Search results for "CORRELATED"

showing 10 items of 1174 documents

Towards nonlocal density functionals by explicit modelling of the exchange-correlation hole in inhomogeneous systems

2013

We put forward new approach for the development of a non-local density functional by a direct modeling of the shape of exchange-correlation (xc) hole in inhomogeneous systems. The functional is aimed at giving an accurate xc-energy and an accurate corresponding xc-potential even in difficult near-degeneracy situations such as molecular bond breaking. In particular we demand that: (1) the xc hole properly contains -1 electron, (2) the xc-potential has the asymptotic -1/r behavior outside finite systems and (3) the xc-potential has the correct step structure related to the derivative discontinuities of the xc-energy functional. None of the currently existing functionals satisfies all these re…

FOS: Physical sciences02 engineering and technologyElectronClassification of discontinuities01 natural sciencesDFTCondensed Matter - Strongly Correlated ElectronsAtomic orbitalQuantum mechanicsPhysics - Chemical Physics0103 physical sciencesPhysics - Atomic and Molecular ClustersSDG 7 - Affordable and Clean Energy010306 general physicsEnergy functionalChemical Physics (physics.chem-ph)PhysicsQuantum Physics/dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energyStrongly Correlated Electrons (cond-mat.str-el)ta114theoretical nanoscienceFunction (mathematics)021001 nanoscience & nanotechnologyAtomic and Molecular Physics and OpticsCondensed Matter - Other Condensed MatterDensity functional theorySum rule in quantum mechanicsLocal-density approximationAtomic and Molecular Clusters (physics.atm-clus)Quantum Physics (quant-ph)0210 nano-technologyOther Condensed Matter (cond-mat.other)Physical Review A
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Generation of energy selective excitations in quantum hall edge states

2011

We operate an on-demand source of single electrons in high perpendicular magnetic fields up to 30T, corresponding to a filling factor below 1/3. The device extracts and emits single charges at a tunable energy from and to a two-dimensional electron gas, brought into well defined integer and fractional quantum Hall (QH) states. It can therefore be used for sensitive electrical transport studies, e.g. of excitations and relaxation processes in QH edge states.

FOS: Physical sciences02 engineering and technologyElectronCorrelated Electron Systems / High Field Magnet Laboratory (HFML)Quantum Hall effect7. Clean energy01 natural sciences0103 physical sciencesMesoscale and Nanoscale Physics (cond-mat.mes-hall)Materials ChemistryPerpendicularElectrical and Electronic EngineeringWell-defined010306 general physicsPhysicsCondensed Matter - Mesoscale and Nanoscale PhysicsCondensed matter physicsFilling factorRelaxation (NMR)021001 nanoscience & nanotechnologyCondensed Matter PhysicsElectronic Optical and Magnetic MaterialsMagnetic fieldComputingMethodologies_DOCUMENTANDTEXTPROCESSING0210 nano-technologyFermi gas
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Orbital Rotations induced by Charges of Polarons and Defects in Doped Vanadates

2020

We explore the competiton of doped holes and defects that leads to the loss of orbital order in vanadate perovskites. In compounds such as La$_{1-{\sf x}}$Ca$_{\,\sf x}$VO$_3$ spin and orbital order result from super-exchange interactions described by an extended three-orbital degenerate Hubbard-Hund model for the vanadium $t_{2g}$ electrons. Long-range Coulomb potentials of charged Ca$^{2+}$ defects and $e$-$e$ interactions control the emergence of defect states inside the Mott gap. The quadrupolar components of the Coulomb fields of doped holes induce anisotropic orbital rotations of degenerate orbitals. These rotations modify the spin-orbital polaron clouds and compete with orbital rotat…

FOS: Physical sciences02 engineering and technologyElectronPolaron01 natural sciencesCondensed Matter - Strongly Correlated ElectronsAtomic orbital0103 physical sciencesCoulomb010306 general physicsSpin (physics)Condensed Matter - Statistical MechanicsPhysicsCondensed Matter - Materials ScienceStrongly Correlated Electrons (cond-mat.str-el)Statistical Mechanics (cond-mat.stat-mech)Condensed matter physicsMaterials Science (cond-mat.mtrl-sci)Order (ring theory)Disordered Systems and Neural Networks (cond-mat.dis-nn)Condensed Matter - Disordered Systems and Neural Networks021001 nanoscience & nanotechnologySuperexchangeCharge carrierCondensed Matter::Strongly Correlated ElectronsAstrophysics::Earth and Planetary Astrophysics0210 nano-technology
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Magnetic and electronic properties of double perovskites and estimation of their Curie temperatures byab initiocalculations

