On-line commissioning of SHIPTRAP

Abstract The on-line commissioning of the Penning-trap mass spectrometer SHIPTRAP was successfully completed with a mass measurement of holmium and erbium radionuclides produced at SHIP. A large fraction of contaminant ions created in the stopping cell was identified to originate from the buffer-gas supply system. Using a liquid nitrogen cold trap they were reduced to a tolerable amount and mass measurements of Er 147 , Er 148 , and Ho 147 with relative uncertainties of about 1 × 1 0 − 6 were performed.

Total absorption study of the \beta decay of 102,104,105Tc

The β-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely 102,104,105Tc, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations. peerReviewed

Mass ofAl23for testing the isobaric multiplet mass equation

The mass excess of the proton-rich nucleus $^{23}\mathrm{Al}$ has been measured with the JYFLTRAP Penning trap setup. As a result of our experiment we obtain a mass excess of 6748.07(34) keV, and by combining the value to existing experimental data we have tested the validity of the isobaric multiplet mass equation $(\mathrm{IMME})$ for the $T=3/2$ quartet in the $A=23$ isobar. The fit to the IMME results in a vanishing cubic term equivalent to zero with high precision [$0.22(42)$ keV].

Smallest KnownQValue of Any Nuclear Decay: The Rareβ−Decay ofIn115(9/2+)→Sn115(3/2+)

The ground-state-to-ground-state Q_{beta;{-}} value of ;{115}In was determined to 497.68(17) keV using a high-precision Penning trap facility at the University of Jyvaskyla, Finland. From this, a Q_{beta;{-}} value of 0.35(17) keV was obtained for the rare beta;{-} decay to the first excited state of ;{115}Sn at 497.334(22) keV. The partial half-life was determined to 4.1(6) x 10;{20} yr using ultra low-background gamma-ray spectrometry in an underground laboratory. Theoretical modeling of this 2nd-forbidden unique beta;{-} transition was also undertaken and resulted in Q_{beta;{-}} = 57_{-12};{+19} eV using the measured half-life. The discrepancy between theory and experiment could be attr…

Precision mass measurements of neutron-rich Tc, Ru, Rh, and Pd isotopes

The masses of neutron-rich $^{106\ensuremath{-}112}\mathrm{Tc}$, $^{106\ensuremath{-}115}\mathrm{Ru}$, $^{108\ensuremath{-}118}\mathrm{Rh}$, and $^{112\ensuremath{-}120}\mathrm{Pd}$ produced in proton-induced fission of uranium were determined using the JYFLTRAP double Penning trap setup. The measured isotopic chains include a number of previously unmeasured nuclei. Typical precisions on the order of 10 keV or better were achieved, representing a factor of 10 improvement over earlier data. In many cases, significant deviations from the earlier measurements were found. The obtained data set of 39 masses is compared with different mass predictions and analyzed for global trends in the nuclear…

Independent Isotopic Product Yields in 25 MeV and 50 MeV Charged Particle Induced Fission of 238U and 232Th

Abstract Independent isotopic yields for most elements from Zn to La in 25-MeV proton-induced fission of 238U and 232Th have been determined at the IGISOL facility in the University of Jyvaskyla. In addition, isotopic yields for Zn, Ga, Rb, Sr, Zr, Pd and Xe in 50-MeV proton-induced fission of 238U and for Zn, Ga, Rb, Sr, Cd and In in 25-MeV deuterium-induced fission of 238U have been measured. The utilised technique recently developed at the University of Jyvaskyla, is based on a combination of the ion guide technique and the ability of a Penning trap to unambiguously identify the isotopes by their atomic mass. Since the yields are determined by ion counting, no prior knowledge beyond the …

Mass measurements in the vicinity of the doubly magic waiting pointNi56

Masses of $^{56,57}\mathrm{Fe}$, $^{53}\mathrm{Co}$${}^{m}$, $^{53,56}\mathrm{Co}$, $^{55,56,57}\mathrm{Ni}$, $^{57,58}\mathrm{Cu}$, and $^{59,60}\mathrm{Zn}$ have been determined with the JYFLTRAP Penning trap mass spectrometer at the Ion-Guide Isotope Separator On-Line facility with a precision of $\ensuremath{\delta}m/m\ensuremath{\leqslant}3\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}$. The ${Q}_{\mathrm{EC}}$ values for $^{53}\mathrm{Co}$, $^{55}\mathrm{Ni}$, $^{56}\mathrm{Ni}$, $^{57}\mathrm{Cu}$, $^{58}\mathrm{Cu}$, and $^{59}\mathrm{Zn}$ have been measured directly with a typical precision of better than $0.7 \mathrm{keV}$ and Coulomb displacement energies have been dete…

