Search results for " Clusters"
showing 10 items of 1091 documents
Many-body origin of the plasmon resonance in small metal clusters
1994
The origin of the plasmon excitation in small metal clusters is studied within the jellium model through ab initio electronic-structure calculations based on the nuclear shell model. In the limit of infinite size, the plasmon classically represents pure harmonic motion of the center of mass of the valence electrons. It is shown that this limit is already well approximated by clusters of only eight electrons.
Imaging Static Charge Distributions: A Comprehensive KPFM Theory
2018
We analyze Kelvin probe force microscopy (KPFM) for tip-sample systems that contain static charges by presenting a rigorous derivation for the respective KPFM signal in all common KPFM modes, namely amplitude modulation, frequency modulation, or heterodyne detection in the static, open-loop or closed-loop variant. The electrostatic model employed in the derivation is based on a general electrostatic analysis of an arbitrary tip-sample geometry formed by two metals, and which can include a static charge distribution and dielectric material in-between. The effect of the electrostatic force on the oscillating tip is calculated from this model within the harmonic approximation, and the observab…
Simulations of continuous-wave sodium laser guide stars with polarization modulation at Larmor frequency
2018
The return flux from a sodium laser guide star suffers, at large angles between the geomagnetic field and the laser beam, from the reduction in optical pumping due to spin-precession of sodium atoms. This detrimental effect can be mitigated by modulating the circular polarization of a continuous-wave laser beam in resonance with the Larmor frequency of sodium atoms in the mesosphere. We present an investigation based on numerical modeling to evaluate the brightness enhancement of a laser guide star with polarization modulation of a continuous-wave laser beam at different observatories.
Calculated Line Broadening Coefficients in the nu2 Band of CH3D Perturbed by Helium
2003
International audience; Line broadening coefficients have been calculated, at room temperature, for lines in the P and R branches of the nu2 band of monodeuterated methane. A properly symmetrized semiclassical model with parabolic relative trajectories has been used. Two interaction potential models have been considered. The first is a Lennard-Jones type atom-atom potential, while the second one was derived from ab initio calculations. The calculated line widths were compared to the available experimental data and a satisfactory agreement was found, although the model contains no other adjustable parameters than the four atomic Lennard-Jones ones. Nonetheless, failures of calculations have …
On the observability of Bell's inequality violation in the two-atoms optical Stern-Gerlach model
2005
Using the optical Stern-Gerlach model, we have recently shown that the non-local correlations between the internal variables of two atoms that successively interact with the field of an ideal cavity in proximity of a nodal region are affected by the atomic translational dynamics. As a consequence, there can be some difficulties in observing violation of the Bell's inequality for the atomic internal variables. These difficulties persist even if the atoms travel an antinodal region, except when the spatial wave packets are exactly centered in an antinodal point.
Shape coexistence in Au 187 studied by laser spectroscopy
2020
Hyperfine-structure parameters and isotope shift of the 9/2$^−$ isomeric state in $^{187}$Au relative to $^{197}$Au for the 267.6-nm atomic transition have been measured for the first time using the in-source resonance-ionization spectroscopy technique. The magnetic dipole moment and change in the mean-square charge radius for this 9/2$^−$ isomer have been deduced. The observed large isomer shift relative to the 1/2$^+$ ground state in $^{187}$Au confirms the occurrence of the shape coexistence in $^{187}$Au proposed earlier from the analysis of the nuclear spectroscopic data and particle plus triaxial rotor calculations. The analysis of the magnetic moment supports the previously proposed …
Electro- and photodisintegration of deuterium
1978
Deuteron break-up by inelastic electron scattering or photoabsorption is discussed with emphasis on effects from meson exchange currents and isobar configurationgurations.
A paradigm of fullerene
2009
We study the dynamics of an electron constrained over the surface of a rigid sphere, with geometrical parameters similar to those of the C60 fullerene, embedded in a low intensity linearly polarized laser field. The model is shown to emit odd harmonics of the laser even at very low field intensity. For more intense laser fields, the spectrum presents odd harmonics and hyper-Raman lines shaped in a broad plateau. The spectrum of the model is compared to that theoretically obtained by other authors for more realistic models of C60. It is concluded that the model can be used as a paradigm for mesoscopic molecules in the fullerene family, particularly in practical applications where it is conve…
Stability chart of small mixed4He−3Heclusters
2003
A stability chart of mixed ${}^{4}\mathrm{He}$ and ${}^{3}\mathrm{He}$ clusters has been obtained by means of the diffusion Monte Carlo method, using both the Aziz HFD-B and the Tang-Toennies-Yiu atom-atom interaction. The investigated clusters contain up to eight ${}^{4}\mathrm{He}$ atoms and up to 20 ${}^{3}\mathrm{He}$ atoms. One single ${}^{4}\mathrm{He}$ binds 20 ${}^{3}\mathrm{He}$ atoms, and two ${}^{4}\mathrm{He}$ bind 1, 2, 8, and more than 14 ${}^{3}\mathrm{He}$ atoms. All clusters with three or more ${}^{4}\mathrm{He}$ atoms are bound, although the combinations ${}^{4}{\mathrm{He}}_{3}^{3}{\mathrm{He}}_{9,10,11}$ and ${}^{4}{\mathrm{He}}_{4}^{3}{\mathrm{He}}_{9}$ are metastable. …
Helium bubbles in metals: Molecular-dynamics simulations and positron states.
1987
By combining molecular-dynamics results for the aluminum-helium interface with positron-state calculations it is demonstrated that a positron is trapped at the surface of a He bubble in Al. The annihilation rate with Al electrons is similar to that at a clean surface, while simultaneously there is a significant annihilation rate with He electrons. This enables one to obtain a useful relation between the positron lifetime and helium densities in bubbles.