Search results for "Diffusion"

showing 10 items of 1615 documents

Finite element simulation of diffusion into polycrystalline materials

2008

Diffusion in polycrystalline materials is investigated by means of numerical finite element simulations for constant source conditions. The grain boundaries are assumed to provide fast diffusion paths. Main emphasis is put on situations that typically occur for nanocrystals, viz. on situations in which (i) the diffusion length is significant compared with grain size, (ii) the influence of boundaries that are parallel to the surface become important in addition to the perpendicular ones. Furthermore, we treat the influence of blocking space charge layers sandwiching the core pathways and thus channeling grain boundary diffusion.

Materials scienceCondensed matter physicsGeneral ChemistryCondensed Matter PhysicsSpace chargeFinite element methodGrain sizeCrystallographyEffective diffusion coefficientGrain boundary diffusion coefficientGeneral Materials ScienceGrain boundaryCrystalliteDiffusion (business)Solid State Sciences
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RANDOM SEQUENTIAL ADSORPTION ON A LINEAR LATTICE: EFFECT OF DIFFUSIONAL RELAXATION

1992

In this paper, the authors offer phenomenological arguments, supported by numerical Monte Carlo data, suggesting that the asymptotic large-time behavior of the coverage in the 1D lattice deposition of k-mers with k {gt} 3, accompanied by k-mer diffusion, is governed by the same mean-field dynamics as the lattice chemical reaction kA {yields} inert. The latter reaction is considered to occur with partial probability. The coverage in the deposition process approaches full saturation for any nonzero diffusion rate, and the void fraction decreases according to the power-law t{sup {minus}1/(k{minus}1)}.

Materials scienceCondensed matter physicsMean field theoryDiffusionLattice (order)Monte Carlo methodThermodynamicsStatistical and Nonlinear PhysicsCrystal structureCondensed Matter PhysicsPorosityChemical reactionRandomnessModern Physics Letters B
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2 H-NMR-Stimulated Echo Study of Ultraslow Reorientational Motion in Viscous Glycerol near Its Glass Transition Temperature

1990

2H-NMR stimulated echo experiments have been performed in order to study the molecular basis of the ?-process in viscous glycerol near its glass transition temperature. Decay functions following modified Jeener-Broekaert pulse sequences were compared with predictions from different models for molecular reorientation. Rotational diffusion, rotational random jumps, rotational fixed-angle jumps and combinations of diffusive and jump motions have been tested. All data are fitted with a log-Gaussian distribution of correlation times. Thereby, small-but finite-angle reorientation processes turn out to dominate in the 10-3 s.. 100 s regime. Pure large-angle rotational jumps can be ruled out with h…

Materials scienceCondensed matter physicsRelaxation (NMR)Turn (geometry)JumpGeneral Physics and AstronomyRotational diffusionRotational temperatureGlass transitionMolecular physicsRotational correlation timePulse (physics)Europhysics Letters (EPL)
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Formation and emission properties of single InGaAs/GaAs quantum dots and pairs grown by droplet epitaxy

2010

Trabajo presentado a la 30th International Conference on the Physics of Semiconductors, celebrada en Seul (Korea) del 25 al 30 de Julio de 2010.

Materials scienceCondensed matter physicsmedia_common.quotation_subjectNucleationPhysics::OpticsCharge (physics)EpitaxyMolecular physicsAsymmetryQuantum dotElectric fieldArea densityDiffusion (business)media_common
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True and Apparent Oxygen Permeabilities of Contact Lenses

1992

We studied the passage of oxygen through some commercially available contact lenses. Oxygen diffusion coefficients were determined by the time-lag method and a 201T Redher permeometer was used to measure the oxygen permeability and transmissibility by the polarographic method. The measurements were carried out at room temperature with 0.09% sodium chloride physiologic solution. The following types of lenses were tested: (1) 12 lenses of cellulose acetate butyrate (CAB) of a mean thickness of 0.194 mm (observed Dk approximately 6.3 barrers) (1 barrier is equivalent to 10(-11) cm3 of O2 (STP).cm2/cm3.s.mm Hg). (2) 13 lenses of a cross-linked polyhydroxyethyl methacrylate (2-HEMA), manufacture…

Materials scienceContact LensesDiffusionSodiumAnalytical chemistrychemistry.chemical_elementMineralogyOxygenPermeabilityOxygenContact lensOphthalmologyOxygen permeabilitychemistryPermeability (electromagnetism)Water contentChemical compositionPolarographyOptometryOptometry and Vision Science
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Numerical analysis of the influence of ultrasonic vibration on crystallization processes