Electron-capture branch ofTc100and tests of nuclear wave functions for double-βdecays

We present a measurement of the electron-capture branch of $^{100}\mathrm{Tc}$. Our value, $B(\mathrm{EC})=(2.6\ifmmode\pm\else\textpm\fi{}0.4)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$, implies that the $^{100}\mathrm{Mo}$ neutrino absorption cross section to the ground state of $^{100}\mathrm{Tc}$ is roughly 50% larger than previously thought. Disagreement between the experimental value and QRPA calculations relevant to double-$\ensuremath{\beta}$ decay matrix elements persists. We find agreement with previous measurements of the 539.5- and 590.8-keV $\ensuremath{\gamma}$-ray intensities.

$Q$-value of the superallowed $\beta$ decay of 62Ga

Masses of the radioactive isotopes 62Ga, 62Zn and 62Cu have been measured at the JYFLTRAP facility with a relative precision of better than 18 ppb. A Q_EC value of (9181.07 +- 0.54) keV for the superallowed decay of 62Ga is obtained from the measured cyclotron frequency ratios of 62Ga-62Zn, 62Ga-62Ni and 62Zn-62Ni ions. The resulting Ft-value supports the validity of the conserved vector current hypothesis (CVC). The mass excess values measured were (-51986.5 +-1.0) keV for 62Ga, (-61167.9 +- 0.9) keV for 62Zn and (-62787.2 +- 0.9) keV for 62Cu.

Upgrade and yields of the IGISOL facility

The front end of the Jyvaskyla IGISOL facility was upgraded in 2003 by increasing its pumping capacity and by improving the radiation shielding. In late 2005, the skimmer electrode of the mass separator was replaced by a sextupole ion guide, which improved the mass separator efficiency up to an order of magnitude. The current design of the facility is described. The updated yield data, achieved with and without the additional JYFLTRAP purification, using both fusion evaporation reactions and particle induced fission is presented to give an overview of the capability of the facility. These data have been determined either by radioactivity measurements or by direct ion counting after the Penn…

Half-life, branching-ratio, andQ-value measurement for the superallowed0+→0+β+emitterTi42

The half-life, the branching ratio, and the decay $Q$ value of the superallowed $\ensuremath{\beta}$ emitter $^{42}\mathrm{Ti}$ were measured in an experiment performed at the JYFLTRAP facility of the Accelerator Laboratory of the University of Jyv\"askyl\"a. $^{42}\mathrm{Ti}$ is the heaviest ${T}_{z}=\ensuremath{-}1$ nucleus for which high-precision measurements of these quantities have been tried. The half-life (${T}_{1/2}=208.14\ifmmode\pm\else\textpm\fi{}0.45$ ms) and the $Q$ value [${Q}_{\mathrm{EC}}=7016.83(25)$ keV] are close to or reach the required precision of about 0.1%. The branching ratio for the superallowed decay branch [$\mathrm{BR}=47.7(12)%$], a by-product of the half-lif…

β-decay data requirements for reactor decay heat calculations: study of the possible source of the gamma-ray discrepancy in reactor heat summation calculations

The decay heat of fission products plays an important role in predictions of the heat up of nuclear fuel in reactors. The released energy is calculated as the summation of the activities of allfission products P(t) = Ei λi Ni(t), where Ei is the decay energy of nuclide i (gamma and beta component), λi is the decay constant of nuclide i and Ni(t) is the number of nuclide i at cooling time t. Even though the reproduction of the measured decay heat has improved in recent years, there is still a long standing discrepancy in the t ∼ 1000s cooling time for some fuels. A possible explanation to this improper description has been found in the work of Yoshida et al. (1), where it has been shown that…

Q values of the 76Ge and 100Mo double-beta decays

Abstract Penning trap measurements using mixed beams of 76Ge–76Se and 100Mo–100Ru have been utilized to determine the double-beta decay Q-values of 76Ge and 100Mo with uncertainties less than 200 eV. The value for 76Ge, 2039.04(16) keV is in agreement with the published SMILETRAP value, 2039.006(50) keV. The new value for 100Mo, 3034.40(17) keV is 30 times more precise than the previous literature value, sufficient for the ongoing neutrinoless double-beta decay searches in 100Mo. Moreover, the precise Q-value is used to calculate the phase-space integrals and the experimental nuclear matrix element of double-beta decay.

