Search results for "Dithiol"
showing 10 items of 143 documents
Aminobisphenolate supported tungsten disulphido and dithiolene complexes
2015
Dioxotungsten(vi) complexes with tetradentate amino bisphenolates were converted into the corresponding Cs-symmetric amino bisphenolate disulphido complexes by a reaction with either Lawesson's reagent or P2S5. Further reaction with diethyl acetylenedicarboxylate leads to the formation of diamagnetic tungsten(iv) dithiolene compounds. The syntheses, crystal structures, spectroscopic and electrochemical characterization of such disulphido and dithiolene complexes are presented.
The Interplay of Inverted Redox Potentials and Aromaticity in the Oxidized States of New π-Electron Donors: 9-(1,3-Dithiol-2-ylidene)fluorene and 9-(…
2006
Derivatives of 9-(1,3-dithiol-2-ylidene)fluorene (9) and 9-(1,3-dithiol-2-ylidene)thioxanthene (10) have been synthesised using Horner-Wadsworth-Emmons reactions of (1,3-dithiol-2-yl)phosphonate reagents with fluorenone and thioxanthen-9-one. X-ray crystallography, solution electrochemistry, optical spectroscopy, spectroelectrochemistry and simultaneous electrochemistry and electron paramagnetic resonance (SEEPR), combined with theoretical calculations performed at the B3P86/6-31G** level, elucidate the interplay of the electronic and structural properties in these molecules. These compounds are strong two-electron donors, and the oxidation potentials depend on the electronic structure of t…
Dithiol-Induced Oligomerization of Thiol-Protected Gold Nanoclusters
2018
Controlled synthesis of nanostructure oligomers requires detailed understanding of their wet chemistry and the forces driving the polymerization process. In this paper, we report the main factors affecting the reaction yields of a dithiol-induced synthesis of covalently bound nanocluster dimers and oligomers and present a detailed analysis of possible reaction mechanisms. We synthesize the nanocluster oligomers using monodisperse para-mercaptobenzoic acid (p-MBA)-protected gold nanoclusters with a nominal composition of Au∼250(p-MBA)n to minimize ensemble effects on size, shape, and surface structure. Ligand exchange was performed on the nanoclusters with five different dithiol linkers: 5,5…
CCDC 854063: Experimental Crystal Structure Determination
2012
Related Article: A.Molina-Ontoria, R.Garcia, A.Gouloumis, F.Giacalone, M.R.Torres, N.Martin|2012|Eur.J.Org.Chem.|2012|3581|doi:10.1002/ejoc.201200115
CCDC 1052254: Experimental Crystal Structure Determination
2015
Related Article: E. Salojärvi, A. Peuronen, R. Sillanpää, P. Damlin, H. Kivelä, A. Lehtonen|2015|Dalton Trans.|44|9409|doi:10.1039/C5DT00995B
CCDC 262735: Experimental Crystal Structure Determination
2005
Related Article: C.Faulmann, S.Dorbes, B.G.de Bonneval, G.Molnar, A.Bousseksou, C.J.Gomez-Garcia, E.Coronado, L.Valade|2005|Eur.J.Inorg.Chem.||3261|doi:10.1002/ejic.200500125
CCDC 262737: Experimental Crystal Structure Determination
2005
Related Article: C.Faulmann, S.Dorbes, B.G.de Bonneval, G.Molnar, A.Bousseksou, C.J.Gomez-Garcia, E.Coronado, L.Valade|2005|Eur.J.Inorg.Chem.||3261|doi:10.1002/ejic.200500125
CCDC 262738: Experimental Crystal Structure Determination
2005
Related Article: C.Faulmann, S.Dorbes, B.G.de Bonneval, G.Molnar, A.Bousseksou, C.J.Gomez-Garcia, E.Coronado, L.Valade|2005|Eur.J.Inorg.Chem.||3261|doi:10.1002/ejic.200500125
CCDC 262736: Experimental Crystal Structure Determination
2005
Related Article: C.Faulmann, S.Dorbes, B.G.de Bonneval, G.Molnar, A.Bousseksou, C.J.Gomez-Garcia, E.Coronado, L.Valade|2005|Eur.J.Inorg.Chem.||3261|doi:10.1002/ejic.200500125
CCDC 966355: Experimental Crystal Structure Determination
2015
Related Article: Alexander Jeremies, Ulrike Lehmann, Sina Gruschinski, Frederik Schleife, Michel Meyer, Vitaly Matulis, Oleg A. Ivashkevich, Marcel Handke, Karolin Stein, Berthold Kersting|2015|Inorg.Chem.|54|3937|doi:10.1021/acs.inorgchem.5b00123