2011

The challenge in the future fabrication of semiconductor bulk crystals is the improvement of the crystal quality with a simultaneous increase of the yield. For that, a proper control of mass transfer within the fluid phase is required. Besides the damping of violent convective fluctuations, the thickness of the diffusion boundary layer, causing morphological instability, has to be decreased. The influence of ultrasound in molten Germanium was analyzed by numerical simulations. The simulations were provided by applying commercial software packages ANSYS ® and FLUENT ® . ANSYS ® was used to model the ultrasonic wave propagation in the whole growth system consisting of melt and crystal, crucib…

Materials scienceCrucibleGeneral ChemistryMechanicsCondensed Matter Physicslaw.inventionDiffusion layerlawFluid dynamicsFluentGeneral Materials ScienceUltrasonic sensorCrystallizationDisplacement (fluid)Melt flow indexCrystal Research and Technology
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A physical description of fractional-order Fourier diffusion

2014

In this paper the authors introduce a physical picture of anomalous heat transfer in rigid conductor. The analysis shows that a fractional-order Fourier transport is obtained by the analysis of the heat transport in a functionally graded conductor. The order of the fractional-type operator obtained is related to the grading of the physical properties of the conductor.

Materials scienceDifferential equationMathematics::Number TheoryOperator (physics)Mathematical analysisCondensed Matter::Mesoscopic Systems and Quantum Hall EffectConductorsymbols.namesakeFourier transformFourier numberThermal diffusion Fourier Equations Fractional-order calculus Temperature evolutionHeat transfersymbolsDiffusion (business)Settore ICAR/08 - Scienza Delle CostruzioniElectrical conductorICFDA'14 International Conference on Fractional Differentiation and Its Applications 2014
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Thermal stability under air of tungsten–titanium diffusion barrier layer between silica and platinum

2014

Abstract The present work investigated the thermal stability of tungsten–titanium diffusion barrier layers intercalated between SiO 2 substrate and platinum thin film. The resulting structures were annealed under air in the temperature range 400–600 °C for annealing times up to 100 h. Chemical and structural characterizations at different stages of the treatment evidenced several phenomena occurring during annealing under air, especially the complete oxidation of the adhesive layer, the diffusion of tungsten oxide through platinum film at particle boundaries as well as the sublimation process of tungsten oxide. The results of film surface chemistry and microstructure were correlated with di…

Materials scienceDiffusion barrierAnnealing (metallurgy)General Chemical EngineeringMetallurgychemistry.chemical_elementGeneral ChemistryTungstenchemistryChemical engineeringGeneral Materials ScienceSublimation (phase transition)Thermal stabilityThin filmPlatinumTitaniumCorrosion Science
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Comparative study of air and vacuum annealing atmosphere towards Pt/Ti–W/SiO2 stability

2013

Abstract The thermal stability of Pt/Ti–W/SiO2 system was studied after annealing under air or vacuum in the present work. A Ti–W adhesive film (30 at. % Ti) was deposited on a SiO2 substrate followed by a thicker Pt layer. Depositions were performed using DC magnetron sputtering. The whole as-deposited films are metallic with a columnar growth of platinum deposit which totally wets the substrate. Whatever the atmosphere is, annealing at 500 °C for 12 h does not change the platinum state but modifies the morphology of platinum particles, the lateral average size of which increasing from less than 10 nm up to ca. 75 nm. Besides, a noticeable diffusion of metallic tungsten through Pt film is …

Materials scienceDiffusion barrierAnnealing (metallurgy)Scanning electron microscopeMetals and AlloysAnalytical chemistrychemistry.chemical_elementSurfaces and InterfacesSputter depositionTungstenSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsX-ray photoelectron spectroscopychemistryMaterials ChemistryThermal stabilityComposite materialPlatinumThin Solid Films
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First-principles calculations of the initial incorporation of carbon into flat and stepped Pd surfaces

2010

We employ density-functional-theory calculations to examine carbon adsorption and diffusion in Pd bulk, and on Pd(111) and Pd(211) surfaces. Different possible subsurface and on-surface structures are explored and the most stable structures are analyzed. We calculate various diffusion paths: lateral diffusion on a surface, migration to a subsurface region, and within the first interlayer. Our calculations show in accordance with the earlier theoretical results that on Pd(111) carbon prefers to adsorb on octahedral interstitial sites. On Pd(211) the fourfold hollow site under the step is energetically the most favorable one and the second best sites are the octahedral sites. The calculations…

Materials scienceDiffusion barrierDiffusionchemistry.chemical_elementNanotechnologyCondensed Matter PhysicsElectronic Optical and Magnetic MaterialsAdsorptionchemistryOctahedronChemical physicsInterstitial defectLateral diffusionCarbon adsorptionCarbonPhysical Review B
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