6533b870fe1ef96bd12cf9ec

RESEARCH PRODUCT

Epitaxial film growth and magnetic properties ofCo2FeSi

Benjamin BalkeMartin AeschlimannGerhard JakobH. AdrianS. WurmehlMirko CinchettiM. KallmayerClaudia FelserH. SchneiderH. J. Elmers

subject

Materials scienceSpin polarizationMagnetic momentCondensed matter physicsMagnetic circular dichroismSputter depositionengineering.materialCondensed Matter PhysicsHeusler compoundElectronic Optical and Magnetic MaterialsCondensed Matter::Materials ScienceMagnetizationElectrical resistivity and conductivityengineeringAnisotropy

description

We have grown thin films of the Heusler compound ${\mathrm{Co}}_{2}\mathrm{Fe}\mathrm{Si}$ by RF magnetron sputtering. On (100)-oriented MgO substrates we find fully epitaxial (100)-oriented and $L{2}_{1}$ ordered growth. On ${\mathrm{Al}}_{2}{\mathrm{O}}_{3}(11\overline{2}0)$ substrates, the film growth is (110)-oriented, and several in-plane epitaxial domains are observed. The temperature dependence of the electrical resistivity shows a power law with an exponent of $7∕2$ at low temperatures. Investigation of the bulk magnetic properties reveals an extrapolated saturation magnetization of $5.0{\ensuremath{\mu}}_{B}∕\mathrm{f.u.}$ at $0\phantom{\rule{0.3em}{0ex}}\mathrm{K}$. The films on ${\mathrm{Al}}_{2}{\mathrm{O}}_{3}$ show an in-plane uniaxial anisotropy, while the epitaxial films are magnetically isotropic in the plane. Measurements of the x-ray magnetic circular dichroism of the films allowed us to determine element specific magnetic moments. Finally we have measured the spin polarization at the surface region by spin-resolved near-threshold photoemission and found it strongly reduced in contrast to the expected bulk value of 100%. Possible reasons for the reduced magnetization are discussed.

https://doi.org/10.1103/physrevb.74.174426