0000000000236019

AUTHOR

Thomas Thundat

0000-0003-1721-1181

showing 10 related works from this author

Effects of temperature and pressure on microcantilever resonance response.

2003

Abstract The variation in resonance response of microcantilevers was investigated as a function of pressure (10 −2 –10 6  Pa) and temperature (290–390 K) in atmospheres of helium (He) and dry nitrogen (N 2 ). Our results for a silicon cantilever under vacuum show that the frequency varies in direct proportion to the temperature. The linear response is explained by the decrease in Young's modulus with increasing the temperature. However, when the cantilever is bimaterial, the response is nonlinear due to differential thermal expansion. Resonance response as a function of pressure shows three different regions, which correspond to molecular flow regime, transition regime, and viscous regime. …

CantileverChemistryMean free pathThermodynamicschemistry.chemical_elementYoung's modulusMolecular physicsAtomic and Molecular Physics and OpticsThermal expansionElectronic Optical and Magnetic Materialssymbols.namesakeFree molecular flowDeflection (engineering)symbolsKnudsen numberInstrumentationHeliumUltramicroscopy
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Probing large area surface plasmon interference in thin metal films using photon scanning tunneling microscopy.

2003

Abstract The interference of surface plasmons can provide important information regarding the surface features of the hosting thin metal film. We present an investigation of the interference of optically excited surface plasmons in the Kretschmann configuration in the visible spectrum. Large area surface plasmon interference regions are generated at several wavelengths and imaged with the photon scanning tunneling microscope. Furthermore, we discuss the non-retarded dispersion relations for the surface plasmons in the probe–metal system modeled as confocal hyperboloids of revolution in the spheroidal coordinate systems.

Materials sciencebusiness.industryScanning tunneling spectroscopySurface plasmonPhysics::OpticsSpin polarized scanning tunneling microscopyAtomic and Molecular Physics and OpticsElectrochemical scanning tunneling microscopeElectronic Optical and Magnetic Materialslaw.inventionScanning probe microscopyOpticsInterference (communication)lawScanning tunneling microscopebusinessInstrumentationLocalized surface plasmonUltramicroscopy
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Microscale Marangoni actuation: All-optical and all-electrical methods

2006

We present experimental results from an all-optical microfluidic platform that may be complimented by a thin film all-electrical network. Using these configurations we have studied the microfluidic convective flow systems of silicone oil, glycerol, and 1,3,5-trinitrotoluene on open surfaces through the production of surface tension gradients derived from thermal gradients. We show that sufficient localized thermal variation can be created utilizing surface plasmons and/or engaging individually addressable resistive thermal elements. Both studies manipulate fluids via Marangoni forces, each having their unique exploitable advantages. Surface plasmon excitation in metal foils are the driving …

GlycerolResistive touchscreenHot TemperatureMaterials scienceMarangoni effectSurface PropertiesMicrofluidicsSurface plasmonNanotechnologyMicroscopy Scanning ProbeAtomic and Molecular Physics and OpticsElectronic Optical and Magnetic MaterialsSurface tensionThermalSilicone OilsInstrumentationMicroscale chemistryPlasmonTrinitrotolueneUltramicroscopy
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Measurement of Mechanical Properties of Cantilever Shaped Materials

2008

Microcantilevers were first introduced as imaging probes in Atomic Force Microscopy (AFM) due to their extremely high sensitivity in measuring surface forces. The versatility of these probes, however, allows the sensing and measurement of a host of mechanical properties of various materials. Sensor parameters such as resonance frequency, quality factor, amplitude of vibration and bending due to a differential stress can all be simultaneously determined for a cantilever. When measuring the mechanical properties of materials, identifying and discerning the most influential parameters responsible for the observed changes in the cantilever response are important. We will, therefore, discuss the…

CantileverMechanical engineeringReviewBendinglcsh:Chemical technologyBiochemistrymaterialsAnalytical ChemistryStress (mechanics)stresspressuresensorResidual stressgaslcsh:TP1-1185Electrical and Electronic EngineeringComposite materialInstrumentationContinuum mechanicsChemistrySurface forcetemperatureMicrocantileverAtomic and Molecular Physics and OpticsVibrationageingMaterial propertiesenvironmentmechanicsSensors
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Imaging standing surface plasmons by photon tunneling

2005

We present a direct method for optically exciting and imaging delocalized standing surface plasmons in thin metal films. We show theoretically that when imaging the field of the plasmons with a photon scanning tunneling microscope, the presence of the dielectric probe has a negligible effect on the surface modes of the metal film. We demonstrate that plasmon interference can be sustained in arbitrarily large regions of the metal film in comparison to the excitation wavelength. This knowledge can be important when seeking the relative distance between two scattering centers such as the presence of micron or submicron structures.

