0000000000956821
AUTHOR
Pasi Karvonen
Total absorption study of the \beta decay of 102,104,105Tc
The β-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely 102,104,105Tc, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations. peerReviewed
Signatures of oblate deformation in the ^{111}Tc nucleus
Monoisotopic samples of exotic, neutron-rich ${}^{111}$Mo nuclei, produced in the deuteron-induced fission of ${}^{238}$U and separated using the IGISOL3 isotope separator, coupled to the JYFLTRAP Penning trap, were used to perform $\ensuremath{\beta}$- and $\ensuremath{\gamma}$-coincidence spectroscopy of ${}^{111}$Tc. New excited levels in ${}^{111}$Tc populated in ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of ${}^{111}$Mo provide the first indication for an oblate deformation in the mass $A\ensuremath{\approx}110$ region. The wide spin range of levels populated in ${}^{111}$Tc following the decay of ${}^{111}$Mo indicates the existence of two $\ensuremath{\beta}$-decaying levels in ${…
New ion-guide for the production of beams of neutron-rich nuclei between Z=20–28
It has been shown for the first time that quasi- and deep-inelastic reactions can be successfully incorporated into the conventional Ion-Guide Isotope Separator On-Line (IGISOL) technique. This is of particular interest for characterizing the decay properties of refractory elements and is applied to neutron rich nuclei between Z = 20-28. As a first step of this project, the kinematics of quasi- and deep-inelastic reactions, such as {sup 197}Au({sup 65}Cu,X)Y, were studied. Based on these studies, a specialized IGISOL target chamber was designed and built. This chamber was tested in on- and off-line conditions at the Jyvaskyla IGISOL facility. Yields of radioactive, projectile-like species s…
Independent Isotopic Product Yields in 25 MeV and 50 MeV Charged Particle Induced Fission of 238U and 232Th
Abstract Independent isotopic yields for most elements from Zn to La in 25-MeV proton-induced fission of 238U and 232Th have been determined at the IGISOL facility in the University of Jyvaskyla. In addition, isotopic yields for Zn, Ga, Rb, Sr, Zr, Pd and Xe in 50-MeV proton-induced fission of 238U and for Zn, Ga, Rb, Sr, Cd and In in 25-MeV deuterium-induced fission of 238U have been measured. The utilised technique recently developed at the University of Jyvaskyla, is based on a combination of the ion guide technique and the ability of a Penning trap to unambiguously identify the isotopes by their atomic mass. Since the yields are determined by ion counting, no prior knowledge beyond the …
New lifetime measurements inPd109and the onset of deformation atN=60
Several new subnanosecond lifetimes were measured in Pd-109 using the fast-timing beta gamma gamma (t) method. Fission fragments of the A = 109 mass chain were produced by bombarding natural uranium with 30 MeV protons at the Jyvaskyla Ion Guide Isotope Separator On-Line (IGISOL) facility. Lifetimes were obtained for excited states in Pd-109 populated following beta decay of Rh-109. The new lifetimes provide some insight into the evolution of nuclear structure in this mass region. In particular, the distinct structure of the two low-lying 7/2(+) states occurring systematically across the Pd isotopic chain is supported by the new lifetime measurements. The available nuclear data indicate a s…
Fission yield studies with SPIG-equipped IGISOL : a novel method for nuclear data measurements
This thesis work consists of two sections. In the first section, the development of a so-called Laser Ion Source Trap (LIST) device is described. The LIST device is based on a double SPIG (SextuPole Ion Guide) system, providing the possibility to improve the elemental selectivity of the IGISOL method via highly discriminative laser ionization occurring outside the ion guide. The improved selectivity enables the production of isotopically pure beams. The double SPIG can be used without laser ionization and replaces the conventional skimmer electrode. In this work, the SPIG is compared to the skimmer and is shown to remarkably improve both the efficiency and beam quality of the IGISOL facilit…
Total Absorption Spectroscopy of Fission Fragments Relevant for Reactor Antineutrino Spectra and Decay Heat Calculations
