0000000000387393
AUTHOR
Olivier Demichel
Delocalization of Nonlinear Optical Responses in Plasmonic Nanoantennas
Remote excitation and emission of two-photon luminescence and second-harmonic generation are observed in micrometer long gold rod optical antennas upon local illumination with a tightly focused near-infrared femtosecond laser beam. We show that the nonlinear radiations can be emitted from the entire antenna and the measured far-field angular patterns bear the information regarding the nature and origins of the respective nonlinear processes. We demonstrate that the nonlinear responses are transported by the propagating surface plasmon at excitation frequency, enabling thereby polariton-mediated tailoring and design of nonlinear responses.
Single-Crystal vs Polycrystalline Gold: A Non-linear-Optics Analysis
Standard gold in the field of plasmonics is obtained by evaporation or sputtering and therefore is polycrystalline. Yet, this gold presents numbers of drawbacks such as roughness, grains and ill-defined electronic band diagrams in addition to the lack of reproducibility from one instrument to another. It is, thus, beneficial to turn to a metal production that can enable well-defined and controlled gold parameters. To that end, we have explored the wet synthesis of gold nanoplates which represents a simple and robust means of obtaining single-crystal gold (Guo Z, Zhang Y, DuanMu Y, Xu L, Xie S, Gu N, Colloids Surf A 278:33–38, 2006). The synthesized nanoplates are from 50 to less than 100 nm…
Improving the transmittance of an epsilon-near-zero-based wavefront shaper
Although Epsilon-Near-Zero metamaterials (ENZ) offer many unconventional ways to play with light, the optical impedance mismatch with surroundings can limit the efficiency of future devices. We report here on the improvement of the transmittance of an Epsilon-Near-Zero (ENZ) wavefront shaper. We first address in this paper the way to enhance the transmittance of a plane wave through a layer of ENZ material thanks to a numerical optimization approach based on the Transfer Matrix Method. We then transpose the one dimensional approach to a two dimensional case where the emission of a dipole is shaped into a plane wave by an ENZ device with a design that optimizes the transmittance. As a result…
Cavity Resonator Integrated Guided mode resonance Filter : Spectral & Modal Reflector
International audience; CRIGF is a new generation of narrowband filter. It consists of subwavelength gratings nearby or upon a waveguide. At the center, a small GMRF (Guided Mode Resonance Filter) or GC (Grating Coupler) coupled radiated & guided mode, then, DBR (Distributed Bragg Reflector) at each side localise mode inside a horizontal Fabry-Pérot cavity. Two PS (Phase sections) are use to fine tune the Fabry-Pérot modes with the grating coupler.
Silicon-microring into a fiber laser cavity for high-repetition-rate pulse train generation
International audience; In 1997, Yoshida et al. inserted a Fabry-Perot filter in a modulation instability fiber laser cavity [1], the free spectral range (FSR) of the Fabry-Perot fixed the RF to 115 GHz; however the pulsed laser was poorly stable. Since then, lasers of increasing performance have been demonstrated using variants of this method. In 2012, Peccianti et al., demonstrated the first fiber laser harmonically mode-locked by integrated high-finesse microresonator [2]. The doped silica, on-chip microresonator provided both high spectral selectivity and nonlinearity, thus promoting the dynamics pulsed at 200 GHz. By using a silicon microring resonator (SMRR), this approach lead to the…
Multimodal reflectivity of CRIGF filters: First experimental observation and modelling
International audience; Cavity Resonator Integrated Guided-mode Resonance Filter (CRIGF) are a new class of filtering reflectors whose selected wavelength and spectral width are independent of the angle of incidence unlike GMRF. These particular properties allow both compactness and a high angular acceptance. However, ours studies show that CRIGFs offer simultaneously spectral and modal filtering and we evidence high-spatial-order reflected modes. In this paper, we will present characterization of the spectral and spatial profile that demonstrates the existence of these high-order modes. In addition, we will present a model based on the physical understanding of implied phenomena to explain…
Near-field properties of plasmonic nanostructures with high aspect ratio
International audience; Using the Green's dyad technique based on cuboidal meshing, we compute the electromagnetic field scattered by metal nanorods with high aspect ratio. We investigate the effect of the meshing shape on the numerical simulations. We observe that discretizing the object with cells with aspect ratios similar to the object's aspect ratio improves the computations, without degrading the convergency. We also compare our numerical simulations to finite element method and discuss further possible improvements.
Towards an efficient epsilon near-zero-based wavefront shaper
Although epsilon-near-zero (ENZ) metamaterials offer many unconventional ways to play with light, the optical impedance mismatch with surroundings can limit the efficiency of future devices. An original example of ENZ-based applications is the wavefront shaping, but up to now devices have transmission efficiency as low as 10-5 [1]. Here, we report strategies to enhance the transmittance through ENZ layer and we demonstrate an enhancement by four orders of magnitude of the transmittance, which reaches up to 15% in the context of ENZ-based wavefront shaping [2].
High Order modes in Cavity Resonator Integrated Guided mode resonance Filters (CRIGFs)
International audience
High-order modes in cavity-resonator-integrated guided-mode resonance filters (CRIGFs)
International audience; Cavity-resonator-integrated guided-mode resonance filters (CRIGFs) are optical filters based on weak coupling by a grating between a free-space propagating optical mode and a guided mode, like guided-mode resonance filters (GMRFs). As compared to GMRFs they offer narrowband reflection with small aperture and high angular acceptance. We report experimental characterization and theoretical modeling of unexpected high-order reflected modes in such devices. Using coupled-mode modeling and moiré analysis we provide physical insight on key mechanisms ruling CRIGF properties. This model could serve as a simple and efficient framework to design new reflectors with tailored s…
Hot electrons and nonlinear optical nanoantennas
The large field enhancement generated at the surface of a resonant plasmonic nanoparticle, or optical antennas, is the key mechanism that eventually led to the development of nonlinear plasmonics [1-2]. While the resonance may boost the nonlinear yield of an adjacent structure or surrounding medium, it was soon realized that optical antennas possess nonlinear coefficients comparable or exceeding those of standard nonlinear optical materials [3]. We discuss here two nonlinear optical processes — incoherent multi-photon luminescence (MPL) and coherent second-harmonic generation (SHG) — emitted from gold rod optical antennas upon local illumination with a tightly focused femtosecond near-infra…
Selective excitation of bright and dark plasmonic resonances of single gold nanorods.
Plasmonic dark modes are pure near-field resonances since their dipole moments are vanishing in far field. These modes are particularly interesting to enhance nonlinear light-matter interaction at the nanometer scale because radiative losses are mitigated therefore increasing the intrinsic lifetime of the resonances. However, the excitation of dark modes by standard far field approaches is generally inefficient because the symmetry of the electromagnetic near-field distribution has a poor overlap with the excitation field. Here, we demonstrate the selective optical excitation of bright and dark plasmonic modes of single gold nanorods by spatial phase-shaping the excitation beam. Using two-p…
Spatial Distribution of the Nonlinear Photoluminescence in Au Nanowires
When gold nanowires are excited with a tightly focused femtosecond laser a distributed nonlinear photoluminescence (N-PL) develops throughout the entire structure. A complete spaced-resolved analysis of the spectral signature of the nanowire nonlinear response is carried out to understand the origin of the distributed nonlinear response. We discuss various mechanisms to explain the experimental data and unambiguously demonstrate that the spatial and spectral extension of the N-PL in the nanowire are mainly dictated by the propagation of a surface plasmon excited at the pump wavelength. We also present experimental signature of near-field excitation of a broadband continuum of surface plasmo…