Search results for " SOLID"

showing 10 items of 1333 documents

From Single Molecules to Nanoscopically Structured Functional Materials

2006

AbstractThe synthesis of MS2 (M = Mo, W) onion-like nanoparticles by means of a high temperature MOCVD process starting from W(CO)6 and elemental sulfur is reported. The reaction can also be carried out in two steps where the intermediate amorphous WS2 nanoparticles formed through the high temperature reaction of tungsten and sulfur in the initial phase of the reaction are isolated and converted in a separate annealing step to onion-type WS2 nanoparticles. Based on a study of the temperature dependence of the reaction a set of conditions could be derived where onion-like structures were formed in a one-step reaction. Onion-like structures obtained in the single-step process were filled, whe…

chemistry.chemical_compoundMaterials scienceNanostructurechemistryChemical engineeringAnnealing (metallurgy)ChalcogenideMoleculechemistry.chemical_elementNanoparticleSurface modificationTungstenAmorphous solidMRS Proceedings
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Influence de l'atmosphère gazeuse sur la cinétique de formation du titanate de baryum par réaction solide-solide

1986

International audience; Les études consacrées à la synthèse, par réaction solide-solide, du titanate de baryum (BaTiO3) ont montré l'importance des propriétés physicochimiques des solides initiaux (BaCO3 et TiO2) sur les propriétés du titanate obtenu. Lors de l'élaboration de céramiques diélectriques, il est en effet nécessaire d'éviter la formation de phases intermédiaires (Ba2TiO4, BaTi4O9, ...) qui nuisent à leurs propriétés diélectriques. La présence de ces phases peut être liée à une maîtrise imparfaite des nombreux paramètres influant sur la cinétique de la réaction. Le rôle de deux de ces paramètres : les traitements mécaniques et la nature de l'atmosphère gazeuse, fait l'objet de ce…

cinétiqueatmosphère gazeuse[SPI.GPROC] Engineering Sciences [physics]/Chemical and Process Engineeringpropriétés diélectriquesréaction solide-solide[SPI.GPROC]Engineering Sciences [physics]/Chemical and Process Engineeringtraitements mécaniques[ SPI.GPROC ] Engineering Sciences [physics]/Chemical and Process Engineeringtitanate de baryum
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Il progetto CEAS: quando l’educazione alla cittadinanza è già attiva e solidale. Buone pratiche di educazione alla solidarietà

2005

cittadinanza diritti integrazione solidarietàSettore M-PED/03 - Didattica E Pedagogia Speciale
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Alkylsilyl compounds as enablers of atomic layer deposition: analysis of (Et3Si)3As through the GaAs process

2016

A new chemistry has been developed to deposit GaAs, the quintessential compound semiconductor. The ALD process is based on a dechlorosilylation reaction between GaCl3 and (Et3Si)3As. Characteristic ALD growth was demonstrated, indicating good applicability of the alkylsilyl arsenide precursor. ALD of GaAs produced uniform, amorphous and stoichiometric films with low impurity content. This was done with saturating growth rates and an easily controlled film thickness. Crystallization was achieved by annealing. Even though the growth rate strongly decreased with increasing deposition temperature, good quality film growth was demonstrated at 175 to 200 °C, indicating the presence of an ALD wind…

compound semiconductorsMaterials scienceAnnealing (metallurgy)Analytical chemistry02 engineering and technology010402 general chemistryEpitaxy01 natural sciencesArsenidelaw.inventionAtomic layer depositionchemistry.chemical_compoundGallium arsenideImpuritylawMaterials ChemistryThin filmCrystallizationta216ta116ta114General Chemistry021001 nanoscience & nanotechnology0104 chemical sciencesAmorphous solidamorphous filmschemistry0210 nano-technologystoichiometric filmsJournal of Materials Chemistry C
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Increased conformational rigidity of humic substances by oxidative biomimetic catalysis

