0000000000181642
AUTHOR
J. Marganiec
Exclusive measurements of nuclear breakup reactions of 17Ne
F. Wamers et al.; 4 pags.; 2 figs. Open Access funded by Creative Commons Atribution Licence 2.0
Comparison of electromagnetic and nuclear dissociation of Ne-17
8 pags., 10 figs., 3 tabs.
New measurement of the 242Pu(n,γ) cross section at n-TOF-EAR1 for MOX fuels: Preliminary results in the RRR
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with 238U to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. The use of MOX fuels in thermal and fast reactors requires accurate capture and fission cross sections. For the particular case of 242Pu, the previous neutron capture cross section measurements were made in the 70’s, providing an uncertainty of about 35% in the keV region. In this context, the Nuclear Energy Agency recommends in its “High Priority Request List” and its report WPEC-26 that the capture cross section of 242Pu…
Thermonuclear reactionS30(p,γ)Cl31studied via Coulomb breakup ofCl31
Coulomb breakup at high energy in inverse kinematics of proton-rich Cl-31 was used to constrain the thermonuclear S-30(p,gamma)Cl-31 capture reaction rate under typical Type I x-ray burst conditions. This reaction is a bottleneck during rapid proton-capture nucleosynthesis (rp process), where its rate depends predominantly on the nuclear structure of Cl-31. Two low-lying states just above the proton-separation threshold of S-p = 296( 50) keV in Cl-31 have been identified experimentally using the (RB)-B-3-LAND setup at the GSI Helmholtzzentrum fur Schwerionenforschung GmbH. Both states are considered to play a key role in the thermonuclear S-30( p,gamma)Cl-31 capture reaction. Excitation ene…
First Measurement of Severalβ-Delayed Neutron Emitting Isotopes BeyondN=126
The β-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with β-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N≳126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the β-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.
7Be(n,α) and 7Be(n,p) cross-section measurement for the cosmological lithium problem at the n-TOF facility at CERN
One of the most puzzling problems in Nuclear Astrophysics is the “Cosmological Lithium Problem”, i.e the discrepancy between the primordial abundance of \(^{7}\)Li observed in metal poor halo stars (Asplund et al. in Astrophys J 644:229–259, 2006, [1]), and the one predicted by Big Bang Nucleosynthesis (BBN). One of the reactions that could have an impact on the problem is \(^{7}\)Be(n,p)\(^{7}\)Li. Despite of the importance of this reaction in BBN, the cross-section has never been directly measured at the energies of interest for BBN. Taking advantage of the innovative features of the second experimental area at the n\(\_\)TOF facility at CERN (Sabate-Gilarte et al. in Eur Phys J A 53:210,…
GEANT4 simulation of the neutron background of the C6D6 set-up for capture studies at n_TOF
The neutron sensitivity of the C6D6 detector setup used at n_TOF facility for capture measurements has been studied by means of detailed GEANT4 simulations. A realistic software replica of the entire n_TOF experimental hall, including the neutron beam line, sample, detector supports and the walls of the experimental area has beeni mplemented in the simulations. The simulations have been analyzed in the same manner as experimental data, in particular by applying the Pulse Height Weighting Technique. The simulations have been validated against a measurement of the neutron background performed with anatC sample, showing an excellent agreement above 1 keV. At lower energies, an additional compo…
The n_TOF facility: Neutron beams for challenging future measurements at CERN
The CERN n TOF neutron beam facility is characterized by a very high instantaneous neutron flux, excellent TOF resolution at the 185 m long flight path (EAR-1), low intrinsic background and coverage of a wide range of neutron energies, from thermal to a few GeV. These characteristics provide a unique possibility to perform high-accuracy measurements of neutron-induced reaction cross-sections and angular distributions of interest for fundamental and applied Nuclear Physics. Since 2001, the n TOF Collaboration has collected a wealth of high quality nuclear data relevant for nuclear astrophysics, nuclear reactor technology, nuclear medicine, etc. The overall efficiency of the experimental prog…
Approaching the precursor nuclei of the third r-process peak with RIBs
The rapid neutron nucleosynthesis process involves an enormous amount of very exotic neutron-rich nuclei, which represent a theoretical and experimental challenge. Two of the main decay properties that affect the final abundance distribution the most are half-lives and neutron branching ratios. Using fragmentation of a primary $^{238}$U beam at GSI we were able to measure such properties for several neutron-rich nuclei from $^{208}$Hg to $^{218}$Pb. This contribution provides a short update on the status of the data analysis of this experiment, together with a compilation of the latest results published in this mass region, both experimental and theoretical. The impact of the uncertainties …
