6533b85dfe1ef96bd12bdbd2

RESEARCH PRODUCT

Resonant hyper-Raman scattering in semiconductors: Excitonic effects

Andrés CantareroAlberto García-cristóbalCarlos Trallero-ginerManuel Cardona

subject

PhysicsCondensed matter physicsPhonon scatteringScatteringScattering lengthMott scatteringInelastic scatteringCondensed Matter PhysicsElectronic Optical and Magnetic MaterialsResonant inelastic X-ray scatteringX-ray Raman scatteringPhysics::Atomic PhysicsScattering theoryElectrical and Electronic Engineering

description

Abstract A theoretical model of resonant hyper-Raman scattering involving two incident photons of frequency ωL is developed. The model is valid for energies 2ℏωL around the absorption edge of the semiconductor, and takes into account Wannier excitons as intermediate states in the scattering process. Both deformation potential and Frohlich interaction are included in the model: It is found that Frohlich-mediated scattering is a dipole-allowed process, in contrast to one-phonon Raman scattering, where the Frohlich mechanism is dipole-forbidden. We have performed numerical calculations of the resonance profile (hyper-Raman cross-section versus 2ℏωL) and applied our model to materials with dipole-allowed and dipole-forbidden optical transitions.

https://doi.org/10.1016/s0921-4526(98)01462-8