Volume: 111 Host publication title: WONDER-2015 Host publication sub-title: 4TH INTERNATIONAL WORKSHOP ON NUCLEAR DATA EVALUATION FOR REACTOR APPLICATIONS Isbn(print): 978-2-7598-1970-6 Beta decay of fission products is at the origin of decay heat and antineutrino emission in nuclear reactors. Decay heat represents about 7% of the reactor power during operation and strongly impacts reactor safety. Reactor antineutrino detection is used in several fundamental neutrino physics experiments and it can also be used for reactor monitoring and non-proliferation purposes. Rb-92,Rb-93 are two fission products of importance in reactor antineutrino spectra and decay heat, but their beta-decay properti…
Total absorption spectroscopy of fission fragments relevant for reactor antineutrino spectra
International audience; The accurate determination of reactor antineutrino spectra remains a very active research topic for which new methods of study have emerged in recent years. Indeed, following the long-recognized reactor anomaly (measured antineutrino deficit in short baseline reactor experiments when compared with spectral predictions), the three international reactor neutrino experiments Double Chooz, Daya Bay and Reno have recently demonstrated the existence of spectral distortions in their measurements with respect to the same predictions. These spectral predictions were obtained through the conversion of integral beta-energy spectra obtained at the ILL research reactor. Several s…
Upgrade and yields of the IGISOL facility
The front end of the Jyvaskyla IGISOL facility was upgraded in 2003 by increasing its pumping capacity and by improving the radiation shielding. In late 2005, the skimmer electrode of the mass separator was replaced by a sextupole ion guide, which improved the mass separator efficiency up to an order of magnitude. The current design of the facility is described. The updated yield data, achieved with and without the additional JYFLTRAP purification, using both fusion evaporation reactions and particle induced fission is presented to give an overview of the capability of the facility. These data have been determined either by radioactivity measurements or by direct ion counting after the Penn…
Isomer and decay studies for the rp process at IGISOL
This article reviews the decay studies of neutron-deficient nuclei within the mass region \ensuremathA=56--100 performed at the Ion-Guide Isotope Separator On-Line (IGISOL) facility in the University of Jyväskylä over last 25 years. Development from He-jet measurements to on-line mass spectrometry, and eventually to atomic mass measurements and post-trap spectroscopy at IGISOL, has yielded studies of around 100 neutron-deficient nuclei over the years. The studies form a solid foundation to astrophysical rp -process path modelling. The focus is on isomers studied either via spectroscopy or via Penning-trap mass measurements. The review is complemented with recent results on the ground and is…
Half-life, branching-ratio, andQ-value measurement for the superallowed0+→0+β+emitterTi42
The half-life, the branching ratio, and the decay $Q$ value of the superallowed $\ensuremath{\beta}$ emitter $^{42}\mathrm{Ti}$ were measured in an experiment performed at the JYFLTRAP facility of the Accelerator Laboratory of the University of Jyv\"askyl\"a. $^{42}\mathrm{Ti}$ is the heaviest ${T}_{z}=\ensuremath{-}1$ nucleus for which high-precision measurements of these quantities have been tried. The half-life (${T}_{1/2}=208.14\ifmmode\pm\else\textpm\fi{}0.45$ ms) and the $Q$ value [${Q}_{\mathrm{EC}}=7016.83(25)$ keV] are close to or reach the required precision of about 0.1%. The branching ratio for the superallowed decay branch [$\mathrm{BR}=47.7(12)%$], a by-product of the half-lif…
β-decay data requirements for reactor decay heat calculations: study of the possible source of the gamma-ray discrepancy in reactor heat summation calculations
The decay heat of fission products plays an important role in predictions of the heat up of nuclear fuel in reactors. The released energy is calculated as the summation of the activities of allfission products P(t) = Ei λi Ni(t), where Ei is the decay energy of nuclide i (gamma and beta component), λi is the decay constant of nuclide i and Ni(t) is the number of nuclide i at cooling time t. Even though the reproduction of the measured decay heat has improved in recent years, there is still a long standing discrepancy in the t ∼ 1000s cooling time for some fuels. A possible explanation to this improper description has been found in the work of Yoshida et al. (1), where it has been shown that…