Neutron capture cross section measurements for nuclear astrophyisics at CERN n_TOF
A series of neutron capture cross section measurements of interest to nuclear astrophysics have been recently performed at n_TOF, the neutron spallation source operating at CERN. The low repetition frequency of the proton beam driver, the extremely high instantaneous neutron flux, and the low background conditions in the experimental area are optimal for capture cross section measurements on low-mass or radioactive samples. An overview of the measurements performed during the two experimental campaigns in 2002 and 2003 is presented with special emphasis on the measurement of the capture cross sections of the Os isotopes relevant for the cosmochronology based on the Re/Os clock. http://www.s…
Neutron measurements for advanced nuclear systems: The n_TOF project at CERN
A few years ago, the neutron time-of-flight facility n_TOF was built at CERN to address some of the urgent needs of high-accuracy nuclear data for Accelerator Driven Systems and other advanced nuclear energy systems, as well as for nuclear astrophysics and fundamental nuclear physics. Thanks to the characteristics of the neutron beam, and to state-of-the-art detection and acquisition systems, high quality neutron cross-section data have been obtained for a variety of isotopes, many of which radioactive. Following an important upgrade of the spallation target and of the experimental area, a new measurement campaign has started last year. After a brief review of the most important results obt…
Be7(n,α)He4Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN
The energy-dependent cross section of the (7)Bed(n,alpha)He-4 reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. The challenges posed by the short half-life of Be-7 and by the low reaction cross section have been overcome at n_TOF thanks to an unprecedented combination of the extremely high luminosity and good resolution of the neutron beam in the new experimental area (EAR2) of the n_TOF facility at CERN, the availability of a sufficient amount of chemically pure Be-7, and a specifically designed experimental setup. Coincidences between the two alpha particles have been…
Neutron cross section measurements at n_TOF for ADS related estudies
A neutron Time-of-Flight facility (n_TOF) is available at CERN since 2001. The innovative features of the neutron beam, in particular the high instantaneous flux, the wide energy range, the high resolution and the low background, make this facility unique for measurements of neutron induced reactions relevant to the field of Emerging Nuclear Technologies, as well as to Nuclear Astrophysics and Fundamental Nuclear Physics. The scientific motivations that have led to the construction of this new facility are here presented. The main characteristics of the n_TOF neutron beam are described, together with the features of the experimental apparata used for cross-section measurements. The main res…
Neutron capture cross section measurement ofU238at the CERN n_TOF facility in the energy region from 1 eV to 700 keV
The aim of this work is to provide a precise and accurate measurement of the U238(n,γ) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the u…
The Nuclear astrophysics program at n_TOF (CERN)
An important experimental program on Nuclear Astrophysics is being carried out at the n_TOF since several years, in order to address the still open issues in stellar and primordial nucleosynthesis. Several neutron capture reactions relevant to s-process nucleosynthesis have been measured so far, some of which on important branching point radioisotopes. Furthermore, the construction of a second experimental area has recently opened the way to challenging measurements of (n, charged particle) reactions on isotopes of short half-life. The Nuclear Astrophysics program of the n_TOF Collaboration is here described, with emphasis on recent results relevant for stellar nucleosynthesis, stellar neut…
Study of the $^{15}$O(2p, γ )$^{17}$Ne cross section by Coulomb dissociation of $^{17}$Ne for the rp process of nucleosynthesis
Acta physica Polonica / B 45(2), 229 - 234 (2014). doi:10.5506/APhysPolB.45.229
The 33S(n,α)30Si cross section measurement at n TOF-EAR2 (CERN): From 0.01 eV to the resonance region
The 33S(n,α)30Si cross section measurement, using 10B(n,α) as reference, at the n TOF Experimental Area 2 (EAR2) facility at CERN is presented. Data from 0.01 eV to 100 keV are provided and, for the first time, the cross section is measured in the range from 0.01 eV to 10 keV. These data may be used for a future evaluation of the cross section because present evaluations exhibit large discrepancies. The 33S(n,α)30Si reaction is of interest in medical physics because of its possible use as a cooperative target to boron in Neutron Capture Therapy (NCT).
