0000000000170831
AUTHOR
Dietrich Althausen
Radiative and dynamic effects of absorbing aerosol particles over the Pearl River Delta, China
Abstract Results are reported from a ground-based measurement campaign conducted in a highly polluted region in southeast of China in October–November 2004. The experiment focused on absorbing aerosol particles and their effects on the solar radiation field and local meteorology. A Raman lidar in conjunction with Sun photometer data measured profiles of particle extinction; ground-based in situ data of aerosol optical properties were collected by nephelometer and absorption photometer. Exceptionally high values of aerosol optical depth of up to 1.5 were observed. The measurements were input to a radiative transfer model, which simulated high solar radiative forcing values for the aerosol pa…
Dust mobilization and transport in the northern Sahara during SAMUM 2006 – a meteorological overview
The SAMUM field campaign in southern Morocco in May/June 2006 provides valuable data to study the emission, and the horizontal and vertical transports of mineral dust in the Northern Sahara. Radiosonde and lidar observations show differential advection of air masses with different characteristics during stable nighttime conditions and up to 5-km deep vertical mixing in the strongly convective boundary layer during the day. Lagrangian and synoptic analyses of selected dust periods point to a topographic channel from western Tunisia to central Algeria as a dust source region. Significant emission events are related to cold surges from the Mediterranean in association with eastward passing upp…
Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China
Abstract During the “Program of Regional Integrated Experiments of Air Quality over Pearl River Delta 2004 (PRIDE-PRD2004)” hygroscopic properties of particles in the diameter range 22 nm to 10 μ m were determined. For that purpose, a Humidifying Differential Mobility Particle Sizer (H-DMPS) and a Micro-Orifice Uniform Deposition Impactor (MOUDI) were operated. The derived size-dependent particle hygroscopic growth factors were interpolated to ambient relative humidity (RH) and used to calculate the particle number size distributions (PNSDs) at ambient conditions. A comparison between the modeled particle extinction coefficients ( σ ext , Mie ) and those observed with a Raman lidar was made…
EARLINET observations of the 14-22-may long-range dust transport event during SAMUM 2006: validation of results from dust transport modelling
We observed a long-range transport event of mineral dust from North Africa to South Europe during the Saharan Mineral Dust Experiment (SAMUM) 2006. Geometrical and optical properties of that dust plume were determined with Sun photometer of the Aerosol Robotic Network (AERONET) and Raman lidar near the North African source region, and with Sun photometers of AERONET and lidars of the European Aerosol Research Lidar Network (EARLINET) in the far field in Europe. Extinction-to-backscatter ratios of the dust plume over Morocco and Southern Europe do not differ. Ångstr¨om exponents increase with distance from Morocco. We simulated the transport, and geometrical and optical properties of the dus…
Vertical profiling of Saharan dust with Raman lidars and airborne HSRL in southern Morocco during SAMUM
Three groundâÂ�Â�based Raman lidars and an airborne highâÂ�Â�spectralâÂ�Â�resolution lidar (HSRL) were operated during SAMUM 2006 in southern Morocco to measure height profiles of the volume extinction coefficient, the extinctionâÂ�Â�toâÂ�Â�backscatter ratio, and the depolarization ratio of dust particles in the Saharan dust layer at several wavelengths. Aerosol Robotic Network (AERONET) Sun photometer observations and radiosounding of meteorological parameters complemented the groundâÂ�Â�based activities at the SAMUM station of Ouarzazate. Four case studies are presented. Two case studies deal with the comparison of observations of the three groundâÂ�Â�based lidars during a heavy du…
Regional Saharan dust modelling during the SAMUM 2006 campaign
The regional dust model system LM-MUSCAT-DES was developed in the framework of the SAMUM project. Using the unique comprehensive data set of near-source dust properties during the 2006 SAMUM field campaign, the performance of the model system is evaluated for two time periods in May and June 2006. Dust optical thicknesses, number size distributions and the position of the maximum dust extinction in the vertical profiles agree well with the observations. However, the spatio-temporal evolution of the dust plumes is not always reproduced due to inaccuracies in the dust source placement by the model. While simulated winds and dust distributions are well matched for dust events caused by dry syn…
Spectral surface albedo over Morocco and its impact on radiative forcing of Saharan dust
In May–June 2006, airborne and ground-based solar (0.3–2.2 μm) and thermal infrared (4–42 μm) radiation measurements have been performed in Morocco within the Saharan Mineral Dust Experiment (SAMUM). Upwelling and downwelling solar irradiances have been measured using the Spectral Modular Airborne Radiation Measurement System (SMART)-Albedometer. With these data, the areal spectral surface albedo for typical surface types in southeastern Morocco was derived from airborne measurements for the first time. The results are compared to the surface albedo retrieved from collocated satellite measurements, and partly considerable deviations are observed. Using measured surface and atmospheric prope…
Vertical profiling of convective dust plumes in southern Morocco during SAMUM
Lifting of dust particles by dust devils and convective plumes may significantly contribute to the global mineral dust budget. During the Saharan Mineral Dust Experiment (SAMUM) in May–June 2006 vertical profiling of dusty plumes was performed for the first time. Polarization lidar observations taken at Ouarzazate (30.9°N, 6.9°W, 1133 m height above sea level) are analyzed. Two cases with typical and vigorous formation of convective plumes and statistical results of 5 d are discussed. The majority of observed convective plumes have diameters on order of 100–400 m. Most of the plumes (typically 50–95%) show top heights <1 km or 0.3DLH with the Saharan dust layer height DLH of typically 3–…
Depolarization�ratio profiling at several wavelengths in pure Saharan dust during SAMUM 2006
Vertical profiles of the linear particle depolarization ratio of pure dust clouds were measured during the Saharan Mineral Dust Experiment (SAMUM) at Ouarzazate, Morocco (30.9°N, –6.9°E), close to source regions in May–June 2006, with four lidar systems at four wavelengths (355, 532, 710 and 1064 nm). The intercomparison of the lidar systems is accompanied by a discussion of the different calibration methods, including a new, advanced method, and a detailed error analysis. Over the whole SAMUM periode pure dust layers show a mean linear particle depolarization ratio at 532 nm of 0.31, in the range between 0.27 and 0.35, with a mean Ångström exponent (AE, 440–870 nm) of 0.18 (range 0.04–0.34…
Influence of Saharan dust on cloud glaciation in southern Morocco during the Saharan Mineral Dust Experiment
[1] Multiwavelength lidar, Sun photometer, and radiosonde observations were conducted at Ouarzazate (30.9°N, 6.9°W, 1133 m above sea level, asl), Morocco, in the framework of the Saharan Mineral Dust Experiment (SAMUM) in May–June 2006. The field site is close to the Saharan desert. Information on the depolarization ratio, backscatter and extinction coefficients, and lidar ratio of the dust particles, estimates of the available concentration of atmospheric ice nuclei at cloud level, profiles of temperature, humidity, and the horizontal wind vector as well as backward trajectory analysis are used to study cases of cloud formation in the dust with focus on heterogeneous ice formation. Surpris…