Independent isotopic yields in 25 MeV and 50 MeV proton-induced fission of natU

Independent isotopic yields for elements from Zn to La in the 25 MeV proton-induced fission of natUnatU were determined with the JYFLTRAP facility. In addition, isotopic yields for Zn, Ga, Rb, Sr, Zr, Pd and Xe in the 50 MeV proton-induced fission of natUnatU were measured. The deduced isotopic yield distributions are compared with a Rubchenya model, the GEF model with universal parameters and the semi-empirical Wahl model. Of these, the Rubchenya model gives the best overall agreement with the obtained data. Combining the isotopic yield data with mass yield data to obtain the absolute independent yields was attempted. The result depends on the mass yield distribution. peerReviewed

Direct mass measurements above uranium bridge the gap to the island of stability

The mass of an atom incorporates all its constituents and their interactions. The difference between the mass of an atom and the sum of its building blocks (the binding energy) is a manifestation of Einstein's famous relation E = mc(2). The binding energy determines the energy available for nuclear reactions and decays (and thus the creation of elements by stellar nucleosynthesis), and holds the key to the fundamental question of how heavy the elements can be. Superheavy elements have been observed in challenging production experiments, but our present knowledge of the binding energy of these nuclides is based only on the detection of their decay products. The reconstruction from extended d…

Precision mass measurements of neutron-rich yttrium and niobium isotopes

Abstract The atomic masses of neutron-rich 95–101 Y and 101–107 Nb produced in proton-induced fission of uranium were determined using the JYFLTRAP double Penning trap setup. Accuracies of better than 10 keV could be reached for most nuclides. The masses of 106,107 Nb were measured for the first time. The energies of the isomeric states in 96 Y and 100 Y were measured as 1541(10) keV and 145(15) keV. The niobium isotopes appear to be systematically less bound than the values given in the latest Atomic Mass Evaluation. The new data lie in a region of the nuclear chart characterised by the transition from spherical to strongly deformed shapes. These structural changes are explored by studying…

Penning-trap-assisted study of 115Ru beta decay

The beta decay of 115Ru has been studied by means of Penning-trap-assisted beta and gamma spectroscopy at the IGISOL facility. The level scheme of 115Rh has been substantially extended and compared with the level systematics of lighter rhodium isotopes. Tentative candidates for three states of the deformed K = 1/2 band have been suggested. The beta-strength distribution of the beta decay of 115Ru differs from the beta decays of 111, 113, 113mRu isotopes due to non-observation of the 3-quasiparticle states in 115Rh. The decay properties of 115Ru indicate a spin-parity of (3/2+ for its beta-decaying ground state. In addition, possible Nilsson states as well as the shape and spin transitions i…

Mass Measurements and Implications for the Energy of the High-Spin Isomer inAg94

Nuclides in the vicinity of {sup 94}Ag have been studied with the Penning trap mass spectrometer JYFLTRAP at the Ion-Guide Isotope Separator On-Line. The masses of the two-proton-decay daughter {sup 92}Rh and the beta-decay daughter {sup 94}Pd of the high-spin isomer in {sup 94}Ag have been measured, and the masses of {sup 93}Pd and {sup 94}Ag have been deduced. When combined with the data from the one-proton- or two-proton-decay experiments, the results lead to contradictory mass excess values for the high-spin isomer in {sup 94}Ag, -46 370(170) or -44 970(100) keV, corresponding to excitation energies of 6960(400) or 8360(370) keV, respectively.

Reactor Decay Heat inPu239: Solving theγDiscrepancy in the 4–3000-s Cooling Period

The {beta} feeding probability of {sup 102,104,105,106,107}Tc, {sup 105}Mo, and {sup 101}Nb nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the {gamma} component of the decay heat for {sup 239}Pu in the 4-3000 s range.

