Search results for " secondary"

showing 10 items of 692 documents

Manganese(iv) oxamato-catalyzed oxidation of secondary alcohols to ketones by dioxygen and pivalaldehyde

1998

A new manganese(IV) oxamato complex possessing a bis(moxo) dimanganese core has been synthesized, magnetically and structurally characterized, and found to catalyze the aerobic oxidation of secondary alcohols to ketones with cooxidation of pivalaldehyde to pivalic acid with good yields and high selectivities. Ruiz Garcia, Rafael, Rafael.Ruiz@uv.es ; Fernandez Picot, Isabel, Isabel.Fernandez@uv.es ; Pedro Llinares, Jose Ramon, Jose.R.Pedro@uv.es ; Rosello Arce, Antonio Luis, Antonio.L.Rosello@uv.es ; Castro Bleda, Isabel, Isabel.Castro@uv.es

ManganesePivalic acidDioxygenUNESCO::QUÍMICA::Química inorgánicaUNESCO::QUÍMICAMetals and Alloyschemistry.chemical_elementGeneral ChemistryManganeseKetones:QUÍMICA::Química inorgánica [UNESCO]:QUÍMICA [UNESCO]CatalysisSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsCatalysischemistry.chemical_compoundchemistryAlcoholsOxidationMaterials ChemistryCeramics and CompositesOxidation of secondary alcohols to ketonesOrganic chemistryManganese ; Oxidation ; Alcohols ; Ketones ; Dioxygen
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Self-Ordering Secondary Structure of d- and l-Arginine-Derived Polyamidoamino Acids

2017

This paper reports on synthesis, acid–base properties and pH-dependent structuring in water of d-, l- and d,l-ARGO7, bioinspired polymers obtained by polyaddition of the corresponding arginine stereoisomers with N,N′-methylenebis(acrylamide). The circular dichroism spectra of d- and l-ARGO7 showed a peak at 228 nm and quickly and reversibly responded to pH changes, but were nearly unaffected by temperature, ionic strength, and denaturating agents. Theoretical modeling studies of L-ARGO7 showed that it assumed a folded structure. Intramolecular interactions led to transoid arrangements of the main chain reminiscent of the protein hairpin motif. Torsion angles showed a quite similar distribut…

Materials Chemistry2506 Metals and AlloysMaterials scienceArgininePolymers and PlasticsStereochemistry02 engineering and technologyOrganic Chemistry; Polymers and Plastics; Inorganic Chemistry; Materials Chemistry2506 Metals and Alloys010402 general chemistry01 natural sciencesSpectral lineInorganic Chemistrychemistry.chemical_compoundMaterials ChemistryProtein secondary structurechemistry.chemical_classificationOrganic ChemistryPolymer021001 nanoscience & nanotechnology0104 chemical scienceschemistryChiral polymers polyamidoamino acids interpenetrating peptides self-structured polymersIonic strengthIntramolecular forceAcrylamide0210 nano-technologySelf ordering
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Experimental dynamic analysis of elastic-plastic shear frames with secondary structures

2003

Various experimental models are developed to study the influence of lightweight secondary structures on the dynamic response of elastic and elastic-plastic shear frames. Small-scale two-story model frames, with an elastic single-degree-of-freedom secondary structure attached, are considered for sinusoidal and random in-plane support excitation. Both elastic and elastic-plastic responses are recorded by varying the material properties of the columns of a distinguished floor. Parametric studies are performed by varying the secondary structure's fundamental frequency and damping. Experimental results are compared with those obtained by computational simulations. Experimental and numerical resu…

Materials scienceSmall-scale modelbusiness.industryMechanical EngineeringAerospace EngineeringStructural engineeringFundamental frequencyNon-structural elementElastic-plastic structureShear (geology)Mechanics of MaterialsExcited stateSupport excitationSolid mechanicsMaterial propertiesbusinessProtein secondary structureExcitationParametric statistics
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Volume growth, capacity estimates, p-parabolicity and sharp integrability properties of p-harmonic Green functions

2023

In a complete metric space equipped with a doubling measure supporting a $p$-Poincar\'e inequality, we prove sharp growth and integrability results for $p$-harmonic Green functions and their minimal $p$-weak upper gradients. We show that these properties are determined by the growth of the underlying measure near the singularity. Corresponding results are obtained also for more general $p$-harmonic functions with poles, as well as for singular solutions of elliptic differential equations in divergence form on weighted $\mathbf{R}^n$ and on manifolds. The proofs are based on a new general capacity estimate for annuli, which implies precise pointwise estimates for $p$-harmonic Green functions…

Mathematics - Analysis of PDEsGeneral MathematicsFOS: MathematicsPrimary: 31C45 Secondary: 30L99 31C12 31C15 31E05 35J08 35J92 46E36 49Q20AnalysisAnalysis of PDEs (math.AP)Journal d'Analyse Mathématique
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Multisummability for generalized power series

2022

We develop multisummability, in the positive real direction, for generalized power series with natural support, and we prove o-minimality of the expansion of the real field by all multisums of these series. This resulting structure expands both $\mathbb{R}_{\mathcal{G}}$ and the reduct of $\mathbb{R}_{\mathrm{an}^*}$ generated by all convergent generalized power series with natural support; in particular, its expansion by the exponential function defines both the Gamma function on $(0,\infty)$ and the Zeta function on $(1,\infty)$.