PhotonMaterials sciencebusiness.industryScatteringSurface plasmonPhysics::OpticsDielectricCondensed Matter PhysicsElectronic Optical and Magnetic Materialslaw.inventionDelocalized electronOpticslawQuasiparticleOptoelectronicsScanning tunneling microscopebusinessPlasmonPhysical Review B
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Activation process of reversible Pd thin film hydrogen sensors

2013

Abstract Microcantilever-based thin film palladium hydrogen sensors have high selectivity and sensitivity. Reproducibility and accuracy of the sensor performance depend on the activation process of the polycrystalline palladium film deposited on the cantilever. When the hydrogen is in solid solution ( α -phase), the cantilever bending is mostly governed by the residual film stress induced by the swelling at the grain boundaries in the film. When the palladium hydride ( β -phase) starts to be formed, the cantilever undergoes a large deflection due to hydrogen absorption-induced film swelling (10% change in volume). Differences in the phase diagrams of the palladium hydride for two film thick…

Materials scienceCantileverHydrogenMetals and AlloysAnalytical chemistrychemistry.chemical_elementPalladium hydrideCondensed Matter PhysicsHydrogen sensorSurfaces Coatings and FilmsElectronic Optical and Magnetic Materialschemistry.chemical_compoundchemistryResidual stressPhase (matter)Materials ChemistryElectrical and Electronic EngineeringThin filmComposite materialInstrumentationPalladiumSensors and Actuators B: Chemical
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Surface plasmon assisted thermal coupling of multiple photon energies

2006

A novel optical effect can be observed in a thin gold foil due to the excitation of surface plasmons which permits a form of all-optical modulation at low pulse rates. Modulated excitation of surface plasmons by infrared photons is shown to couple to several beams at visible-photon energies. The coupling is manifested by the observation of the visible photons being pulsed by the action of the infrared pulses, and by the far field diffraction of the visible beams into concentric rings. When each visible beam also excites surface plasmons, then a quadratic dependence of the visible photon power upon the infrared incident power is measured. The decay of surface plasmons is implicated as the pr…

DiffractionPulse repetition frequencyPhotonInfraredbusiness.industryChemistrySurface plasmonMetals and AlloysPhysics::OpticsNear and far fieldOptical polarizationSurfaces and InterfacesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsOpticsMaterials ChemistrybusinessExcitationThin Solid Films
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Visible photothermal deflection spectroscopy using microcantilevers

2012

International audience; Photothermal deflection spectroscopy based on bi-material cantilevers combines the sensitivity of miniature sensors and the selectivity of optical spectroscopy. In this paper, we report on the photothermal response of the microcantilevers functionalized with nanometer thin organic films in the visible region. Unlike responses in the infrared regime, in the optical region, light absorption by all the cantilever constituents must be considered for extraction of the physical parameters of the organic layer. A model of photothermal deflection for the optical region has been developed for two absorbing layers consisting of a thick metal (>200 nm) and a thin organic film. …

Materials scienceCantileverADSORPTIONInfrared02 engineering and technologyDEVICE01 natural sciencesRhodamine 6Gchemistry.chemical_compoundUltraviolet visible spectroscopyOptics0103 physical sciencesMaterials ChemistrySENSORSElectrical and Electronic EngineeringThin filmSpectroscopyInstrumentation010302 applied physicsThin layersbusiness.industryFORCE MICROSCOPYMetals and AlloysPhotothermal therapyPERFORMANCE021001 nanoscience & nanotechnologyCondensed Matter PhysicsSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsCANTILEVERchemistryENHANCED RAMAN-SPECTROSCOPY0210 nano-technologybusinessRHODAMINE 6G
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Curvature effects in surface plasmon dispersion and coupling

2005

We have studied the resonant coupling of surface plasmons in curved thin-film tunneling geometries by obtaining the dispersion relations for the system. The surface plasmon dispersion relations are calculated for a metal-coated dielectric probe above a dielectric half space with and without metal coating. The system is modeled in the prolate spheroidal system, and the dispersion relations are studied as functions of the parameter that defines the boundaries of the tip and the corresponding coating, and as functions of the involved coating thicknesses. Using this type of probe-substrate configuration, the nonradiative surface plasmon coupling mechanism is investigated in the visible spectrum…

Materials sciencebusiness.industrySurface plasmonPhysics::OpticsDielectricCondensed Matter PhysicsMolecular physicsSurface plasmon polaritonElectronic Optical and Magnetic MaterialsScanning probe microscopyOpticsDispersion relationDispersion (optics)Surface plasmon resonancebusinessLocalized surface plasmonPhysical Review B
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Observation of Knudsen effect with microcantilevers

2003

The Knudsen effect is estimated theoretically and observed experimentally using a U-shaped silicon microcantilever. Though Knudsen forces are extremely small in most cases involving microcantilevers, there exist situations where these forces can be significant and may be important in atomic force microscopy and in microelectromechanical systems (MEMS). The criteria for the presence of Knudsen forces are outlined and an analytical expression in the form of a linear function of the pressure is given for the force in the free molecular regime. The experimental results display peaks in the transitional regime while varying linearly in the molecular regime.

Microelectromechanical systemsMicroscopeSiliconAtomic force microscopyAnalytical chemistrychemistry.chemical_elementMechanicsAtomic and Molecular Physics and OpticsLinear functionComputer Science::OtherElectronic Optical and Magnetic Materialslaw.inventionKnudsen flowchemistryFree molecular flowlawKnudsen numberInstrumentationUltramicroscopy
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