7Be(n,α) and 7Be(n,p) cross-section measurement for the cosmological lithium problem at the n-TOF facility at CERN

One of the most puzzling problems in Nuclear Astrophysics is the “Cosmological Lithium Problem”, i.e the discrepancy between the primordial abundance of \(^{7}\)Li observed in metal poor halo stars (Asplund et al. in Astrophys J 644:229–259, 2006, [1]), and the one predicted by Big Bang Nucleosynthesis (BBN). One of the reactions that could have an impact on the problem is \(^{7}\)Be(n,p)\(^{7}\)Li. Despite of the importance of this reaction in BBN, the cross-section has never been directly measured at the energies of interest for BBN. Taking advantage of the innovative features of the second experimental area at the n\(\_\)TOF facility at CERN (Sabate-Gilarte et al. in Eur Phys J A 53:210,…

Neutron transmission measurements at nELBE

International Conference on Nuclear Data for Science and Technology, ND 2019, Bejing, China, 19 May 2019 - 24 May 2019; The European physical journal / Web of Conferences 239, 01006 (2020). doi:10.1051/epjconf/202023901006

Determination of the Bi209(n,γ)Bi210g cross section using the NICE detector

The capture cross section of $^{209}\mathrm{Bi}(n,\ensuremath{\gamma})^{210g}\mathrm{Bi}$ was measured at different astrophysically relevant energies including thermal capture cross section (25 meV), resonance integral, and the Maxwellian averaged cross section at a thermal energy of $kT=30$ keV. The partial capture cross section $({\ensuremath{\sigma}}_{g})$ was determined using the activation technique and by measuring the $^{210}\mathrm{Po}$ activity. The newly developed and tested NICE detector setup was used to measure the $\ensuremath{\alpha}$ activity of the $^{210}\mathrm{Po}$. Using this setup the thermal and resonance integral cross sections were determined to be $16.2\phantom{\ru…

Measurement of the92,93,94,100Mo(γ,n) reactions by Coulomb Dissociation

6th Nuclear Physics in Astrophysics Conference (NPA), Lisbon, Portugal, 19 May 2013 - 24 May 2013; Journal of physics / Conference Series 665, 012034 (2016). doi:10.1088/1742-6596/665/1/012034

Be7(n,α)He4Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN

The energy-dependent cross section of the (7)Bed(n,alpha)He-4 reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. The challenges posed by the short half-life of Be-7 and by the low reaction cross section have been overcome at n_TOF thanks to an unprecedented combination of the extremely high luminosity and good resolution of the neutron beam in the new experimental area (EAR2) of the n_TOF facility at CERN, the availability of a sufficient amount of chemically pure Be-7, and a specifically designed experimental setup. Coincidences between the two alpha particles have been…

The 33S(n,α)30Si cross section measurement at n TOF-EAR2 (CERN): From 0.01 eV to the resonance region

The 33S(n,α)30Si cross section measurement, using 10B(n,α) as reference, at the n TOF Experimental Area 2 (EAR2) facility at CERN is presented. Data from 0.01 eV to 100 keV are provided and, for the first time, the cross section is measured in the range from 0.01 eV to 10 keV. These data may be used for a future evaluation of the cross section because present evaluations exhibit large discrepancies. The 33S(n,α)30Si reaction is of interest in medical physics because of its possible use as a cooperative target to boron in Neutron Capture Therapy (NCT).

Measurement of the Pu-242(n,gamma) cross section from thermal to 500 keV at the Budapest research reactor and CERN n_TOF-EAR1 facilities

The design and operation of innovative nuclear systems requires a better knowledge of the capture and fission cross sections of the Pu isotopes. For the case of capture on 242Pu, a reduction of the uncertainty in the fast region down to 8-12% is required. Moreover, aiming at improving the evaluation of the fast energy range in terms of average parameters, the OECD NEA High Priority Request List (HPRL) requests high-resolution capture measurements with improved accuracy below 2 keV. The current uncertainties also affect the thermal point, where previous experiments deviate from each other by 20%. A fruitful collaboration betwen JGU Mainz and HZ Dresden-Rossendorf within the EC CHANDA project…

Nuclear Data for the Thorium Fuel Cycle and the Transmutation of Nuclear Waste

Neutron-induced reaction cross sections play an important role in a wide variety of research fields, ranging from stellar nucleosynthesis, the investigation of nuclear level density studies, to applications of nuclear technology, including the transmutation of nuclear waste, accelerator-driven systems, and nuclear fuel cycle investigations. Simulations of nuclear technology applications largely rely on evaluated nuclear data libraries. These libraries are based both on experimental data and theoretical models. An outline of experimental nuclear data activities at CERN’s neutron time-of-flight facility, n_TOF, will be presented.

