0000000000346100

AUTHOR

Alessandro Calabrese

showing 8 related works from this author

Sintesi di nuovi low molecular weight (LMW) hydrogelators fluorurati

2010

Settore CHIM/06 - Chimica OrganicaGels composti fluorurati ossadiazoli nanomateriali autoassemblanti
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Synthesis of fluorinated oxadiazoles with gelation and oxygen storage ability

2012

A new family of fluorinated low molecular weight (LMW) gelators has been synthesized through SNAr substitution of 5-polyfluoroaryl-3-perfluoroheptyl-1,2,4-oxadiazoles with glycine ester. The obtained compounds give thermal and pH-sensitive hydrogels or thermo-reversible organogels in DMSO. Oxygen solubility studies showed the ability to maintain high oxygen levels in solution and in gel blend with plate counter agar (PCA).

HalogenationOxygen storageGlycinechemistry.chemical_elementBiochemistryPhase TransitionNucleophilic aromatic substitutionOrganic chemistryDimethyl SulfoxidePhysical and Theoretical ChemistrySolubilityOxadiazolesHydrogen bondChemistryOrganic ChemistryHalogenationEstersHydrogen BondingFluorineSettore CHIM/06 - Chimica OrganicaHydrogen-Ion ConcentrationMolecular WeightOxygenSolubilityGlycineSelf-healing hydrogelsFluorineMicroscopy Electron Scanninglow molecular weight gelators(LMWG) oxadiazoles fluorinated compounds oxgyen carriersThermodynamicsGels
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Fluorescent Hg2+ Sensors: Synthesis and Evaluation of a Tren-Based Starburst Molecule Containing Fluorinated 1,2,4-Oxadiazoles.

2010

A new tren-based starburst molecule containing fluorinated 1,2,4-oxadiazoles as fluorophores has been synthesized and its sensing behavior toward several metal cations has been investigated by UV/Vis, fluorescence, 1 H NMR and 19 F NMR spectroscopy. Selective sensing for Hg 2+ ions through a PET-based mechanism was evidenced, suggesting application as fluorescent sensor for Hg 2+ of the off-on type.

FluorophoreStereochemistryOrganic ChemistryNuclear magnetic resonance spectroscopySettore CHIM/06 - Chimica OrganicaPhotochemistryFluorescenceChemical synthesischemistry.chemical_compoundElectron transferchemistryProton NMRMoleculePhysical and Theoretical ChemistrySelectivity124-Oxadiazoles Sensors Electron transfer Fluorinated ligands Mercury
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Synthesis of Fluorinated Bent-Core Mesogens (BCMs) Containing the 1,2,4-Oxadiazole Ring

2015

New fluorinated bent-core mesogens containing the 1,2,4-oxadiazole or 1,2,4-triazole nucleus have been synthesized taking advantage of the ANRORC (Addition of Nucleophile, Ring-Opening, Ring-Closure) reactivity of 5-perfluoroalkyl-1,2,4-oxadiazoles. Physical state changes of the obtained compounds were characterized through DSC, POM, and SAXS. Besides the formation of a smectic mesophase, a novel behavior as organic molecular glass was evidenced for some 1,2,4-oxadiazole derivatives.

Small-angle X-ray scatteringChemistryOrganic ChemistryBent molecular geometryMesophaseOxadiazole02 engineering and technology010402 general chemistry021001 nanoscience & nanotechnologyRing (chemistry)01 natural sciences0104 chemical sciencesCore (optical fiber)chemistry.chemical_compoundNucleophilePolymer chemistryReactivity (chemistry)0210 nano-technologyJournal of Heterocyclic Chemistry
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Uncatalyzed photofunctionalization of C-H bonds

2010

Settore CHIM/06 - Chimica Organicaphotochemistry C-C bond formation olefins functionization
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Sintesi di nuovi bent-core LC fluorurati

2011

Oxadiazoles fluorinated compounds liquid crystalsSettore CHIM/06 - Chimica Organica
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Sintesi di composti eterociclici fluorurati per applicazioni in optoelettronica.

2012

composti eterociclici fluoruratioptoelettronica.Settore CHIM/06 - Chimica Organica
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Sintesi di un nuovo sensore fluorescente selettivo per Hg2++ contenente ossadiazoli fluorurati

2009

ssadiazoli sensori fluorescenti rilevazione metalli pesanti composti fluoruratiSettore CHIM/06 - Chimica Organica
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