Mathematics - Classical Analysis and ODEsGeneral MathematicsClassical Analysis and ODEs (math.CA)FOS: Mathematics[MATH] Mathematics [math]Mathematics - LogicLogic (math.LO)Primary 40C10 03C64 26E10 Secondary 30D60
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Uniformization of metric surfaces using isothermal coordinates

2021

We establish a uniformization result for metric surfaces - metric spaces that are topological surfaces with locally finite Hausdorff 2-measure. Using the geometric definition of quasiconformality, we show that a metric surface that can be covered by quasiconformal images of Euclidean domains is quasiconformally equivalent to a Riemannian surface. To prove this, we construct suitable isothermal coordinates.

Mathematics - Complex VariablesMathematics::Complex VariablesPrimary 30L10 Secondary 30C65 28A75 51F99 52A38Metric Geometry (math.MG)ArticlesreciprocalityuniformizationisothermalMathematics - Metric GeometryQuasiconformalFOS: Mathematicssurfaceapproximate metric differentialComplex Variables (math.CV)
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Optimal transport maps on Alexandrov spaces revisited

2018

We give an alternative proof for the fact that in $n$-dimensional Alexandrov spaces with curvature bounded below there exists a unique optimal transport plan from any purely $(n-1)$-unrectifiable starting measure, and that this plan is induced by an optimal map.

Mathematics - Differential GeometryClass (set theory)Pure mathematicsGeneral MathematicsExistential quantificationPlan (drawing)Algebraic geometryoptimaalisuusCurvatureMeasure (mathematics)Primary 53C23. Secondary 49K30Mathematics - Analysis of PDEsMathematics - Metric GeometryFOS: Mathematicsmass transportationMathematics::Metric GeometryMathematicsAlexandrov-avaruudetMetric Geometry (math.MG)Number theoryDifferential Geometry (math.DG)Bounded functionMathematics::Differential GeometrymassasiirtoAlexandrov spacesAnalysis of PDEs (math.AP)
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Evolution by mean curvature flow of Lagrangian spherical surfaces in complex Euclidean plane

2016

We describe the evolution under the mean curvature flow of embedded Lagrangian spherical surfaces in the complex Euclidean plane $\mathbb{C}^2$. In particular, we answer the Question 4.7 addressed in [Ne10b] by A. Neves about finding out a condition on a starting Lagrangian torus in $\mathbb{C}^2$ such that the corresponding mean curvature flow becomes extinct at finite time and converges after rescaling to the Clifford torus.

Mathematics - Differential GeometryMean curvature flowApplied Mathematics010102 general mathematicsMathematical analysisTorusClifford torus01 natural sciencessymbols.namesakeDifferential Geometry (math.DG)0103 physical sciencesEuclidean geometrysymbolsFOS: MathematicsPrimary 53C44 53C40 Secondary 53D12010307 mathematical physics0101 mathematicsFinite timeMathematics::Symplectic GeometryAnalysisLagrangianMathematics
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A rigidity problem on the round sphere

2015

We consider a class of overdetermined problems in rotationally symmetric spaces, which reduce to the classical Serrin's overdetermined problem in the case of the Euclidean space. We prove some general integral identities for rotationally symmetric spaces which imply a rigidity result in the case of the round sphere.

Mathematics - Differential GeometryPure mathematicsEuclidean spaceApplied MathematicsGeneral Mathematics010102 general mathematicsMathematics::Analysis of PDEsComputer Science::Numerical Analysis01 natural sciencesOverdetermined systemrotationally symmetric spaceMathematics - Analysis of PDEsRigidity (electromagnetism)rigidityDifferential Geometry (math.DG)Settore MAT/05 - Analisi Matematica0103 physical sciencesRound sphereFOS: MathematicsPrimary 35R01 35N25 Secondary: 53C24 58J05Overdetermined PDE010307 mathematical physics0101 mathematicsAnalysis of PDEs (math.AP)Mathematics
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Manifolds with vectorial torsion

2015

Abstract The present note deals with the properties of metric connections ∇ with vectorial torsion V on semi-Riemannian manifolds ( M n , g ) . We show that the ∇-curvature is symmetric if and only if V ♭ is closed, and that V ⊥ then defines an ( n − 1 ) -dimensional integrable distribution on M n . If the vector field V is exact, we show that the V-curvature coincides up to global rescaling with the Riemannian curvature of a conformally equivalent metric. We prove that it is possible to construct connections with vectorial torsion on warped products of arbitrary dimension matching a given Riemannian or Lorentzian curvature—for example, a V-Ricci-flat connection with vectorial torsion in di…

Mathematics - Differential GeometrySpinor010102 general mathematicsSpinor bundlePrimary 53C25 Secondary 81T30CurvatureDirac operator01 natural sciencesManifoldsymbols.namesakeDifferential Geometry (math.DG)Computational Theory and MathematicsSpinor fieldKilling spinor0103 physical sciencesFOS: MathematicssymbolsMathematics::Differential Geometry010307 mathematical physicsGeometry and Topology0101 mathematicsAnalysisScalar curvatureMathematicsMathematical physicsDifferential Geometry and its Applications
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