Independent isotopic yields in 25 MeV and 50 MeV proton-induced fission of natU
Independent isotopic yields for elements from Zn to La in the 25 MeV proton-induced fission of natUnatU were determined with the JYFLTRAP facility. In addition, isotopic yields for Zn, Ga, Rb, Sr, Zr, Pd and Xe in the 50 MeV proton-induced fission of natUnatU were measured. The deduced isotopic yield distributions are compared with a Rubchenya model, the GEF model with universal parameters and the semi-empirical Wahl model. Of these, the Rubchenya model gives the best overall agreement with the obtained data. Combining the isotopic yield data with mass yield data to obtain the absolute independent yields was attempted. The result depends on the mass yield distribution. peerReviewed
Total Absorption Spectroscopy of Fission Fragments Relevant for Reactor Antineutrino Spectra and Decay Heat Calculations
Beta decay of fission products is at the origin of decay heat and antineutrino emission in nuclear reactors. Decay heat represents about 7% of the reactor power during operation and strongly impacts reactor safety. Reactor antineutrino detection is used in several fundamental neutrino physics experiments and it can also be used for reactor monitoring and non-proliferation purposes. 92,93Rb are two fission products of importance in reactor antineutrino spectra and decay heat, but their β-decay properties are not well known. New measurements of 92,93Rb β-decay properties have been performed at the IGISOL facility (Jyväskylä, Finland) using Total Absorption Spectroscopy (TAS). TAS is complemen…
New insights into triaxiality and shape coexistence from odd-mass Rh109
Rapid shape evolutions near A = 100 are now the focus of much attention in nuclear science. Much of the recent work has been centered on isotopes with Z <= 40, where the shapes are observed to transition between near-spherical to highly deformed with only a single pair of neutrons added. At higher Z, the shape transitions become more gradual as triaxiality sets in, yet the coexistence of varying shapes continues to play an important role in the low-energy nuclear structure, particularly in the odd-Z isotopes. This work aims to characterize competing shapes in the triaxial region between Zr and Sn isotopes using ultrafast timing techniques to measure lifetimes of excited states in the neutro…
Penning-trap-assisted study of 115Ru beta decay
The beta decay of 115Ru has been studied by means of Penning-trap-assisted beta and gamma spectroscopy at the IGISOL facility. The level scheme of 115Rh has been substantially extended and compared with the level systematics of lighter rhodium isotopes. Tentative candidates for three states of the deformed K = 1/2 band have been suggested. The beta-strength distribution of the beta decay of 115Ru differs from the beta decays of 111, 113, 113mRu isotopes due to non-observation of the 3-quasiparticle states in 115Rh. The decay properties of 115Ru indicate a spin-parity of (3/2+ for its beta-decaying ground state. In addition, possible Nilsson states as well as the shape and spin transitions i…
Excited states inPd115populated in theβ−decay ofRh115
Excited states in $^{115}\mathrm{Pd}$, populated following the ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of $^{115}\mathrm{Rh}$ have been studied by means of $\ensuremath{\gamma}$ spectroscopy after the Penning-trap station at the IGISOL facility, University of Jyv\"askyl\"a. The $1$$/$$2$${}^{+}$ spin and parity assignment of the ground state of $^{115}\mathrm{Pd}$, confirmed in this work, may indicate a transition to an oblate shape in Pd isotopes at high neutron number.
Reactor Decay Heat inPu239: Solving theγDiscrepancy in the 4–3000-s Cooling Period
The {beta} feeding probability of {sup 102,104,105,106,107}Tc, {sup 105}Mo, and {sup 101}Nb nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the {gamma} component of the decay heat for {sup 239}Pu in the 4-3000 s range.
