firman como Universidad Autónoma de Madrid y el grupo de colaboración en el caso de que aparezca en el artículo

Coulomb excitation of Na-29,Na-30: Mapping the borders of the island of inversion

Seidlitz, M., et all ; 10 pags. ; 9 figs. ; 1 tab. ; PACS number(s): 21.60.Cs, 23.20.Js, 25.70.De, 29.38.Gj

Evolution of proton single-particle states in neutron-rich Sb isotopes beyond N=82

11 pags., 8 figs., 2 tabs.

The observation of vibrating pear-shapes in radon nuclei

6 pags., 4 fig.s, 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0

Coulomb excitation of pear-shaped nuclei

There is a large body of evidence that atomic nuclei can undergo octupole distortion and assume the shape of a pear. This phenomenon is important for measurements of electric-dipole moments of atoms, which would indicate CP violation and hence probe physics beyond the Standard Model of particle physics. Isotopes of both radon and radium have been identified as candidates for such measurements. Here, we have observed the low-lying quantum states in 224Rn and 226Rn by accelerating beams of these radioactive nuclei. We show that radon isotopes undergo octupole vibrations but do not possess static pear-shapes in their ground states. We conclude that radon atoms provide less favourable condition…