2008

First principles electronic structure calculations have been carried out on ordered double perovskites Sr_2B'B"O_6 (for B' = Cr or Fe and B" 4d and 5d transition metal elements) with increasing number of valence electrons at the B-sites, and on Ba_2MnReO_6 as well as Ba_2FeMoO_6. The Curie temperatures are estimated ab initio from the electronic structures obtained with the local spin-density functional approximation, full-potential generalized gradient approximation and/or the LDA+U method (U - Hubbard parameter). Frozen spin-spirals are used to model the excited states needed to evaluate the spherical approximation for the Curie temperatures. In cases, where the induced moments on the oxy…

FOS: Physical sciences02 engineering and technologyElectronic structure01 natural sciencesCondensed Matter::Materials ScienceCurie's lawAb initio quantum chemistry methods0103 physical sciences010306 general physicsPhysicsCondensed Matter - Materials ScienceCurie–Weiss lawCondensed matter physicsMaterials Science (cond-mat.mtrl-sci)021001 nanoscience & nanotechnologyCondensed Matter Physics3. Good healthElectronic Optical and Magnetic MaterialsCondensed Matter - Other Condensed MatterCurie temperatureCondensed Matter::Strongly Correlated ElectronsCurie constantLocal-density approximation0210 nano-technologyValence electronOther Condensed Matter (cond-mat.other)Physical Review B
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Quantum Phases and Spin Liquid Properties of 1T-TaS2

2021

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled fluid-like state of matter. Previous experiments on QSL candidate materials are usually interpreted in terms of a single QP, although theories indicate that many distinct QPs are closely competing in typical frustrated spin models. Here we report on combined temperature-dependent muon spin relaxation and specific heat measurements for the triangular-lattice QSL candidate material 1T-TaS2 that provide evidence for competing QPs. The measured properties are assig…

FOS: Physical sciences02 engineering and technologyQuantum phases01 natural sciencesCondensed Matter - Strongly Correlated ElectronsMesoscale and Nanoscale Physics (cond-mat.mes-hall)0103 physical sciencesTopological orderAtomic physics. Constitution and properties of matter010306 general physicsSpin (physics)MaterialsQuantumMaterials of engineering and construction. Mechanics of materialsPhysicsCondensed Matter - Materials ScienceStrongly Correlated Electrons (cond-mat.str-el)Condensed matter physicsCondensed Matter - Mesoscale and Nanoscale PhysicsQuàntums Teoria delsMaterials Science (cond-mat.mtrl-sci)Muon spin spectroscopy021001 nanoscience & nanotechnologyCondensed Matter PhysicsElectronic Optical and Magnetic MaterialsState of matterTA401-492Quantum spin liquid0210 nano-technologyCharge density waveQC170-197
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Engineering Topological Nodal Line Semimetals in Rashba Spin-Orbit Coupled Atomic Chains

2019

We study an atomic chain in the presence of modulated charge potential and modulated Rashba spin-orbit coupling (RSOC) of equal period. We show that for commensurate periodicities $\lambda=4 n$ with integer $n$, the three-dimensional synthetic space obtained by sliding the two phases of the charge potential and RSOC features a topological nodal line semimetal protected by an antiunitary particle-hole symmetry. The location and shape of the nodal lines strongly depend on the relative amplitude between the charge potential and RSOC.

FOS: Physical sciences02 engineering and technologySpace (mathematics)TopologyLambda01 natural sciencessemimetals0103 physical sciencesMesoscale and Nanoscale Physics (cond-mat.mes-hall)spin-orbit coupled systems010306 general physicsSpin (physics)Condensed Matter::Quantum GasesCouplingPhysicsCondensed Matter - Mesoscale and Nanoscale PhysicsAntiunitary operatorCharge (physics)topological phases021001 nanoscience & nanotechnologyCondensed Matter PhysicsSymmetry (physics)lcsh:QC1-999Electronic Optical and Magnetic MaterialsOrbit (dynamics)Computer Science::Programming LanguagesCondensed Matter::Strongly Correlated Electrons0210 nano-technologylcsh:PhysicsCondensed Matter
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Strongly interacting Fermi gases with density imbalance

2005

We consider density-imbalanced Fermi gases of atoms in the strongly interacting, i.e. unitarity, regime. The Bogoliubov-deGennes equations for a trapped superfluid are solved. They take into account the finite size of the system, as well as give rise to both phase separation and FFLO type oscillations in the order parameter. We show how radio-frequency spectroscopy reflects the phase separation, and can provide direct evidence of the FFLO-type oscillations via observing the nodes of the order parameter.

