Search results for "Carbohydrazide"

showing 10 items of 11 documents

Synthesis of pyrazole-4-carbohydrazide derivatives of pharmaceutical interest

2003

New 1-phenylor 1-methyl-5-benzamidopyrazole-4-carbohydrazide derivatives were prepared in 70–90% yields from 1-methylor 1-phenyl-6-phenylpyrazolo[3,4-d]1,3-oxazin-4(1H)-one derivatives and hydrazine hydrate. Small quantities of the isomeric 5-aminopyrazole-4-(Nbenzoyl)hydrazides were detected in some reaction mixtures, proving that intramolecular benzoyl migration can take place in the 5-benzamidopyrazole-4-carbohydrazide molecule. The direct formation of pyrazole-4-carbohydrazides from 5-benzamidopyrazole-4-carboxylic acid ethyl esters and hydrazine hydrate was unsuccessful.

lcsh:QD241-441chemistry.chemical_compoundlcsh:Organic chemistrychemistryIntramolecular forceOrganic ChemistryHydrazineMoleculePyrazoleCarbohydrazideEthyl esterHydrateMedicinal chemistryArkivoc
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ChemInform Abstract: Pyrazolo[3,4-d]pyrimidine Derivatives as COX-2 Selective Inhibitors: Synthesis and Molecular Modelling Studies.

2009

The pyrazolo[3,4-d]pyrimidine system shows a multitude of interesting pharmacological properties. Owing to the potential anti-inflammatory activity of 5-benzamido-pyrazolo[3,4-d]pyrimidin-4-one derivatives and considering the easy synthesis of this class of compounds, a set of new 5-benzamido-1H-pyrazolo[3,4-d]pyrimidin-4-ones has been prepared in 42-80% yields by reacting 5-aminopyrazole-4(N-benzoyl)carbohydrazide derivatives and the opportune triethylorthoesters. Compounds 8a, b, 10a-d, and 11a, b revealed a superior inhibitory profile against COX-2, when compared to that of reference standards NS398 and indomethacin. Molecular modelling studies confirmed the obtained biological results.

chemistry.chemical_compoundPyrimidineChemistryGeneral MedicineCarbohydrazideCombinatorial chemistryReference standardsChemInform
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Intramolecular 1,5-S...N σ-hole interaction in (E)-N′-(pyridin-4-ylmethylidene)thiophene-2-carbohydrazide

2020

The hydrazide-hydrazone forms inverse dimers via hydrogen bonding, but its conformation is defined by the presence of an intra­molecular chalcogen bond. Electrostatic forces dominate in the crystal packing and give rise to a layered supra­molecular structure.

crystal structurehirshfeld surfaceDouble bondImineStackingCrystal structureCarbohydrazide010402 general chemistryRing (chemistry)01 natural sciencesResearch Communicationsenergy frameworkslcsh:Chemistrychemistry.chemical_compoundchalcogen bondingGeneral Materials Sciencechemistry.chemical_classificationQuantitative Biology::Biomoleculesintermolecular interaction energies010405 organic chemistryHydrogen bondGeneral Chemistryinter­molecular inter­action energieshydrogen bondingCondensed Matter Physics4-pyridinecarboxaldehyde 2-thienyl hydrazone0104 chemical sciencesCrystallographylcsh:QD1-999chemistry4-pyridine­carboxaldehyde 2-thienyl hydrazoneMonoclinic crystal systemActa Crystallographica Section E Crystallographic Communications
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1,2,4-Triazoles. Improved synthesis of 5-substituted 4-amino-3-mer-cato-(4H)-1,2,4-triazoles and a facile route to 3,6-disubstituted 1,2,4-triazolo[3…

1997

The reaction of thiocarbohydrazide with carboxylic acids at the melting temperature allows an improved preparation of the S-substituted 4-amino-3-mercapto-1,2,4-triazole heterocycles. The crude 4-amino-5-mercapto-1,2,4-triazoles react easily with carboxylic acids or carboxylic acid chlorides to afford the 1,2,4-triazolo[3,4-fc][1,3,4]thiadiazole ring system.

chemistry.chemical_classificationThiocarbohydrazidechemistry.chemical_compoundThiadiazoleschemistryMelting temperatureCarboxylic acidOrganic ChemistryRing (chemistry)Medicinal chemistryJournal of Heterocyclic Chemistry
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Coordination versatility of 1,5-bis(salicylidene)carbohydrazide in Ni(II) complexes