Decay study ofTc114with a Penning trap

The level structure of $^{114}\mathrm{Ru}$ has been investigated via the $\ensuremath{\beta}$ decay of very neutron-rich $^{114}\mathrm{Tc}$ by means of Penning-trap-assisted $\ensuremath{\gamma}$ spectroscopy. The deduced $\ensuremath{\beta}$-decay scheme suggests the existence of two $\ensuremath{\beta}$-decaying states in $^{114}\mathrm{Tc}$ with ${I}^{\ensuremath{\pi}}={1}^{+}$ and $I\ensuremath{\geqslant}$ 4, with half-lives of ${t}_{1/2}({1}^{+})=90(20)$ ms and ${t}_{1/2}(I\ensuremath{\geqslant}4)=100(20)$ ms, respectively. The ${Q}_{\ensuremath{\beta}}$ value, which covers a possible mixture of two states, has been determined to be ${Q}_{\ensuremath{\beta}}=11 785(12)$ keV. The level…

QValues of the SuperallowedβEmittersAlm26,Sc42, andV46and Their Impact onVudand the Unitarity of the Cabibbo-Kobayashi-Maskawa Matrix

The $\ensuremath{\beta}$-decay ${Q}_{\mathrm{EC}}$ values of the superallowed beta emitters $^{26}\mathrm{Al}^{m}$, $^{42}\mathrm{Sc}$, and $^{46}\mathrm{V}$ have been measured with a Penning trap to a relative precision of better than $8\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}$. Our result for $^{46}\mathrm{V}$, 7052.72(31) keV, confirms a recent measurement that differed from the previously accepted reaction-based ${Q}_{\mathrm{EC}}$ value. However, our results for $^{26}\mathrm{Al}^{m}$ and $^{42}\mathrm{Sc}$, 4232.83(13) keV and 6426.13(21) keV, are consistent with previous reaction-based values. By eliminating the possibility of a systematic difference between the two t…

Quenching of the SnSbTe Cycle in the rp-Process

Systematic studies of the accuracy of the Penning trap mass spectrometer JYFLTRAP

Abstract Measurements to quantify the mass-dependent systematic effect and the residual uncertainty of the JYFLTRAP setup have been performed with carbon-cluster ions. The primary quantities reported in this work are a mass-dependent uncertainty of σ m ( r ) / r = ( 7.8 ± 0.3 × 10 - 10 / u ) × Δ m and a residual uncertainty of σ res ( r ) / r = 1.2 × 10 - 8 for the JYFLTRAP mass spectrometer. By restricting the mass difference between the reference ion and ion of interest to | m meas - m ref | ≤ 24 , the values for the mass-dependent effect and the corresponding residual uncertainty are σ m , lim ( r ) / r = ( 7.5 ± 0.4 × 10 - 10 / u ) × Δ m and σ res , lim ( r ) / r = 7.9 × 10 - 9 , respec…

Improvements on Decay Heat Summation Calculations by Means of Total Absorption Gamma-ray Spectroscopy Measurements

The decay heat of fission products plays an important role in predictions of the heat released by nuclear fuel in reactors. In this contribution we present results of the analysis of the measurement of the beta decay of some refractory isotopes that were considered possible important contributors to the decay heat in reactors. The measurements presented here were performed at the IGISOL facility of the University of Jyvaeskylae, Finland. In our measurements we have combined for the first time a Penning trap (JYFLTRAP), which was used as a high resolution isobaric separator, with a total absorption spectrometer. The results of the measurements as well as their consequences for decay heat sum…

Masses of neutron-rich Ni and Cu isotopes and the shell closure at Z = 28 , N = 40

The Penning trap mass spectrometer JYFLTRAP, coupled to the Ion Guide Isotope Separator On-Line (IGISOL) facility at Jyvaskyla, was employed to measure the atomic masses of neutron-rich 70-73Ni and 73, 75Cu isotopes with a typical accuracy less than 5keV. The mass of 73Ni was measured for the first time. Comparisons with the previous data are discussed. Two-neutron separation energies show a weak subshell closure at 68 28Ni40 . A well established proton shell gap is observed at Z = 28 .