FOS: Physical sciencesGeneral Physics and Astronomy01 natural sciencesElectromagnetic radiation010305 fluids & plasmasSuperconductivity (cond-mat.supr-con)SuperfluidityCondensed Matter - Strongly Correlated ElectronsCondensed Matter::Superconductivity0103 physical sciences010306 general physicsSpectroscopyPhysicsCondensed Matter::Quantum GasesStrongly Correlated Electrons (cond-mat.str-el)UnitarityCondensed matter physicsCondensed Matter::OtherCondensed Matter - SuperconductivityFermionCondensed Matter - Other Condensed MatterQuantum electrodynamicsFermi gasOther Condensed Matter (cond-mat.other)Dimensionless quantityFermi Gamma-ray Space Telescope
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Time-dependent transport in Aharonov–Bohm interferometers

2010

A numerical approach is employed to explain transport characteristics in realistic, quantum Hall based Aharonov-Bohm interferometers. First, the spatial distribution of incompressible strips, and thus the current channels, are obtained applying a self-consistent Thomas-Fermi method to a realistic heterostructure under quantized Hall conditions. Second, the time-dependent Schr\"odinger equation is solved for electrons injected in the current channels. Distinctive Aharonov-Bohm oscillations are found as a function of the magnetic flux. The oscillation amplitude strongly depends on the mutual distance between the transport channels and on their width. At an optimal distance the amplitude and t…

FOS: Physical sciencesGeneral Physics and AstronomyFlux02 engineering and technologySTRIPSElectronQuantum Hall effect01 natural sciencesSchrödinger equationlaw.inventionCondensed Matter - Strongly Correlated Electronssymbols.namesakelawMesoscale and Nanoscale Physics (cond-mat.mes-hall)0103 physical sciences010306 general physicsPhysicsStrongly Correlated Electrons (cond-mat.str-el)Condensed Matter - Mesoscale and Nanoscale PhysicsCondensed Matter::Mesoscopic Systems and Quantum Hall Effect021001 nanoscience & nanotechnologyMagnetic fluxMagnetic fieldAmplitudeQuantum electrodynamicssymbols0210 nano-technologyNew Journal of Physics
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Frustrated quantum spin models with cold coulomb crystals

2011

We exploit the geometry of a zig-zag cold-ion crystal in a linear trap to propose the quantum simulation of a paradigmatic model of long-ranged magnetic frustration. Such a quantum simulation would clarify the complex features of a rich phase diagram that presents ferromagnetic, dimerized antiferromagnetic, paramagnetic, and floating phases, together with previously unnoticed features that are hard to assess by numerics. We analyze in detail its experimental feasibility, and provide supporting numerical evidence on the basis of realistic parameters in current ion-trap technology.

FOS: Physical sciencesGeneral Physics and AstronomyQuantum simulatorQuantum phases01 natural sciences010305 fluids & plasmasParamagnetismCondensed Matter - Strongly Correlated ElectronsQuantum mechanics0103 physical sciencesAtom010306 general physicsPhase diagramPhysicsQuantum PhysicsStrongly Correlated Electrons (cond-mat.str-el)Condensed matter physicsANNNI modelCondensed Matter - Other Condensed MatterFerromagnetismZigzagQuantum Gases (cond-mat.quant-gas)Condensed Matter::Strongly Correlated ElectronsQuantum Physics (quant-ph)Condensed Matter - Quantum GasesOther Condensed Matter (cond-mat.other)Physical Review Letters
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Defects, Disorder, and Strong Electron Correlations in Orbital Degenerate, Doped Mott Insulators.

2015

We elucidate the effects of defect disorder and $e$-$e$ interaction on the spectral density of the defect states emerging in the Mott-Hubbard gap of doped transition-metal oxides, such as Y$_{1-x}$Ca$_{x}$VO$_{3}$. A soft gap of kinetic origin develops in the defect band and survives defect disorder for $e$-$e$ interaction strengths comparable to the defect potential and hopping integral values above a doping dependent threshold, otherwise only a pseudogap persists. These two regimes naturally emerge in the statistical distribution of gaps among different defect realizations, which turns out to be of Weibull type. Its shape parameter $k$ determines the exponent of the power-law dependence o…

FOS: Physical sciencesGeneral Physics and Astronomylaw.inventionCondensed Matter - Strongly Correlated ElectronsPhysics and Astronomy (all)lawMesoscale and Nanoscale Physics (cond-mat.mes-hall)Spin (physics)Condensed Matter - Statistical MechanicsPhysicsCondensed Matter - Materials ScienceStrongly Correlated Electrons (cond-mat.str-el)Statistical Mechanics (cond-mat.stat-mech)Condensed Matter - Mesoscale and Nanoscale PhysicsCondensed matter physicsMott insulatorDopingDegenerate energy levelsMaterials Science (cond-mat.mtrl-sci)Disordered Systems and Neural Networks (cond-mat.dis-nn)Condensed Matter - Disordered Systems and Neural NetworksKröger–Vink notationDensity of statesCondensed Matter::Strongly Correlated ElectronsScanning tunneling microscopePseudogapPhysical review letters
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