Shape coexistence in the neutron-deficient even-even Hg182-188 isotopes studied via Coulomb excitation

Coulomb-excitation experiments to study electromagnetic properties of radioactive even-even Hg isotopes were performed with 2.85  MeV/nucleon mercury beams from REX-ISOLDE. Magnitudes and relative signs of the reduced E2 matrix elements that couple the ground state and low-lying excited states in Hg182-188 were extracted. Information on the deformation of the ground and the first excited 0+ states was deduced using the quadrupole sum rules approach. Results show that the ground state is slightly deformed and of oblate nature, while a larger deformation for the excited 0+ state was noted in Hg182,184. The results are compared to beyond mean field and interacting-boson based models and interp…

Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes

Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po196,198,200,202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po200,202, the transitional and diagonal matrix elements of the 2+1 state are determined. In Po196,198 multistep Coulomb excitation is observed, populating the 4+1,0+2, and 2+2 states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from Po196 onwards. Three model descriptions are used to compare to the data. Calculati…

Shape Coexistence in the Neutron-Deficient Even-EvenHg182−188Isotopes Studied via Coulomb Excitation

Coulomb-excitation experiments to study electromagnetic properties of radioactive even-even Hg isotopes were performed with 2.85 MeV/nucleon mercury beams from REX-ISOLDE. Magnitudes and relative signs of the reduced E2 matrix elements that couple the ground state and low-lying excited states in Hg182-188 were extracted. Information on the deformation of the ground and the first excited 0(+) states was deduced using the quadrupole sum rules approach. Results show that the ground state is slightly deformed and of oblate nature, while a larger deformation for the excited 0(+) state was noted in Hg-182; 184. The results are compared to beyond mean field and interacting-boson based models and i…

Decay studies of the long-lived states in $^{186}$Tl

Decay spectroscopy of the long-lived states in $^{186}$Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The $\alpha$ decay from the low-spin $(2^-)$ state in $^{186}$Tl was observed for the first time and a half-life of $3.4^{+0.5}_{-0.4}$ s was determined. Based on the $\alpha$-decay energy, the relative positions of the long-lived states were fixed, with the $(2^-)$ state as the ground state, the $7^{(+)}$ state at 77(56)~keV and the $10^{(-)}$ state at 451(56) keV. The level scheme of the internal decay of the $^{186}$Tl($10^{(-)}$) state ($T_{1/2} = 3.40(9)$ s), which was known to decay solely through emission of 374 keV $\gamma$-ray transition, was extended and a lowe…

Collective 2$^{+1}$ excitations in$^{206}$Po and$^{208,210}$Rn

In the present study, $B(E2; 2^{+}_{1}\rightarrow 0^{+}_{1})$ values have been measured in the 208,210Rn and 206Po nuclei through Coulomb excitation of re-accelerated radioactive beams in inverse kinematics at CERN-ISOLDE. These nuclei have been proposed to lie in, or at the boundary of the region where the seniority scheme should persist. However, contributions from collective excitations are likely to be present when moving away from the N=126 closed shell. Such an effect is confirmed by the observed increased collectivity of the $2^{+}_{1}\rightarrow 0^{+}_{1}$ transitions. Experimental results have been interpreted with the aid of theoretical studies carried out within the BCS-based QRP…

Decay studies of the long-lived states in Tl-186

9 pags., 12 figs., 3 tabs.

Coulomb excitation of re-accelerated 208Rn and 206Po beams

In the present study, B( E2; 2(+)-> 0(+) ) values have been measured in the Rn-208 and Po-206 nuclei through Coulomb excitation of re-accelerated radioactive beams in inverse kinematics at CERN-ISOLDE. The resulting B(E2; 2(+)-> 0(+)) in 208Rn is similar to 0.08 e(2)b(2). These nuclei lie in, or at the boundary of the region where seniority scheme should persist. However, contributions from collective excitations may be present when moving away from the N = 126 shell closure. To date, surprisingly little is known of the transition probabilities between the low-spin states in this region.

Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements in 184,186Hg and two-state mixing calculations

The neutron-deficient mercury isotopes, $^{184,186}$Hg, were studied with the Recoil Distance Doppler Shift (RDDS) method using the Gammasphere array and the K\"oln Plunger device. The Differential Decay Curve Method (DDCM) was employed to determine the lifetimes of the yrast states in $^{184,186}$Hg. An improvement on previously measured values of yrast states up to $8^{+}$ is presented as well as first values for the $9_{3}$ state in $^{184}$Hg and $10^{+}$ state in $^{186}$Hg. $B(E2)$ values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia (VMI) model, allowing for extraction of spin-dependent mixing strengths and amplitudes.

