Search results for " Spectra"

showing 10 items of 709 documents

Ab initio determination of the ionization potentials of DNA and RNA nucleobases

2006

Quantum chemical high level ab initio coupled-cluster and multiconfigurational perturbation methods have been used to compute vertical and adiabatic ionization potentials of the five canonical DNA and RNA nucleobases: uracil, thymine, cytosine, adenine, and guanine. Several states of their cations have been also calculated. The present results represent a systematic compendium of these magnitudes, establishing theoretical reference values at a level not reported before, calibrating computational strategies, and guiding the assignment of the features in the experimental photoelectron spectra. Daniel.Roca@uv.es Mercedes.Rubio@uv.es Manuela.Merchan@uv.es Luis.Serrano@uv.es

DNA ; Macromolecules ; Ionisation potential ; Photoelectron spectra ; Molecular biophysics ; Ab initio calculations ; Coupled cluster calculations ; Perturbation theoryGuanineGuaninePhotochemistryAb initioBiophysicsGeneral Physics and AstronomyIonisation potentialPerturbation theoryNucleobasechemistry.chemical_compoundCytosinePhotoelectron spectraCoupled cluster calculationsAb initio quantum chemistry methodsComputational chemistryIonizationPhysics::Atomic and Molecular ClustersPhysical and Theoretical ChemistryUracil:FÍSICA::Química física [UNESCO]IonsPhysics::Biological PhysicsQuantitative Biology::BiomoleculesBase CompositionChemistry PhysicalAdenineUracilDNAMolecular biophysicsQuantitative Biology::GenomicsThymineUNESCO::FÍSICA::Química físicachemistryMacromoleculesCalibrationQuantum TheoryRNAAb initio calculationsCytosineSoftwareThymine
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A new fast and fault-tolerant identification algorithm for spectral databases

1995

A new method for an automatic, computer and database driven identification of UV/VIS spectra is described. It is shown that an identification algorithm must consider the spectral differences as well as their common features. The described identification method allows identifications, even if the spectra are distorted or shifted.

Data processingDatabaseComputer sciencePattern analysisFault toleranceVis spectraFuzzy control systemcomputer.software_genreBiochemistrySpectral lineAnalyse qualitativeAnalytical ChemistryIdentification (information)ComputingMethodologies_PATTERNRECOGNITIONcomputerAlgorithmAnalytical and Bioanalytical Chemistry
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Climate Data Records of Vegetation Variables from Geostationary SEVIRI/MSG Data: Products, Algorithms and Applications

2019

The scientific community requires long-term data records with well-characterized uncertainty and suitable for modeling terrestrial ecosystems and energy cycles at regional and global scales. This paper presents the methodology currently developed in EUMETSAT within its Satellite Application Facility for Land Surface Analysis (LSA SAF) to generate biophysical variables from the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) on board MSG 1-4 (Meteosat 8-11) geostationary satellites. Using this methodology, the LSA SAF generates and disseminates at a time a suite of vegetation products, such as the leaf area index (LAI), the fraction of the photosynthetically active radiation absorbed …

Data records010504 meteorology & atmospheric sciencesData productsSciencemeteosat second generation (MSG); biophysical parameters (LAI; FVC; FAPAR); SEVIRI; climate data records (CDR); stochastic spectral mixture model (SSMM); Satellite Application Facility for Land Surface Analysis (LSA SAF)0211 other engineering and technologiesstochastic spectral mixture model (SSMM)02 engineering and technology01 natural sciencesFAPAR)climate data records (CDR)Leaf area index021101 geological & geomatics engineering0105 earth and related environmental sciencesQVegetationSEVIRIMixture modelSatellite Application Facility for Land Surface Analysis (LSA SAF)FVCbiophysical parameters (LAIPhotosynthetically active radiationGeostationary orbitGeneral Earth and Planetary SciencesEnvironmental sciencemeteosat second generation (MSG)SatelliteAlgorithmRemote Sensing; Volume 11; Issue 18; Pages: 2103
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Etude numérique d'équations aux dérivées partielles non linéaires et dispersives

