0000000001227692

AUTHOR

Marco Peccianti

Solid-state-biased coherent detection of ultra-broadband terahertz pulses

Significant progress in nonlinear and ultrafast optics has recently opened new and exciting opportunities for terahertz (THz) science and technology, which require the development of reliable THz sources, detectors, and supporting devices. In this work, we demonstrate the first solid-state technique for the coherent detection of ultra-broadband THz pulses (0.1-10 THz), relying on the electric-field-induced second-harmonic generation in a thin layer of ultraviolet fused silica. The proposed CMOS-compatible devices, which can be realized with standard microfabrication techniques, allow us to perform ultra-broadband detection with a high dynamic range by employing probe laser powers and bias v…

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Invited Article: Ultra-broadband terahertz coherent detection via a silicon nitride-based deep sub-wavelength metallic slit

We present a novel class of CMOS-compatible devices aimed to perform the solid-state-biased coherent detection of ultrashort terahertz pulses, i.e., featuring a gap-free bandwidth at least two decades-wide. Such a structure relies on a 1-µm-wide slit aperture located between two parallel aluminum pads, embedded in a 1-µm-thick layer of silicon nitride, and deposited on a quartz substrate. We show that this device can detect ultra-broadband terahertz pulses by employing unprecedented low optical probe energies of only a few tens of nanojoules. This is due to the more than one order of magnitude higher nonlinear coefficient of silicon nitride with respect to silica, the nonlinear material emp…

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Counter-propagating difference frequency mixing in diamond with terahertz waves

We investigate four-wave mixing between terahertz and optical pulses in diamond. We observe the occurrence of sum and difference frequency generation, with the latter being phase-matched for terahertz pulses counter-propagating to the optical field.

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3084329.pdf

Supplementary Materials

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Wideband THz time domain spectroscopy based on optical rectification and electro-optic sampling

We present an analytical model describing the full electromagnetic propagation in a THz time-domain spectroscopy (THz-TDS) system, from the THz pulses via Optical Rectification to the detection via Electro Optic-Sampling. While several investigations deal singularly with the many elements that constitute a THz-TDS, in our work we pay particular attention to the modelling of the time-frequency behaviour of all the stages which compose the experimental set-up. Therefore, our model considers the following main aspects: (i) pump beam focusing into the generation crystal; (ii) phase-matching inside both the generation and detection crystals; (iii) chromatic dispersion and absorption inside the c…

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Exact reconstruction of thz sub-λ source features in knife-edge measurements

The spatial features of a sub-wavelength terahertz source are not accessible using time-integrated knife-edge techniques due to the non-separable space-time nature of the radiated field and to systematic modifications induced by the blade itself. We show that combining knife-edge with a time resolved electro-optical sampling, the space-time coupling can be addressed and the source field profile can be exactly reconstructed.

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Affordable, ultra-broadband coherent detection of terahertz pulses via CMOS-compatible solid-state devices

We demonstrate the first fully solid-state technique for the coherent detection of ultra-broadband THz pulses (0.1-10 THz), relying on the electric-field-induced second-harmonic generation attained in integrated CMOS-compatible devices.

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Observation of collapse arrest in pure kerr media sustained by a parametric interaction

We demonstrate a parametric interaction based on four wave mixing that can arrest the collapse and stabilize solitary propagation in a pure Kerr material by controlling the wavelength of the interacting beams.

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Space-time features of THz emission from optical rectification in sub-wavelength areas

We present our investigation on the THz space-time emission characteristic induced by the non-paraxial generation regime in highly localized THz generation via optical rectification on sub-wavelength areas.

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Asymmetric Dual-Grating Micro-Slit Configuration for Broadband Solid State Coherent Detection of THz Pulses

We demonstrated solid-state broadband coherent Terahertz characterization based on the Terahertz Field Induced Second Harmonic effect in Silica. The THz detector consists of an asymmetric micro-slit array which can be operated at 200V applied bias.

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Silicon nitride-based deep sub-λ slit for ultra-broadband THz coherent detection

We report on the characterization of a new type of CMOS-compatible device for terahertz solid-state biased coherent detection, which relies on a 1-µm-wide metallic slit embedded in a thin film of PECVD-grown silicon nitride.

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Counter-propagating frequency mixing with Terahertz waves in diamond

Frequency conversion by means of Kerr nonlinearity is one of the most common and exploited nonlinear optical processes in the UV, visible, IR, and mid-IR spectral regions. Here we show that wave mixing of an optical field and a terahertz wave can be achieved in diamond, resulting in the frequency conversion of the terahertz radiation either by sum- or difference-frequency generation. In the latter case, we show that this process is phase matched and most efficient in a counterpropagating geometry.

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A wideband THz Time Domain Spectroscopy table-top system based on ultrafast pulsed laser: Model and experiments

We present an analytical model carefully describing the time-frequency behavior of all the stages composing our whole Terahertz Time Domain Spectroscopy laser based system, from the THz pulses generation via Optical Rectification, to their detection through Electro-Optic Sampling technique, by way of diffraction, collecting and focusing effects. In order to prove the effectiveness of our work, we report on the comparison among the experimental waveforms and the simulation results.

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Spatio-temporal Characteristics of THz Emission at the Subwavelength Scale via Optical Rectification

Highly localized THz emission via optical rectification in thin nonlinear crystals is a promising method for subwavelength microscopy. We present here the peculiar THz spatio-temporal characteristics induced by the non-paraxial generation regime.

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Spatial and spectral properties of small area THz generation for sub-wavelength microscopy

A highly localized THz source is a promising candidate for sub-wavelength microscopy, due to its superior radiation power throughput with respect to others near-field techniques. Here, we report on the spatial and the spectral near-field properties of our highly localized THz source.

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Counter-propagating difference-frequency generation in diamond with terahertz fields

The nonlinear interaction of terahertz (THz) pulses with optical fields in Kerr, gaseous media is a key ingredient for broadband THz detection schemes [1]. Terahertz field-induced second harmonic generation in solid-state media has also been considered for THz detection and as a tool e.g. for liquid dynamics investigations [2,3], while four-wave mixing has been addressed as a possible mechanism for THz generation [4,5]. © 2013 IEEE.

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Supplementary document for Hyperspectral terahertz microscopy via nonlinear ghost-Imaging - 4386178.pdf

Supplementary Material

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Hyperspectral terahertz microscopy via nonlinear ghost imaging

Ghost imaging, based on single-pixel detection and multiple pattern illumination, is a crucial investigative tool in difficult-to-access wavelength regions. In the terahertz domain, where high-resolution imagers are mostly unavailable, ghost imaging is an optimal approach to embed the temporal dimension, creating a “hyperspectral” imager. In this framework, high resolution is mostly out of reach. Hence, it is particularly critical to developing practical approaches for microscopy. Here we experimentally demonstrate time-resolved nonlinear ghost imaging, a technique based on near-field, optical-to-terahertz nonlinear conversion and detection of illumination patterns. We show how space–time c…

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