Measurement of the Pu-242(n,gamma) cross section from thermal to 500 keV at the Budapest research reactor and CERN n_TOF-EAR1 facilities
The design and operation of innovative nuclear systems requires a better knowledge of the capture and fission cross sections of the Pu isotopes. For the case of capture on 242Pu, a reduction of the uncertainty in the fast region down to 8-12% is required. Moreover, aiming at improving the evaluation of the fast energy range in terms of average parameters, the OECD NEA High Priority Request List (HPRL) requests high-resolution capture measurements with improved accuracy below 2 keV. The current uncertainties also affect the thermal point, where previous experiments deviate from each other by 20%. A fruitful collaboration betwen JGU Mainz and HZ Dresden-Rossendorf within the EC CHANDA project…
Experimental study of the 15O(2p, γ)17Ne cross section by Coulomb Dissociation for the rp process
6th Nuclear Physics in Astrophysics Conference (NPA), Lisbon, Portugal, 19 May 2013 - 24 May 2013; Journal of physics / Conference Series 665, 012046 (2016). doi:10.1088/1742-6596/665/1/012046
Experimental neutron capture data of 58Ni from the CERN n_TOF facility
The $^{58}$Ni $(n,\gamma)$ cross section has been measured at the neutron time of flight facility n_TOF at CERN, in the energy range from 27 meV up to 400 keV. In total, 51 resonances have been analyzed up to 122 keV. Maxwellian averaged cross sections (MACS) have been calculated for stellar temperatures of kT$=$5-100 keV with uncertainties of less than 6%, showing fair agreement with recent experimental and evaluated data up to kT = 50 keV. The MACS extracted in the present work at 30 keV is 34.2$\pm$0.6$_\mathrm{stat}\pm$1.8$_\mathrm{sys}$ mb, in agreement with latest results and evaluations, but 12% lower relative to the recent KADoNIS compilation of astrophysical cross sections. When in…
β -decay half-lives and β -delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126
Background: Previous measurements of Beta-delayed neutron emitters comprise around 230 nuclei, spanning from the 8He up to 150La. Apart from 210Tl, with a minuscule branching ratio of 0.07%, no other neutron emitter is measured yet beyond A = 150. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at A 195. Purpose: To measure both, Beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond N = 126. Method: Ions of interest are produced by fragmentation of a 238U beam, selected and identifed via the GSI-FRS fra…
Nuclear Data for the Thorium Fuel Cycle and the Transmutation of Nuclear Waste
Neutron-induced reaction cross sections play an important role in a wide variety of research fields, ranging from stellar nucleosynthesis, the investigation of nuclear level density studies, to applications of nuclear technology, including the transmutation of nuclear waste, accelerator-driven systems, and nuclear fuel cycle investigations. Simulations of nuclear technology applications largely rely on evaluated nuclear data libraries. These libraries are based both on experimental data and theoretical models. An outline of experimental nuclear data activities at CERN’s neutron time-of-flight facility, n_TOF, will be presented.
The 236U neutron capture cross-section measured at the n TOF CERN facility
International audience; The $^{236}$U isotope plays an important role in nuclear systems, both for future and currently operating ones. The actual knowledge of the capture reaction of this isotope is satisfactory in the thermal region, but it is considered insufficient for Fast Reactor and ADS applications. For this reason the $^{236} \text{U}(n, \gamma)$ reaction cross-section has been measured for the first time in the whole energy region from thermal energy up to 1 MeV at the n_TOF facility with two different detection systems: an array of C$_6$D$_6$ detectors, employing the total energy deposited method, and a 4$\pi$ total absorption calorimeter (TAC), made of 40 BaF$_2$ crystals. The t…
High precision measurement of the radiative capture cross section of 238U at the n_TOF CERN facility
The importance of improving the accuracy on the capture cross-section of 238U has been addressed by the Nuclear Energy Agency, since its uncertainty significantly affects the uncertainties of key design parameters for both fast and thermal nuclear reactors. Within the 7th framework programme ANDES of the European Commission three different measurements have been carried out with the aim of providing the 238U(n,γ) cross-section with an accuracy which varies from 1 to 5%, depending on the energy range. Hereby the final results of the measurement performed at the n-TOF CERN facility in a wide energy range from 1 eV to 700 keV will be presented. © The Authors, published by EDP Sciences, 2017.
Fission fragment angular distribution of 232Th(n,f) at the CERN n TOF facility
The angular distribution of fragments emitted in neutron-induced fission of 232Th was measured in the white spectrum neutron beam at the n_TOF facility at CERN. A reaction chamber based on Parallel Plate Avalanche Counters (PPAC) was used, where the detectors and the targets have been tilted 45 degrees with respect to the neutron beam direction in order to cover the full angular range of the fission fragments. A GEANT4 simulation has been developed to study the setup efficiency. The data analysis and the preliminary results obtained for the 232Th(n,f) between fission threshold and 100 MeV are presented here.
Radiative neutron capture on Pu242 in the resonance region at the CERN n_TOF-EAR1 facility
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluat…
The measurement programme at the neutron time-of-flight facility n_TOF at CERN
Neutron-induced reaction cross sections are important for a wide variety of research fields ranging from the study of nuclear level densities, nucleosynthesis to applications of nuclear technology like design, and criticality and safety assessment of existing and future nuclear reactors, radiation dosimetry, medical applications, nuclear waste transmutation, accelerator-driven systems and fuel cycle investigations. Simulations and calculations of nuclear technology applications largely rely on evaluated nuclear data libraries. The evaluations in these libraries are based both on experimental data and theoretical models. CERN’s neutron time-of-flight facility n TOF has produced a considerabl…
Measurement of the 151Sm n,gamma 152Sm cross section at n_TOF
The 151 Sm(n, γ ) 152 Sm cross section, which is important for the interpretation of the 151 Sm branching as an s -process thermometer, was measured from 1 eV up to 1 MeV at the innovative n_TOF facility at CERN. Based on these data, the Maxwellian-averaged cross section at k T = 30 keV is found to be 3100±160 mb. This value can be used to constrain the thermodynamical conditions in Asymptotic Giant Branch (AGB) stars during He-shell burning.