2011

Numerical analysis becomes a powerful resource in the study of partial differential equations (PDEs), allowing to illustrate existing theorems and find conjectures. By using sophisticated methods, questions which seem inaccessible before, like rapid oscillations or blow-up of solutions can be addressed in an approached way. Rapid oscillations in solutions are observed in dispersive PDEs without dissipation where solutions of the corresponding PDEs without dispersion present shocks. To solve numerically these oscillations, the use of efficient methods without using artificial numerical dissipation is necessary, in particular in the study of PDEs in some dimensions, done in this work. As stud…

Davey-Stewartson systems[ MATH.MATH-GM ] Mathematics [math]/General Mathematics [math.GM]equations dispersivesdispersive shocksexponential time-differencing[MATH.MATH-GM]Mathematics [math]/General Mathematics [math.GM][MATH.MATH-MP]Mathematics [math]/Mathematical Physics [math-ph]spectral methodschocs dispersifsnumerical methodsdispersive equationsNo english keywordssplit stepschemas de decomposition d'operateursmethodes spectrales[MATH.MATH-MP] Mathematics [math]/Mathematical Physics [math-ph]Kadomtsev-Petviashvili equationintegrating factor methodparallel computing[ MATH.MATH-MP ] Mathematics [math]/Mathematical Physics [math-ph]Pas de mot clé en français[MATH.MATH-GM] Mathematics [math]/General Mathematics [math.GM]methodes numeriquesblow upequation de Kadomtsev-PetviashviliIntegrateurs exponentielssystemes de Davey-Stewartsoncalcul parallele
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Perovskite CH3NH3PbI3–XClx Solar Cells. Experimental Study of Initial Degradation Kinetics and Fill Factor Spectral Dependence

2021

The main drawback of the methylammonium lead halide perovskite solar cells is their degradation in ambient atmosphere. To investigate ambient-air-induced cell degradation, spec-tral dependencies of open-circuit voltage (VOC), fill factor (FF) and the power conversion effi-ciency (PCE) have been acquired (for the first time reported in literature). Our custom-made measurement system allowed us to perform measurements of the above-mentioned entities in situ directly in vacuum during and after thermal deposition of the elec-trode. We also studied how these parameters in vacuum changed after cell exposure to ambient air for 85 min (50 nm top electrode) and for 180 min (100 nm top Ag electrode).…

Degradation kineticsSolid-state physicsQC1-999General Physics and AstronomyDegradation kinetics02 engineering and technology010402 general chemistry01 natural sciences7. Clean energy:NATURAL SCIENCES:Physics [Research Subject Categories]media_common.cataloged_instanceEuropean unionfill factor spectral dependencePerovskite (structure)media_commonPhysicsHorizon (archaeology)PhysicsEnergy conversion efficiencyGeneral Engineering021001 nanoscience & nanotechnologyEngineering physics0104 chemical sciencespower conversion efficiencydegradation kineticslead halide perovskitesolar cellsFill factor0210 nano-technology
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Red emitting [Ir(C^N)2(N^N)]+ complexes employing bidentate 2,2':6,2''-terpyridine ligands for light-emitting electrochemical cells

2014

2,2':6',2''-Terpyridine (tpy), 4'-(4-HOC6H4)-2,2':6',2''-terpyridine (1), 4'-(4-MeOC6H4)-2,2':6',2''-terpyridine (2), 4'-(4-MeSC6H4)-2,2':6',2''-terpyridine (3), 4'-(4-H2NC6H4)-2,2':6',2''-terpyridine (4) and 4'-(4-pyridyl)-2,2':6',2''-terpyridine (4) act as N^N chelates in complexes of the type [Ir(C^N)2(N^N)][PF6] in which the cyclometallating ligand, C^N, is derived from 2-phenylpyridine (Hppy) or 3,5-dimethyl-1-phenyl-1H-pyrazole (Hdmppz). The single crystal structures of eight complexes have been determined, and in each iridium(III) complex cation, the non-coordinated pyridine ring of the tpy unit is involved in a face-to-face π-stacking interaction with the cyclometallated ring of an …

DenticityChemistryHydrogen bondLigandAnalytical chemistrychemistry.chemical_elementInorganic ChemistryNMR spectra databasechemistry.chemical_compoundCrystallographyPyridineIridiumTerpyridineSingle crystal
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Characterization of complexes formed between [Me2Sn(IV)]2+ and carboxymethylcelluloses.