Decay study ofTc114with a Penning trap
The level structure of $^{114}\mathrm{Ru}$ has been investigated via the $\ensuremath{\beta}$ decay of very neutron-rich $^{114}\mathrm{Tc}$ by means of Penning-trap-assisted $\ensuremath{\gamma}$ spectroscopy. The deduced $\ensuremath{\beta}$-decay scheme suggests the existence of two $\ensuremath{\beta}$-decaying states in $^{114}\mathrm{Tc}$ with ${I}^{\ensuremath{\pi}}={1}^{+}$ and $I\ensuremath{\geqslant}$ 4, with half-lives of ${t}_{1/2}({1}^{+})=90(20)$ ms and ${t}_{1/2}(I\ensuremath{\geqslant}4)=100(20)$ ms, respectively. The ${Q}_{\ensuremath{\beta}}$ value, which covers a possible mixture of two states, has been determined to be ${Q}_{\ensuremath{\beta}}=11 785(12)$ keV. The level…
New lifetime measurements in 109 Pd and the onset of deformation at N = 60
Several new subnanosecond lifetimes were measured in 109Pd using the fast-timing βγγ (t) method. Fission fragments of the A = 109 mass chain were produced by bombarding natural uranium with 30 MeV protons at the Jyvaskyl ¨ a Ion Guide Isotope Separator On-Line (IGISOL) facility. Lifetimes were obtained for excited states ¨ in 109Pd populated following β decay of 109Rh. The new lifetimes provide some insight into the evolution of nuclear structure in this mass region. In particular, the distinct structure of the two low-lying 7/2+ states occurring systematically across the Pd isotopic chain is supported by the new lifetime measurements. The available nuclear data indicate a sudden increase i…
Total Absorption Spectroscopy Study ofRb92Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape
The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. (92)Rb makes the dominant contribution to the reactor antineutrino spectrum in the 5-8 MeV range but its decay properties are in question. We have studied (92)Rb decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.
A sextupole ion beam guide to improve the efficiency and beam quality at IGISOL
The laser ion source project at the IGISOL facility, Jyvaskyla, has motivated the development and construction of an rf sextupole ion beam guide (SPIG) to replace the original skimmer electrode. The SPIG has been tested both off-line and on-line in proton-induced fission, light-ion and heavy-ion induced fusion-evaporation reactions and, in each case, has been directly compared to the skimmer system. For both fission and light-ion induced fusion, the SPIG has improved the mass-separated ion yields by a factor of typically 4 to 8. Correspondingly, the transmission efficiency of both systems has been studied in simulations with and without space charge effects. The transport capacity of the SP…
Improvements on Decay Heat Summation Calculations by Means of Total Absorption Gamma-ray Spectroscopy Measurements
The decay heat of fission products plays an important role in predictions of the heat released by nuclear fuel in reactors. In this contribution we present results of the analysis of the measurement of the beta decay of some refractory isotopes that were considered possible important contributors to the decay heat in reactors. The measurements presented here were performed at the IGISOL facility of the University of Jyvaeskylae, Finland. In our measurements we have combined for the first time a Penning trap (JYFLTRAP), which was used as a high resolution isobaric separator, with a total absorption spectrometer. The results of the measurements as well as their consequences for decay heat sum…
Gas jet studies towards an optimization of the IGISOL LIST method
Abstract Gas jets emitted from an ion guide have been studied as a function of nozzle type and gas cell-to-background pressure ratio in order to obtain a low divergent, uniform jet over a distance of several cm. The jet has been probed by imaging the light emitted from excited argon or helium gas atoms. For a simple exit hole or converging-diverging nozzle, the jet diameter was found to be insensitive to the nozzle shape and inlet pressure. Sonic jets with a FWHM below 6 mm were achieved with a background pressure larger than 1 mbar in the expansion chamber. The measurements are supported by the detection of radioactive 219 Rn recoils from an alpha recoil source mounted within the gas cell.…