The 236U neutron capture cross-section measured at the n TOF CERN facility

International audience; The $^{236}$U isotope plays an important role in nuclear systems, both for future and currently operating ones. The actual knowledge of the capture reaction of this isotope is satisfactory in the thermal region, but it is considered insufficient for Fast Reactor and ADS applications. For this reason the $^{236} \text{U}(n, \gamma)$ reaction cross-section has been measured for the first time in the whole energy region from thermal energy up to 1 MeV at the n_TOF facility with two different detection systems: an array of C$_6$D$_6$ detectors, employing the total energy deposited method, and a 4$\pi$ total absorption calorimeter (TAC), made of 40 BaF$_2$ crystals. The t…

High precision measurement of the radiative capture cross section of 238U at the n_TOF CERN facility

The importance of improving the accuracy on the capture cross-section of 238U has been addressed by the Nuclear Energy Agency, since its uncertainty significantly affects the uncertainties of key design parameters for both fast and thermal nuclear reactors. Within the 7th framework programme ANDES of the European Commission three different measurements have been carried out with the aim of providing the 238U(n,γ) cross-section with an accuracy which varies from 1 to 5%, depending on the energy range. Hereby the final results of the measurement performed at the n-TOF CERN facility in a wide energy range from 1 eV to 700 keV will be presented. © The Authors, published by EDP Sciences, 2017.

Fission fragment angular distribution of 232Th(n,f) at the CERN n TOF facility

The angular distribution of fragments emitted in neutron-induced fission of 232Th was measured in the white spectrum neutron beam at the n_TOF facility at CERN. A reaction chamber based on Parallel Plate Avalanche Counters (PPAC) was used, where the detectors and the targets have been tilted 45 degrees with respect to the neutron beam direction in order to cover the full angular range of the fission fragments. A GEANT4 simulation has been developed to study the setup efficiency. The data analysis and the preliminary results obtained for the 232Th(n,f) between fission threshold and 100 MeV are presented here.

Radiative neutron capture on Pu242 in the resonance region at the CERN n_TOF-EAR1 facility

The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluat…

The measurement programme at the neutron time-of-flight facility n_TOF at CERN

Neutron-induced reaction cross sections are important for a wide variety of research fields ranging from the study of nuclear level densities, nucleosynthesis to applications of nuclear technology like design, and criticality and safety assessment of existing and future nuclear reactors, radiation dosimetry, medical applications, nuclear waste transmutation, accelerator-driven systems and fuel cycle investigations. Simulations and calculations of nuclear technology applications largely rely on evaluated nuclear data libraries. The evaluations in these libraries are based both on experimental data and theoretical models. CERN’s neutron time-of-flight facility n TOF has produced a considerabl…

Measurement of the 241Am neutron capture cross section at the n-TOF facility at CERN

New neutron cross section measurements of minor actinides have been performed recently in order to reduce the uncertainties in the evaluated data, which is important for the design of advanced nuclear reactors and, in particular, for determining their performance in the transmutation of nuclear waste. We have measured the 241 Am(n,γ) cross section at the n TOF facility between 0.2 eV and 10 keV with a BaF2 Total Absorption Calorimeter, and the analysis of the measurement has been recently concluded. Our results are in reasonable agreement below 20 eV with the ones published by C. Lampoudis et al. in 2013, who reported a 22% larger capture cross section up to 110 eV compared to experimental …

Nuclear data activities at the n_TOF facility at CERN

International audience; Nuclear data in general, and neutron-induced reaction cross sections in particular, are important for a wide variety of research fields. They play a key role in the safety and criticality assessment of nuclear technology, not only for existing power reactors but also for radiation dosimetry, medical applications, the transmutation of nuclear waste, accelerator-driven systems, fuel cycle investigations and future reactor systems as in Generation IV. Applications of nuclear data are also related to research fields as the study of nuclear level densities and stellar nucleosynthesis. Simulations and calculations of nuclear technology applications largely rely on evaluate…

Thermal neutron capture cross section of the radioactive isotopeFe60

Background: Fifty percent of the heavy element abundances are produced via slow neutron capture reactions in different stellar scenarios. The underlying nucleosynthesis models need the input of neutron capture cross sections.Purpose: One of the fundamental signatures for active nucleosynthesis in our galaxy is the observation of long-lived radioactive isotopes, such as $^{60}\mathrm{Fe}$ with a half-life of $2.60\ifmmode\times\else\texttimes\fi{}{10}^{6}$ yr. To reproduce this $\ensuremath{\gamma}$ activity in the universe, the nucleosynthesis of $^{60}\mathrm{Fe}$ has to be understood reliably.Methods: An $^{60}\mathrm{Fe}$ sample produced at the Paul Scherrer Institut (Villigen, Switzerla…

Thermal (n,γ) cross section and resonance integral ofTm171