6533b856fe1ef96bd12b26bd

RESEARCH PRODUCT

Strain pattern in supercooled liquids

Sebastian FritschiMatthias FuchsBernd IllingPeter KeimDavid HajnalChristian L. Klix

subject

PhysicsCondensed matter physicsStrain (chemistry)Zero (complex analysis)FOS: Physical sciencesGeneral Physics and AstronomyVideo microscopy02 engineering and technologyCondensed Matter - Soft Condensed Matter021001 nanoscience & nanotechnology01 natural sciencesShear modulusCondensed Matter::Soft Condensed Matter0103 physical sciencesShear stressSoft Condensed Matter (cond-mat.soft)ddc:530010306 general physics0210 nano-technologySupercoolingGlass transitionBrownian motion

description

Investigations of strain correlations at the glass transition reveal unexpected phenomena. The shear strain fluctuations show an Eshelby-strain pattern ($\,\sim \cos{(4\theta)}/r^2\,$), characteristic for elastic response, even in liquids at long times [1]. We address this using a mode-coupling theory for the strain fluctuations in supercooled liquids and data from both, video microscopy of a two-dimensional colloidal glass former and simulations of Brownian hard disks. We show that long-ranged and long-lived strain-signatures follow a scaling law valid close to the glass transition. For large enough viscosities, the Eshelby-strain pattern is visible even on time scales longer than the structural relaxation time $\tau$ and after the shear modulus has relaxed to zero.

10.1103/physrevlett.117.208002http://arxiv.org/abs/1606.03353