0000000000353061
AUTHOR
I. Dillmann
First determination of β-delayed multiple neutron emission beyond A = 100 through direct neutron measurement : The P2n value of 136Sb
Background: β-delayed multiple neutron emission has been observed for some nuclei with A≤100, being the Rb100 the heaviest β2n emitter measured to date. So far, only 25P2n values have been determined for the ≈300 nuclei that may decay in this way. Accordingly, it is of interest to measure P2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A>100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of a…
Measurement of the heaviest Beta-delayed 2-neutron emitter: 136Sb
The Beta-delayed neutron emission probability, Pn , of very exotic nuclei is crucial for the understanding of nuclear structure properties of many isotopes and astrophysical processes such as the rapid neutron capture process (r-process). In addition Beta-delayed neutrons are important in a nuclear power reactor operated in a prompt sub-critical, delayed critical condition, as they contribute to the decay heat inducing fission reactions after a shut down. The study of neutron-rich isotopes and the measurement of Beta-delayed one-neutron emitters (Beta1n) is possible thanks to the Rare Isotope Beam (RIB) facilities, where radioactive beams allow the production of exotic nuclei of interest, w…
Selective laser ionization of N≥82 indium isotopes: The new r-process nuclide 135In
Production yields and beta-decay half-lives of very neutron-rich indium isotopes were determined at CERN/ISOLDE using isobaric selectivity of a resonance-ionization laser ion-source. Beta-delayed neutron multiscaling measurements have yielded improved half-lives for 206(6)~ms $^{132}$In, 165(3)~ms $^{133}$In and 141(5)~ms $^{134}$In. With 92(10)~ms $^{135}$In, a new r-process nuclide has been identified which acts as an important `waiting-point' in the In isotopic chain for neutron densities in the range n$_n \simeq 10^{24}$--10$^{26}$ n/cm$^3$, where the r-matter flow has already passed the ${\rm A} \simeq 130$ abundance-peak region.
Neutron measurements for advanced nuclear systems: The n_TOF project at CERN
A few years ago, the neutron time-of-flight facility n_TOF was built at CERN to address some of the urgent needs of high-accuracy nuclear data for Accelerator Driven Systems and other advanced nuclear energy systems, as well as for nuclear astrophysics and fundamental nuclear physics. Thanks to the characteristics of the neutron beam, and to state-of-the-art detection and acquisition systems, high quality neutron cross-section data have been obtained for a variety of isotopes, many of which radioactive. Following an important upgrade of the spallation target and of the experimental area, a new measurement campaign has started last year. After a brief review of the most important results obt…
β-decay of22O
A mass-separated 12 C 22 O molecular ion beam from the ISOLDE facility was used to study the decay of neutron-rich 22 O. The experimental results were compared with the results from an earlier experiment and predictions by shellmodel calculations using various effective interactions. The mechanism leading to the vanishing decay strength to the first 1 + level of the 22 F nucleus, predicted with the USD effective interaction but not supported by the experimental data, is analysed.
First Evidence of Axial Shape Asymmetry and Configuration Coexistence in 74Zn : Suggestion for a Northern Extension of the N = 40 Island of Inversion
The excited states of N=44 74Zn were investigated via γ-ray spectroscopy following 74Cu β decay. By exploiting γ−γ angular correlation analysis, the 2+2, 3+1, 0+2, and 2+3 states in 74Zn were firmly established. The γ-ray branching and E2/M1 mixing ratios for transitions deexciting the 2+2, 3+1, and 2+3 states were measured, allowing for the extraction of relative B(E2) values. In particular, the 2+3→0+2 and 2+3→4+1 transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are discussed in terms of underlying shapes, as well as the role of neutron excitations across the N=40 gap. Enhanced axial shape asy…
Neutron cross section measurements at n_TOF for ADS related estudies
A neutron Time-of-Flight facility (n_TOF) is available at CERN since 2001. The innovative features of the neutron beam, in particular the high instantaneous flux, the wide energy range, the high resolution and the low background, make this facility unique for measurements of neutron induced reactions relevant to the field of Emerging Nuclear Technologies, as well as to Nuclear Astrophysics and Fundamental Nuclear Physics. The scientific motivations that have led to the construction of this new facility are here presented. The main characteristics of the n_TOF neutron beam are described, together with the features of the experimental apparata used for cross-section measurements. The main res…
N=82Shell Quenching of the Classicalr-Process “Waiting-Point” NucleusCd130
First $\ensuremath{\beta}$- and $\ensuremath{\gamma}$-spectroscopic decay studies of the $N=82$ $r$-process ``waiting-point'' nuclide $^{130}\mathrm{C}\mathrm{d}$ have been performed at CERN/ISOLDE using the highest achievable isotopic selectivity. Several nuclear-physics surprises have been discovered. The first one is the unanticipatedly high energy of 2.12 MeV for the [$\ensuremath{\pi}{g}_{9/2}\ensuremath{\bigotimes}\ensuremath{\nu}{g}_{7/2}]$ ${1}^{+}$ level in $^{130}\mathrm{I}\mathrm{n}$, which is fed by the main Gamow-Teller transition. The second surprise is the rather high ${Q}_{\ensuremath{\beta}}$ value of 8.34 MeV, which is in agreement only with recent mass models that include…
First Evidence of Axial Shape Asymmetry and Configuration Coexistence in $^{74}$Zn: Suggestion for a Northern Extension of the $N=40$ Island of Inversion
International audience; The excited states of $N=44$$^{74}$Zn were investigated via $\gamma$-ray spectroscopy following $^{74}$Cu $\beta$ decay. By exploiting $\gamma$-$\gamma$ angular correlation analysis, the $2_2^+$, $3_1^+$, $0_2^+$ and $2_3^+$ states in $^{74}$Zn were firmly established. The $\gamma$-ray branching and $E2/M1$ mixing ratios for transitions de-exciting the $2_2^+$, $3_1^+$ and $2_3^+$ states were measured, allowing for the extraction of relative $B(E2)$ values. In particular, the $2_3^+ \to 0_2^+$ and $2_3^+ \to 4_1^+$ transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are disc…
First evidence of multiple β-delayed neutron emission for isotopes with a > 100
The β-delayed neutron emission probability, Pn, of very neutron-rich nuclei allows us to achieve a better understanding of the nuclear structure above the neutron separation energy, Sn. The emission of neutrons can become the dominant decay process in neutron-rich astrophysical phenomena such as the rapid neutron capture process (r-process). There are around 600 accessible isotopes for which β-delayed one-neutron emission (β1n) is energetically allowed, but the branching ratio has only been determined for about one third of them. β1n decays have been experimentally measured up to the mass A ∼ 150, plus a single measurement of 210Tl. Concerning two-neutron emitters (β2n), ∼ 300 isotopes are …
β -decay half-lives and β -delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126
Background: Previous measurements of Beta-delayed neutron emitters comprise around 230 nuclei, spanning from the 8He up to 150La. Apart from 210Tl, with a minuscule branching ratio of 0.07%, no other neutron emitter is measured yet beyond A = 150. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at A 195. Purpose: To measure both, Beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond N = 126. Method: Ions of interest are produced by fragmentation of a 238U beam, selected and identifed via the GSI-FRS fra…
Horizons: Nuclear Astrophysics in the 2020s and Beyond
Nuclear astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated.We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field…