0000000000084310
AUTHOR
B. G. C. Lackenby
Calculation of atomic spectra and transition amplitudes for superheavy element Db (Z=105)
Atomic spectra and other properties of superheavy element dubnium (Db, $Z=105$) are calculated using recently developed method combining configuration interaction with perturbation theory [the CIPT method, V. A. Dzuba, J. C. Berengut, C. Harabati, and V. V. Flambaum, Phys. Rev. A 95, 012503 (2017)]. These include energy levels for low-lying states of Db and Db II, electric dipole transition amplitudes between the ground state and low-lying states of opposite parity, isotope shift for these transitions, and the ionization potential of Db. Similar calculations for Ta, which is a lighter analog of Db, are performed to control the accuracy of the calculations.
Time reversal violating Magnetic Quadrupole Moment in heavy deformed nuclei
The existence of permanent electric dipole moments (EDMs) and magnetic quadrupole moments (MQMs) violate both time reversal invariance (T) and parity (P). Following the CPT theorem they also violate combined CP symmetry. Nuclear EDMs are completely screened in atoms and molecules while interaction between electrons and MQMs creates atomic and molecular EDMs which can be measured and used to test CP-violation theories. Nuclear MQMs are produced by the nucleon-nucleon T, P-odd interaction and by nucleon EDMs. In this work we study the effect of enhancement of the nuclear MQMs due to the nuclear quadrupole deformation. Using the Nilsson model we calculate the nuclear MQMs for deformed nuclei o…
Theoretical study of the electron structure of superheavy elements with an open 6d shell: Sg, Bh, Hs, and Mt
We use recently developed efficient versions of the configuration interaction method to perform {\em ab initio} calculations of the spectra of superheavy elements seaborgium (Sg, $Z=106$), bohrium (Bh, $Z=107$), hassium (Hs, $Z=108$) and meitnerium (Mt, $Z=109$). We calculate energy levels, ionization potentials, isotope shifts and electric dipole transition amplitudes. Comparison with lighter analogs reveals significant differences caused by strong relativistic effects in superheavy elements. Very large spin-orbit interaction distinguishes subshells containing orbitals with a definite total electron angular momentum $j$. This effect replaces Hund's rule holding for lighter elements.
Theoretical calculation of atomic properties of superheavy elements Z=110-112 and their ions
We calculate the spectra, electric dipole transition rates and isotope shifts of the super heavy elements Ds (Z=110), Rg (Z=111) and Cn (Z=112) and their ions. These calculations were performed using a recently developed, efficient version of the ab initio configuration interaction combined with perturbation theory to treat distant effects. The successive ionization potentials of the three elements are also calculated and compared to lighter elements.
Atomic structure calculations of superheavy noble element oganesson (Z=118)
We calculate the spectrum and allowed E1 transitions of the superheavy element Og (Z=118). A combination of configuration interaction (CI) and perturbation theory (PT) is used (Dzuba \textit{et at.} Phys. Rev. A, \textbf{95}, 012503 (2017)). The spectrum of lighter analog Rn I is also calculated and compared to experiment with good agreement.
Weak quadrupole moments
Collective effects in deformed atomic nuclei present possible avenues of study on the non-spherical distribution of neutrons and the violation of the local Lorentz invariance. We introduce the weak quadrupole moment of nuclei, related to the quadrupole distribution of the weak charge in the nucleus. The weak quadrupole moment produces tensor weak interaction between the nucleus and electrons and can be observed in atomic and molecular experiments measuring parity nonconservation. The dominating contribution to the weak quadrupole is given by the quadrupole moment of the neutron distribution, therefore, corresponding experiments should allow one to measure the neutron quadrupoles. Using the …
Calculation of atomic properties of superheavy elements Z=110–112 and their ions
We calculate the spectra, electric dipole transition rates, and isotope shifts of the superheavy elements Ds ($Z=110$), Rg ($Z=111$), and Cn ($Z=112$) and their ions. These calculations were performed using a recently developed, efficient version of the ab intio configuration-interaction combined with perturbation theory to treat distant effects. The successive ionization potentials of the three elements are also calculated and compared to lighter analogous elements.