0000000000373238
AUTHOR
V. Liberati
Single-neutron orbits near Ni-78: Spectroscopy of the N=49 isotope Zn-79
5 pags., 6 figs.
New developments of the in-source spectroscopy method at RILIS/ISOLDE
At the CERN ISOLDE facility, long isotope chains of many elements are produced by proton-induced reactions in target materials such as uranium carbide. The Resonance Ionization Laser Ion Source (RILIS) is an efficient and selective means of ionizing the reaction products to produce an ion beam of a chosen isotope. Coupling the RILIS with modern ion detection techniques enables highly sensitive studies of nuclear properties (spins, electromagnetic moments and charge radii) along an isotope chain, provided that the isotope shifts and hyperfine structure splitting of the atomic transitions can be resolved. At ISOLDE the campaign to measure the systematics of isotopes in the lead region (Pb, Bi…
β-delayed fission andαdecay ofAt196
A nuclear-decay spectroscopy study of the neutron-deficient isotope $^{196}\mathrm{At}$ is reported where an isotopically pure beam was produced using the selective Resonance Ionization Laser Ion Source and On-Line Isotope Mass Separator (CERN). The fine-structure $\ensuremath{\alpha}$ decay of $^{196}\mathrm{At}$ allowed the low-energy excited states in the daughter nucleus $^{192}\mathrm{Bi}$ to be investigated. A $\ensuremath{\beta}$-delayed fission study of $^{196}\mathrm{At}$ was also performed. A mixture of symmetric and asymmetric fission-fragment mass distributions of the daughter isotope $^{196}\mathrm{Po}$ (populated by $\ensuremath{\beta}$ decay of $^{196}\mathrm{At}$) was deduce…
Measurement of the first ionization potential of astatine by laser ionization spectroscopy
The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of the minute quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential. Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states enabled the first determination of the ionization potential of the astatine atom, 9.31751(8) eV. New ab initio calculations are performed to sup…
Changes in mean-squared charge radii and magnetic moments of $^{179–184}$Tl measured by in-source laser spectroscopy
Hyperfine structure and isotope shifts have been measured for the ground and isomeric states in the neutron-deficient isotopes 179–184Tl using the 276.9-nm transition. The experiment has been performed at the CERN-Isotope Separator On-Line facility using the in-source resonance-ionization laser spectroscopy technique. Spins for the ground states in 179,181,183Tl have been determined as I=1/2. Magnetic moments and changes in the nuclear mean-square charge radii have been deduced. By applying the additivity relation for magnetic moments of the odd-odd Tl nuclei the leading configuration assignments were confirmed. A deviation of magnetic moments for isomeric states in 182,184Tl from the trend…
Single-neutron orbits near 78 Ni: Spectroscopy of theN=49isotope 79 Zn
Single-neutron states in the Z=30, N=49isotope 79Zn have been populated using the 78Zn(d,p)79Zn transfer reaction at REX-ISOLDE, CERN. The experimental setup allowed the combined detection of protons ejected in the reaction, and of γrays emitted by 79Zn. The analysis reveals that the lowest excited states populated in the reaction lie at approximately 1MeV of excitation, and involve neutron orbits above the N=50shell gap. From the analysis of γ-ray data and of proton angular distributions, characteristic of the amount of angular momentum transferred, a5/2+configuration was assigned to a state at 983keV. Comparison with large-scale-shell-model calculations supports a robust neutron N=50shell…
Change in structure between the $I = 1/2$ states in $^{181}$Tl and $^{177,179}$Au
Abstract The first accurate measurements of the α-decay branching ratio and half-life of the I π = 1 / 2 + ground state in 181Tl have been made, along with the first determination of the magnetic moments and I = 1 / 2 spin assignments of the ground states in 177,179Au. The results are discussed within the complementary systematics of the reduced α-decay widths and nuclear g factors of low-lying, I π = 1 / 2 + states in the neutron-deficient lead region. The findings shed light on the unexpected hindrance of the 1 / 2 + → 1 / 2 + , 181Tl → g 177 Aug α decay, which is explained by a mixing of π 3 s 1 / 2 and π 2 d 3 / 2 configurations in 177Aug, whilst 181Tlg remains a near-pure π 3 s 1 / 2 .…
Charge radii and electromagnetic moments of At195–211
Hyperfine-structure parameters and isotope shifts of At195-211 have been measured for the first time at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy method. The hyperfine structures of isotopes were recorded using a triad of experimental techniques for monitoring the photo-ion current. The Multi-Reflection Time-of-Flight Mass Spectrometer, in connection with a high-resolution electron multiplier, was used as an ion-counting setup for isotopes that either were affected by strong isobaric contamination or possessed a long half-life; the ISOLDE Faraday cups were used for cases with high-intensity beams; and the Windmill decay station was used for short-lived, predominantl…