2006

Complexes formed between carboxymethylcellulose (CMC) and the [Me(2)Sn(IV)]2+ cation have been prepared in the solid state and characterized by FTIR and Mossbauer spectroscopy. The complexes contained CMC with varying molar weight and degree of carboxylation, and the complexes were isolated both from acidic and from neutral solutions at varying metal-to-ligand ratios. The characteristic vibration bands of the ligands were identified from their pH-dependent FTIR spectra. In the organotin(IV) complexes obtained at pH approximately 2, the -COO- moieties were found to be coordinated in a monodentate manner, and the band characteristic of the protonated (unbound) -COO- group(s) was also identifi…

DenticityMetal ions in aqueous solutionInorganic chemistryInfrared spectroscopyBiochemistryAnalytical ChemistrySpectroscopy MossbauerDeprotonationSpectroscopy Fourier Transform InfraredOrganotin CompoundsCarboxymethylcelluloseValence (chemistry)Sn(IV)Molecular StructureLigandChemistryOrganic ChemistryStructureTin CompoundsGeneral MedicineQuadrupole splittingInfrared spectraTrigonal bipyramidal molecular geometryCrystallographyCarboxymethylcellulose SodiumMössbauer spectraCarbohydrate research
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Trimethylplatinum(IV) complexes with ON bidentate ligands

1972

Abstract Complexes of the trimethylplatinum(IV) moiety with bidentate monobasic salicylaldimines C 6 H 5 (OH)CHNR (R = ethyl, propyl, phenyl) have been prepared and characterized by IR, UV and NMR spectra and magnetic susceptibility measurements. The complexes are dimeric with double PtOPt bridges, and the metal appears to be pseudo-octahedrally hexacoordinated.

DenticityStereochemistryChemistryMonobasic acidOrganic ChemistryBiochemistryMagnetic susceptibilityInorganic ChemistryNMR spectra databaseMetalvisual_artPolymer chemistryMaterials Chemistryvisual_art.visual_art_mediumMoietyPhysical and Theoretical ChemistryJournal of Organometallic Chemistry
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Development of an imaging system dedicated to the acquisition analysis and multispectral characterisation of skin lesion

2011

Visual evaluation of cutaneous lesions is the analysis the most commonly performedby dermatologists. This diagnostic is mainly done by naked eye and is based on criterionsuch as the size, shape, symmetry but principally on colour of the lesions. However, thisanalysis is subjective because it depends on the practician experience and the acquisitionconditions. We propose in this dissertation (1) the development of a multispectralcamera specifically dedicated for dermatological use. This device is based on a filterwheel composed of interferential filters and a neural network-based algorithm, generatinga hyperspectral cube of cutaneous data. This setting combines advantage of both spectrophotom…

Dermatologie[SDV.MHEP] Life Sciences [q-bio]/Human health and pathologyAlgorithmes évolutionnairesReconstruction spectrale[INFO.INFO-OH]Computer Science [cs]/Other [cs.OH]DermatologyLight propagation model in skinImagerie multispectrale[INFO.INFO-OH] Computer Science [cs]/Other [cs.OH]Multispectral imagingSpectral reconstructionModèle de propagation de la lumière dans la peau[ SDV.MHEP ] Life Sciences [q-bio]/Human health and pathology[ INFO.INFO-OH ] Computer Science [cs]/Other [cs.OH]Evolutionnary algorithms[SDV.MHEP]Life Sciences [q-bio]/Human health and pathology
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Raman scattering and infrared reflectivity in [(InP)5(In0.49Ga0.51As)8]30 superlattices

2000

6 páginas, 6 figuras, 1 tabla.

DiffractionMaterials scienceIII-V semiconductorsInfraredPhononSuperlatticeGeneral Physics and AstronomyReflectivityMolecular physicsSpectral linesymbols.namesakeCondensed Matter::Materials ScienceGallium arsenideIndium compounds:FÍSICA [UNESCO]Interface phononsbusiness.industryIndium compounds ; Gallium arsenide ; III-V semiconductors ; Semiconductor superlattices ; Raman spectra ; Infrared spectra ; Reflectivity ; Interface phonons ; Semiconductor epitaxial layersUNESCO::FÍSICASemiconductor epitaxial layersInfrared spectraCondensed Matter::Mesoscopic Systems and Quantum Hall EffectsymbolsOptoelectronicsRaman spectrabusinessRaman spectroscopySemiconductor superlatticesRaman scatteringMolecular beam epitaxy
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