Preparing isomerically pure beams of short-lived nuclei at JYFLTRAP

A new procedure to prepare isomerically clean samples of ions with a mass resolving power of more than 100,000 has been developed at the JYFLTRAP tandem Penning trap system. The method utilises a dipolar rf-excitation of the ion motion with separated oscillatory fields in the precision trap. During a subsequent retransfer to the purification trap, the contaminants are rejected and as a consequence, the remaining bunch is isomerically cleaned. This newly-developed method is suitable for very high-resolution cleaning and is at least a factor of five faster than the methods used so far in Penning trap mass spectrometry.

Mass measurements of neutron-deficient nuclides close to A=80 with a Penning trap

The masses of 80,81,82,83Y, 83,84,85,86,88Zr and 85,86,87,88Nb have been measured with a typical precision of 7 keV by using the Penning trap setup at IGISOL. The mass of 84Zr has been measured for the first time. These precise mass measurements have improved Sp and QEC values for astrophysically important nuclides. peerReviewed

JYFLTRAP: a Penning trap for precision mass spectroscopy and isobaric purification

In this article a comprehensive description and performance of the double Penning-trap setup JYFLTRAP will be detailed. The setup is designed for atomic mass measurements of both radioactive and stable ions and additionally serves as a very high-resolution mass separator. The setup is coupled to the IGISOL facility at the accelerator laboratory of the University of Jyväskylä. The trap has been online since 2003 and it was shut down in the summer of 2010 for relocation to the upgraded IGISOL facility. Numerous atomic mass and decay energy measurements have been performed using the time-of-flight ion-cyclotron resonance technique. The trap has also been used in several decay spectroscopy expe…

Development of a carbon-cluster ion source for JYFLTRAP

Abstract A carbon-cluster ion source based on laser ablation and ionization of a carbon sample has been built and tested for the JYFLTRAP setup. In the present configuration the ion source is situated in the electrostatic switchyard in front of the radiofrequency (RFQ) cooler and buncher. In this position the beam quality of the carbon clusters injected into the Penning trap system is considerably improved by the RFQ. Moreover, the mass-dependence of the RFQ’s transmission can be used to some extent to suppress unwanted cluster sizes.

An ion guide for the production of a low energy ion beam of daughter products of α-emitters

A new ion guide has been modeled and tested for the production of a low energy ($\approx$ 40 kV) ion beam of daughter products of alpha-emitting isotopes. The guide is designed to evacuate daughter recoils originating from the $\alpha$-decay of a $^{233}$U source. The source is electroplated onto stainless steel strips and mounted along the inner walls of an ion guide chamber. A combination of electric fields and helium gas flow transport the ions through an exit hole for injection into a mass separator. Ion guide efficiencies for the extraction of $^{229}$Th$^{+}$ (0.06%), $^{221}$Fr$^{+}$ (6%), and $^{217}$At$^{+}$ (6%) beams have been measured. A detailed study of the electric field and …

Total absorption study of theβdecay of102,104,105Tc

The $\ensuremath{\beta}$-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely ${}^{102,104,105}$Tc, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations.

AccurateQValue for theSn112Double-βDecay and its Implication for the Search of the Neutrino Mass

The $Q$ value of the $^{112}\mathrm{Sn}$ double-beta decay was determined by using a Penning trap mass spectrometer. The new atomic-mass difference between $^{112}\mathrm{Sn}$ and $^{112}\mathrm{Cd}$ of 1919.82(16) keV is 25 times more precise than the previous value of 1919(4) keV. This result removes the possibility of enhanced resonance capture of the neutrinoless double-EC decay to the excited ${0}^{+}$ state at 1871.00(19) keV in $^{112}\mathrm{Cd}$.

Quenching of the SnSbTe Cycle in therpProcess

The nuclides 104-108Sn, 106-110Sb, 108,109Te, and 111I at the expected endpoint of the astrophysical rp process have been produced in 58Ni+natNi fusion-evaporation reactions at IGISOL and their mass values were precisely measured with the JYFLTRAP Penning trap mass spectrometer. For 106Sb, 108Sb, and 110Sb these are the first direct experimental mass results obtained. The related one-proton separation energies have been derived and the value for 106Sb, Sp=424(8) keV, shows that the branching into the closed SnSbTe cycle in the astrophysical rp process is weaker than expected.