Coulomb excitation of Rn-222

The nature of quadrupole and octupole collectivity in 222Rn was investigated by determining the electric-quadrupole (E2) and octupole (E3) matrix elements using subbarrier, multistep Coulomb excitation. The radioactive 222Rn beam, accelerated to 4.23 MeV/u, was provided by the HIE-ISOLDE facility at CERN. Data were collected in the Miniball γ-ray spectrometer following the bombardment of two targets, 120Sn and 60Ni. Transition E2 matrix elements within the ground-state and octupole bands were measured up to 10ℏ and the results were consistent with a constant intrinsic electric-quadrupole moment, 518(11)efm2. The values of the intrinsic electric-octupole moment for the 0+→3− and 2+→5− transi…

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around Z=82 and the neutron midshell at N=104. Purpose: Evidence for shape coexistence has been inferred from α-decay measurements, laser spectroscopy, and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of Rn202 and Rn…

Determination of the B(E3, 0+ → 3−)-excitation strength in octupole-correlated nuclei near A ≈224 by the means of Coulomb excitation at REX-ISOLDE

The IS475 collaboration conducted Coulomb-excitation experiments with postaccelerated radioactive 220Rn and 224Ra beams at the REX-ISOLDE facility. The beam particles (Ebeam ≈ 2.83 MeV/u) were Coulomb excited using 60Ni, 114Cd, and 120Sn scattering targets. De-excitation γ-rays were detected employing the Miniball array and scattered particles were detected in a silicon detector. Exploiting the Coulomb-excitation code GOSIA for each nucleus several matrix elements could be obtained from the measured γ-ray yields. The extracted 3−||Ê3||0+ matrix element allows for the conclusion that, while 220Rn represents an octupole vibrational system, 224Ra has already substantial octupole correlations i…

Decay studies of the long-lived states in Tl186

Decay spectroscopy of the long-lived states in 186Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The α decay from the low-spin (2−) state in 186Tl was observed for the first time and a half-life of 3.4+0.5−0.4 s was determined. Based on the α-decay energy, the relative positions of the long-lived states were fixed, with the (2−) state as the ground state, the 7(+) state at 77(56) keV, and the 10(−) state at 451(56) keV. The level scheme of the internal decay of the 186Tl(10(−)) state [T1/2=3.40(9) s], which was known to decay solely through emission of 374-keV γ-ray transition, was extended and a lower limit for the β-decay branching bβ>5.9(3)% was determined. The extrac…

The Miniball spectrometer

The Miniball germanium detector array has been operational at the REX (Radioactive ion beam EXperiment) post accelerator at the Isotope Separator On-Line facility ISOLDE at CERN since 2001. During the last decade, a series of successful Coulomb excitation and transfer reaction studies have been performed with this array, utilizing the unique and high-quality radioactive ion beams which are available at ISOLDE. In this article, an overview is given of the technical details of the full Miniball setup, including a description of the γ-ray and particle detectors, beam monitoring devices and methods to deal with beam contamination. The specific timing properties of the REX-ISOLDE facility are hi…

Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements in Hg-184,Hg-186 and two-state mixing calculations

Abstract: The neutron-deficient mercury isotopes, 184 , 186 Hg, were studied with the recoil distance Doppler-shift method using the Gammasphere array and the K ̈ oln plunger device. The differential decay curve method was employed to determine the lifetimes of the yrast states in 184 , 186 Hg. An improvement on previously measured values of yrast states up to 8 + is presented as well as first values for the 9 3 state in 184 Hg and 10 + state in 186 Hg. B ( E 2) values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia model, allowing for extraction of spin-dependent mixing strengths and amplitudes. peerReviewed

X-ray production with heavy post-accelerated radioactive-ion beams in the lead region of interest for Coulomb-excitation measurements

Abstract Characteristic K X-rays have been observed in Coulomb-excitation experiments with heavy radioactive-ion beams in the lead region (Z = 82), produced at the REX-ISOLDE facility, and were used to identify the decay of strongly converted transitions as well as monopole 0 2 + → 0 1 + transitions. Different targets were used, and the X-rays were detected by the Miniball γ-ray spectrometer surrounding the target position. A stable mercury isotope, as well as neutron-deficient mercury, lead, polonium, and radon isotopes were studied, and a detailed description of the analysis using the radioactive 182,184,186,188Hg isotopes is presented. Apart from strongly converted transitions originatin…

Analysis methods of safe Coulomb-excitation experiments with radioactive ion beams using the gosia code

With the recent advances in radioactive ion beam technology, Coulomb excitation at safe energies becomes an important experimental tool in nuclear-structure physics. The usefulness of the technique to extract key information on the electromagnetic properties of nuclei has been demonstrated since the 1960's with stable beam and target combinations. New challenges present themselves when studying exotic nuclei with this technique, including dealing with low statistics or number of data points, absolute and relative normalisation of the measured cross sections and a lack of complimentary experimental data, such as excited-state lifetimes and branching ratios. This paper addresses some of these…

In-gas laser ionization and spectroscopy of actinium isotopes near the N=126 closed shell

The in-gas laser ionization and spectroscopy (IGLIS) techniquewas applied on the $^{212–215}$Ac isotopes, produced at the Leuven Isotope Separator On-Line (LISOL) facility by using the in-gas-cell and the in-gas-jet methods. The first application under on-line conditions of the in-gas-jet laser spectroscopy method showed a superior performance in terms of selectivity, spectral resolution, and efficiency in comparison with the in-gas-cell method. Following the analysis of both experiments, the magnetic-dipole moments for the $^{212–215}$Ac isotopes, electric-quadrupole moments and nuclear spins for the $^{214,215}$Ac isotopes are presented and discussed. A good agreement is obtained with lar…

Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements inHg184,186and two-state mixing calculations

The neutron-deficient mercury isotopes, $^{184,186}$Hg, were studied with the Recoil Distance Doppler Shift (RDDS) method using the Gammasphere array and the Koln Plunger device. The Differential Decay Curve Method (DDCM) was employed to determine the lifetimes of the yrast states in $^{184,186}$Hg. An improvement on previously measured values of yrast states up to $8^{+}$ is presented as well as first values for the $9_{3}$ state in $^{184}$Hg and $10^{+}$ state in $^{186}$Hg. $B(E2)$ values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia (VMI) model, allowing for extraction of spin-dependent mixing strengths and amplitudes.

Studies of pear-shaped nuclei using accelerated radioactive beams

There is strong circumstantial evidence that certain heavy, unstable atomic nuclei are ‘octupole deformed’, that is, distorted into a pear shape. This contrasts with the more prevalent rugby-ball shape of nuclei with reflection-symmetric, quadrupole deformations. The elusive octupole deformed nuclei are of importance for nuclear structure theory, and also in searches for physics beyond the standard model; any measurable electric-dipole moment (a signature of the latter) is expected to be amplified in such nuclei. Here we determine electric octupole transition strengths (a direct measure of octupole correlations) for short-lived isotopes of radon and radium. Coulomb excitation experiments we…

Shapes and Collectivity in Neutron Deficient Even-Mass 188–198Pb Isotopes

Shapes and Collectivity in Neutron Deficient Even-Mass 188–198Pb Isotopes

The neutron deficient 188−198Pb isotopes have been studied in a Coulomb excitation measurement employing the Miniball spectrometer and radioactive beams from REX-ISOLDE, CERN. These isotopes are of particular importance as they lie in a transitional region, where the intruding structures, associated with different deformed shapes, come down in energy close to the spherical ground state. For detailed analysis of the Coulomb excitation data, the understanding of the beam composition is essential. peerReviewed

Collectivity in ${}^{\mathrm{196,198}}$Pb isotopes probed in Coulomb-excitation experiments at REX-ISOLDE

The neutron-deficient ${}^{\mathrm{196,198}}$Pb isotopes have been studied in Coulomb-excitation experiments employing the Miniball γ-ray spectrometer and radioactive ion beams from the REX-ISOLDE post-accelerator at CERN. The reduced transition probabilities of the first excited 2+ states in 196Pb and 198Pb nuclei have been measured for the first time. Values of $B(E2)={18.2}_{-4.1}^{+4.8}$ W.u. and $B(E2)={13.1}_{-3.5}^{+4.9}$ W.u., were obtained, respectively. The experiment sheds light on the development of collectivity when moving from the regime governed by the generalised seniority scheme to a region, where intruding structures, associated with different deformed shapes, start to com…

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes: Coulomb excitation of Hg-182, Hg-184, Hg-186 and Hg-188

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate…

Evolution of Octupole Deformation in Radium Nuclei from Coulomb Excitation of Radioactive Ra222 and Ra228 Beams

There is sparse direct experimental evidence that atomic nuclei can exhibit stable "pear" shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole (E3) matrix elements have been determined for transitions in ^{222,228}Ra nuclei using the method of sub-barrier, multistep Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of E3 matrix elements for different nuclear transitions is explained by describing ^{222}Ra as pear shaped with stable octupole deformation, while ^{228}Ra behaves like an octupole vibrator.

Do nuclei go pear-shaped? Coulomb excitation of 220Rn and 224Ra at REX-ISOLDE (CERN)

Artículo escrito por muchos autores, sólo se referencian el primero, los autores que firman como Universidad Autónoma de Madrid y el grupo de colaboración en el caso de que aparezca en el artículo

Coulomb excitation of Na-29,Na-30: Mapping the borders of the island of inversion

Seidlitz, M., et all ; 10 pags. ; 9 figs. ; 1 tab. ; PACS number(s): 21.60.Cs, 23.20.Js, 25.70.De, 29.38.Gj

Coulomb excitation of 222Rn

International audience; The nature of quadrupole and octupole collectivity in $^{222}$Rn was investigated by determining the electric-quadrupole (E2) and octupole (E3) matrix elements using subbarrier, multistep Coulomb excitation. The radioactive $^{222}$Rn beam, accelerated to 4.23 MeV/u, was provided by the HIE-ISOLDE facility at CERN. Data were collected in the Miniball $\gamma$ -ray spectrometer following the bombardment of two targets, $^{120}$Sn and $^{60}$Ni. Transition E2 matrix elements within the ground-state and octupole bands were measured up to 10 ¯h and the results were consistent with a constant intrinsic electric-quadrupole moment, 518(11) $e$ fm$^2$ . The values of the int…

The observation of vibrating pear-shapes in radon nuclei

6 pags., 4 fig.s, 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0