2005

A synthetic water-soluble meso-tetra(2,6-dichloro-3-sulfonatophenyl)porphyrinate of iron(III) chloride, Fe(TDCPPS)Cl, was employed as a biomimetic catalyst in the oxidative coupling of terrestrial humic materials. High-performance size-exclusion chromatography (HPSEC), solid-state nuclear magnetic resonance (CPMAS-(13)C NMR), electron paramagnetic resonance (EPR), and diffuse reflectance infrared spectroscopy (DRIFT) were used to follow conformational and structural changes brought about in different humic materials by the oxidative coupling. Increase in apparent weight-average molecular weight (Mw(a)) occurred invariably for all humic substances with the oxidative polymerization catalyzed …

conformationMagnetic Resonance SpectroscopySpectrophotometry InfraredPolymers and PlasticsDiffuse reflectance infrared spectroscopy (DRIFT)Biomimetic materialsaromatic compoundgel permeation chromatographyMolecular ConformationPhotochemistryIron compoundslaw.inventionPolymerizationenvironmental managementcovalent bondlawSize exclusion chromatographyBiomimetic catalysisBiomimeticsMaterials ChemistryOrganic chemistryHumic acidElectron paramagnetic resonanceInfrared spectroscopyChromatography High Pressure Liquidchemistry.chemical_classificationSettore CHIM/03 - Chimica Generale e InorganicaCarbon IsotopesChromatographyindustryCatalystsChemistrytetra(2articleelectrophoretic mobilitybiomimetic materialNuclear magnetic resonance spectroscopyunclassified drugConformationsacetic acidpriority journalCovalent bondSpectrophotometrySynthesis (chemical)High Pressure Liquidtechnology6 dichloro 3 sulfonatophenyl)porphyrinic acid derivativeInfraredOxidation-Reductionmolecular stabilityHumic materialsoxidationSettore AGR/13 - Chimica AgrariaSupramolecular chemistryBioengineeringcomplex mixturesCatalysisCatalysisdiffuse reflectance spectroscopyhumic substanceBiomaterialsalkyl etherElectron spin resonance spectroscopycomplex formationParticle SizeNuclear magnetic resonance spectroscopyHumic Substancesfree radicalbiomimetic oxidative humicelectron spin resonanceHigh performance size exclusion chromatography (HPSEC)ferrous chloridemolecular weightsolid statecarbon nuclear magnetic resonancePolymerizationSolubilitychemical structureOxidative coupling of methaneCatalysts; Conformations; Electron spin resonance spectroscopy; Infrared spectroscopy; Iron compounds; Nuclear magnetic resonance spectroscopy; Oxidation; Polymerization; Size exclusion chromatography; Solubility; Synthesis (chemical); Biomimetic catalysis; Diffuse reflectance infrared spectroscopy (DRIFT); High performance size exclusion chromatography (HPSEC); Humic materials; Biomimetic materials; acetic acid; alkyl ether; aromatic compound; biomimetic material; ferrous chloride; free radical; tetra(26 dichloro 3 sulfonatophenyl)porphyrinic acid derivative; unclassified drug; article; carbon nuclear magnetic resonance; catalysis; catalyst; chemical structure; complex formation; conformation; covalent bond; diffuse reflectance spectroscopy; electron spin resonance; electrophoretic mobility; environmental management; gel permeation chromatography; humic substance; industry; molecular stability; molecular weight; oxidation; polymerization; priority journal; solid state; technology; Biomimetics; Carbon Isotopes; Catalysis; Chromatography High Pressure Liquid; Electron Spin Resonance Spectroscopy; Humic Substances; Magnetic Resonance Spectroscopy; Molecular Conformation; Oxidation-Reduction; Particle Size; Spectrophotometry Infraredcatalyst
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Agere 'ex asse in solidum' e agere 'pro parte in solidum'. Per un'interpretazione di Venul. 7 stip. D. 10, 2, 7

2020

The paper proposes a revised analysis of D. 10.2.7 (Venul. 7 stip.), from which it seems reasonable to suggest that Venuleius discussed a particular kind of co-inheritance: the coniunctim attribution of a hereditas or an inheritance quota regarding two heirs. The substantially classical text, which can be glimpsed therein, offers evidence of the coexistence of different patterns of co-inheritance in classical private Roman law.