2014

Abstract Versatile coordination behavior of a polydentate Schiff base ligand 1,5-bis(salicylidene)carbohydrazide (H3bsc) has been explored in Ni(II) complexes. [Ni(H3bsc)2](ClO4)2 (1)·H2O·3CH3CN is a bis chelate mononuclear complex of H3bsc in keto form, and [Ni4(H0.5bsc)2(O2CCMe3)3(CH3OH)4](2)·2H2O·2CH3OH is a tetranuclear complex of H3bsc with an unusual coordination. In 2, one phenolate group of the ligand coordinates in a monodentate way and the other coordinates in a μ2-bridging mode to the Ni(II) center. This unusual coordination mode of the ligand stabilizes the Ni(II) complex in a tetranuclear form where the carbonyl oxygen of the ligand exists in between keto and enol form of bond …

Schiff baseDenticityLigandStereochemistryCarbohydrazideEnolBond orderInorganic Chemistrychemistry.chemical_compoundCrystallographychemistryMaterials ChemistryAntiferromagnetismChelationPhysical and Theoretical ChemistryInorganic Chemistry Communications
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Pyrazolo[3,4‐d]pyrimidine Derivatives as COX‐2 Selective Inhibitors: Synthesis and Molecular Modelling Studies

2009

The pyrazolo[3,4-d]pyrimidine system shows a multitude of interesting pharmacological properties. Owing to the potential anti-inflammatory activity of 5-benzamido-pyrazolo[3,4-d]pyrimidin-4-one derivatives and considering the easy synthesis of this class of compounds, a set of new 5-benzamido-1H-pyrazolo[3,4-d]pyrimidin-4-ones has been prepared in 42-80% yields by reacting 5-aminopyrazole-4(N-benzoyl)carbohydrazide derivatives and the opportune triethylorthoesters. Compounds 8a, b, 10a-d, and 11a, b revealed a superior inhibitory profile against COX-2, when compared to that of reference standards NS398 and indomethacin. Molecular modelling studies confirmed the obtained biological results.

chemistry.chemical_compoundPyrimidineChemistryStereochemistryDocking (molecular)Drug DiscoveryPharmaceutical ScienceCarbohydrazideReference standardsArchiv der Pharmazie
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CCDC 1587259: Experimental Crystal Structure Determination

2019

Related Article: P. Sivajeyanthi, B. Edison, K. Balasubramani, G. Premkumar, T. Swu|2019|Acta Crystallogr.,Sect.E:Cryst.Commun.|75|804|doi:10.1107/S2056989019006492

Space GroupCrystallographyCrystal System(E)-N'-((3-hydroxy-4-methoxyphenyl)methylidene)pyridine-3-carbohydrazide monohydrateCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 799323: Experimental Crystal Structure Determination

2012

Related Article: L.Brelot, Xiao-yu Cao, J.Harrowfield, J.-M.Lehn, K.Rissanen, L.Russo|2011|CrystEngComm|13|2346|doi:10.1039/c0ce00814a

Space GroupCrystallography2581118212427-Octaoxatricyclo[26.3.1.0^1217^]dotriaconta-1(32)1214162830-hexaene-30-carbohydrazideCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 799324: Experimental Crystal Structure Determination

2012

Related Article: L.Brelot, Xiao-yu Cao, J.Harrowfield, J.-M.Lehn, K.Rissanen, L.Russo|2011|CrystEngComm|13|2346|doi:10.1039/c0ce00814a

Space GroupCrystallographyCrystal SystemCrystal Structure23568911121415-Decahydro-147101316-benzohexaoxacyclooctadecine-18-carbohydrazide chloroform solvateCell ParametersExperimental 3D Coordinates
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CCDC 1432912: Experimental Crystal Structure Determination

2015

Related Article: K. Karrouchi, M. Ansar, S. Radi, M. Saadi, L. El Ammari|2015|Acta Crystallogr.,Sect.E:Cryst.Commun.|71|o890|doi:10.1107/S2056989015020071

Space GroupCrystallographyCrystal SystemN'-(Diphenylmethylene)-5-methyl-1H-pyrazole-3-carbohydrazideCrystal StructureCell ParametersExperimental 3D Coordinates
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