β-delayed neutron emission measurements around the third r-process abundance peak
This contribution summarizes an experiment performed at GSI (Germany) in the neutron-rich region beyond N=126. The aim of this measurement is to provide the nuclear physics input of relevance for r-process model calculations, aiming at a better understanding of the third r-process abundance peak. Many exotic nuclei were measured around 211Hg and 215Tl. Final ion identification diagrams are given in this contribution. For most of them, we expect to derive halflives and and β-delayed neutron emission probabilities. The detectors used in this experiment were the Silicon IMplantation and Beta Absorber (SIMBA) detector, based on an array of highly segmented silicon detectors, and the BEta deLayE…
Coulomb dissociation of P 27 at 500 MeV/u
J. Marganiec et al. ; 15 págs.; 14 figs.; 6 tabs.
First Observation of the Unbound NucleusNe15
We report on the first observation of the unbound proton-rich nucleus Ne-15. Its ground state and first excited state were populated in two-neutron knockout reactions from a beam of 500 MeV/u Ne-17. The Ne-15 ground state is found to be unbound by 2.522(66) MeV. The decay proceeds directly to O-13 with simultaneous two-proton emission. No evidence for sequential decay via the energetically allowed 2(-) and 1(-) states in F-14 is observed. The Ne-15 ground state is shown to have a strong configuration with two protons in the (sd) shell around O-13 with a 63(5)% (1s(1/2))(2) component.
Measurement of the 241Am neutron capture cross section at the n-TOF facility at CERN
New neutron cross section measurements of minor actinides have been performed recently in order to reduce the uncertainties in the evaluated data, which is important for the design of advanced nuclear reactors and, in particular, for determining their performance in the transmutation of nuclear waste. We have measured the 241 Am(n,γ) cross section at the n TOF facility between 0.2 eV and 10 keV with a BaF2 Total Absorption Calorimeter, and the analysis of the measurement has been recently concluded. Our results are in reasonable agreement below 20 eV with the ones published by C. Lampoudis et al. in 2013, who reported a 22% larger capture cross section up to 110 eV compared to experimental …
Nuclear data activities at the n_TOF facility at CERN
International audience; Nuclear data in general, and neutron-induced reaction cross sections in particular, are important for a wide variety of research fields. They play a key role in the safety and criticality assessment of nuclear technology, not only for existing power reactors but also for radiation dosimetry, medical applications, the transmutation of nuclear waste, accelerator-driven systems, fuel cycle investigations and future reactor systems as in Generation IV. Applications of nuclear data are also related to research fields as the study of nuclear level densities and stellar nucleosynthesis. Simulations and calculations of nuclear technology applications largely rely on evaluate…
β-decay and β-delayed Neutron Emission Measurements at GSI-FRS Beyond N=126, for r-process Nucleosynthesis
New measurements of very exotic nuclei in the neutron-rich region beyond N=126 have been performed at the GSI facility with the fragment separator (FRS). The aim of the experiment is to determine half-lives and β-delayed neutron emission branching ratios of isotopes of Hg, Tl and Pb in this region. This contribution summarizes final counting statistics for identification and for implantation, as well as the present status of the data analysis of the half-lives. In summary, isotopes of Pt, Au, Hg, Tl, Pb, Bi, Po, At, Rn and Fr were clearly identified and several of them (208-211Hg, 211-215Tl, 214-218Pb) were implanted with enough statistics to determine their half-lives. About half of them a…
Measurements of the 90,91,92,94,96 Zr n, gamma cross-sections at n_TOF
Neutron capture cross sections of the 90,91,92,94,96Zr have been measured over the energy range from 1 eV to 1 MeV at the spallation neutron facility n TOF at CERN in 2003. The innovative features of the neutron beam, in particular the high instantaneous flux, the high energy resolution and low background, together with improvements of the neutron sensitivity of the capture detectors make this facility unique for neutron-induced reaction cross section measurements with much improved accuracy. The preliminary results of the Zr measurements show capture resonance strengths generally smaller than in previous measurements. Peer Reviewed
Coulomb and nuclear excitations of narrow resonances in 17Ne
Physics letters / B 759, 200 - 205 (2016). doi:10.1016/j.physletb.2016.05.073