coniunctioCommunio coeredità Venuleio agere in solidumSettore IUS/18 - Diritto Romano E Diritti Dell'Antichita'
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La vegetazione a protezione di processi di escavazione localizzata: risultati di uno studio sperimentale

2018

Diversi studi di letteratura mostrano come la vegetazione debba essere considerata un fattore chiave per analizzare i meccanismi di trasporto che si realizzano lungo un corso d’acqua naturale (Jarvela, 2002; Folkard, 2011). In particolare, la presenza di vegetazione sul fondo e/o sulle sponde del corso d’acqua contribuisce sia a stabilizzare i sedimenti che ad aumentare la resistenza al moto della corrente (Tsujimoto 1999; Nepf and Vivoni, 2000; Afzalimehr and Dey, 2009; Nepf, 2012), influenzando i processi di trasporto solido e i conseguenti fenomeni di erosione e di deposito lungo lo stesso corso d’acqua. In questo contesto, nel presente lavoro sono riportati alcuni risultati di uno studi…

corsi d'acqua erosione trasporto solido vegetazioneSettore ICAR/01 - Idraulica
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Opere di sistemazione idraulico-forestale

2019

Il volume illustra, nella visione unitaria del sistema “bacino idrografico”, i processi fisici, le problematiche applicative e le tipologie di intervento disponibili per la sistemazione del reticolo fluviale e dei versanti. Il trasporto solido delle correnti a pelo libero viene introdotto con l’intento di esaminare i processi evolutivi del cavo fluviale, di fornire indicazioni per la progettazione delle opere di correzione ed inalveazione del tracciato del corso d’acqua e di stabilire l’influenza dell’inserimento di manufatti sul delicato equilibrio del sistema fluviale. La trattazione, seguendo il percorso della corrente dalle propaggini più montane fino allo sbocco a mare, esamina opere c…

costruzioni idraulichecorsi d'acquaidraulicatrasporto solidoSettore AGR/08 - Idraulica Agraria E Sistemazioni Idraulico-Forestali
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Un «salto di specie» per l’UE? La solidarietà europea alla prova della crisi pandemica

2020

La crisi da covid-19 ha riportato al centro del dibattito gli interrogativi sull’effettiva portata della solidarietà europea, quale parte integrante del modello sociale dell’Unione. L’emergenza sanitaria ha mostrato i limiti del processo di integrazione sovranazionale, caratterizzato da un perdurante deficit di legittimazione democratica dell’Unione e dall’assenza di strumenti di condivisione dei rischi tra gli Stati membri. Il paper ripercorre le iniziative prese dalle Istituzioni europee per fronteggiare la crisi pandemica, mettendo in evidenza il cambio di passo dell’Unione rispetto alla precedente crisi finanziaria, e soffermandosi sulle prospettive di approfondimento della sua dimensio…

covid-19 europa solidarietà diritti sociali lavoro
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Enhancing the luminescence efficiency of silicon-nanocrystals by interaction with H+ions

2018

The emission of silicon nanocrystals (Si-NCs), synthesized by pulsed laser ablation in water, was investigated on varying the pH of the solution. These samples emit μs decaying orange photoluminescence (PL) associated with radiative recombination of quantum-confined excitons. Time-resolved spectra reveal that both the PL intensity and the lifetime increase by a factor of ∼20 when the pH decreases from 10 to 1 thus indicating that the emission quantum efficiency increases by inhibiting nonradiative decay rates. Infrared (IR) absorption and electron paramagnetic resonance (EPR) experiments allow addressing the origin of defects on which the excitons nonradiatively recombine. The linear correl…

defectMaterials sciencePhotoluminescenceExcitonGeneral Physics and Astronomy02 engineering and technology010402 general chemistryPhotochemistry01 natural sciencesIonlaw.inventionlawluminescenceSpontaneous emissionQuantum confinementPhysical and Theoretical ChemistryElectron paramagnetic resonanceSilicon nanocrystalsilicon021001 nanoscience & nanotechnologyphotoluminescence efficiencysilicon nanoparticles luminescence0104 chemical sciencesAmorphous solidlaser ablationQuantum efficiencynanoparticles0210 nano-technologyLuminescence
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