JYFLTRAP: a Penning trap for precision mass spectroscopy and isobaric purification
In this article a comprehensive description and performance of the double Penning-trap setup JYFLTRAP will be detailed. The setup is designed for atomic mass measurements of both radioactive and stable ions and additionally serves as a very high-resolution mass separator. The setup is coupled to the IGISOL facility at the accelerator laboratory of the University of Jyväskylä. The trap has been online since 2003 and it was shut down in the summer of 2010 for relocation to the upgraded IGISOL facility. Numerous atomic mass and decay energy measurements have been performed using the time-of-flight ion-cyclotron resonance technique. The trap has also been used in several decay spectroscopy expe…
A facility for fast-neutron irradiations at Jyväskylä and its use for nuclide cross-section measurements in fission
Abstract An efficient and reliable transport system for fast-neutron irradiations has been built at the Physics Department, Jyvaskyla, Finland. It is constructed from commercial bicycle components and is driven by a computer-controlled stepping motor. It can be operated in single or cyclic mode. The neutron irradiated targets are moved within 1.2 s (full stop to full stop) to a well-shielded position 3 m away where they can be removed or directly investigated by γ spectroscopy. The system has been built with the aim to experimentally verify the calculated production rates of neutron-rich nuclei in the SPIRAL2 uranium target. However, the facility can be used for various kinds of fast-neutro…
Trap-assisted separation of nuclear states for gamma-ray spectroscopy: the example of100Nb
Low-lying levels in 100Mo are known to be populated by beta decay from both the ground and isomeric states in 100Nb. The small energy difference (~3 ppm) between the two parent states and the similarity of their half-lives make it difficult to distinguish experimentally between the two decay paths. A new technique for separating different states of nuclei has recently been developed in a series of experiments at the IGISOL facility, using the JYFLTRAP installation, at the University of Jyvaskyla where mass resolution ~2 ppm was achieved in mass measurements and in the production of 133mXe. This paper reports on the extension of this technique to allow the separate study of the gamma-ray dec…
An ion guide for the production of a low energy ion beam of daughter products of α-emitters
A new ion guide has been modeled and tested for the production of a low energy ($\approx$ 40 kV) ion beam of daughter products of alpha-emitting isotopes. The guide is designed to evacuate daughter recoils originating from the $\alpha$-decay of a $^{233}$U source. The source is electroplated onto stainless steel strips and mounted along the inner walls of an ion guide chamber. A combination of electric fields and helium gas flow transport the ions through an exit hole for injection into a mass separator. Ion guide efficiencies for the extraction of $^{229}$Th$^{+}$ (0.06%), $^{221}$Fr$^{+}$ (6%), and $^{217}$At$^{+}$ (6%) beams have been measured. A detailed study of the electric field and …
Total absorption study of theβdecay of102,104,105Tc
The $\ensuremath{\beta}$-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely ${}^{102,104,105}$Tc, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations.
New isomer and decay half-life ofRu115
Exotic, neutron-rich nuclei of mass $A=115$ produced in proton-induced fission of $^{238}\mathrm{U}$ were extracted using the IGISOL mass separator. The beam of isobars was transferred to the JYFLTRAP Penning trap system for further separation to the isotopic level. Monoisotopic samples of $^{115}\mathrm{Ru}$ nuclei were used for $\ensuremath{\gamma}$and $\ensuremath{\beta}$ coincidence spectroscopy. In $^{115}\mathrm{Ru}$ we have observed excited levels, including an isomer with a half-life of 76(6) ms and ($7/{2}^{\ensuremath{-}}$) spin and parity. The first excited 61.7-keV level in $^{115}\mathrm{Ru}$ with spins and parity ($3/{2}^{+}$) may correspond to an $\mathit{oblate}$ $3/{2}^{+}$…