Search results for "FEMTOSECOND"
showing 10 items of 238 documents
Ultrabroadband single-cycle terahertz pulses with peak fields of 300 kV cm-1 from a metallic spintronic emitter
2017
To explore the capabilities of metallic spintronic thin-film stacks as a source of intense and broadband terahertz electromagnetic fields, we excite a W/CoFeB/Pt trilayer on a large-area glass substrate (diameter of 7.5 cm) by a femtosecond laser pulse (energy 5.5 mJ, duration 40 fs, wavelength 800 nm). After focusing, the emitted terahertz pulse is measured to have a duration of 230 fs, a peak field of 300 kV cm$^{-1}$ and an energy of 5 nJ. In particular, the waveform exhibits a gapless spectrum extending from 1 to 10 THz at 10% of amplitude maximum, thereby facilitating nonlinear control over matter in this difficult-to-reach frequency range and on the sub-picosecond time scale.
Photoinduced interfacial electron injection in RuN3–TiO2 thin films: Resolving picosecond timescale injection from the triplet state of the protonate…
2008
Using femtosecond transient absorption spectroscopy we have studied light-induced electron injection from the sensitizer RuN3 and its partly deprotonated tetrabutylamonium salt to nano-structured TiO2 film. Previous studies have suggested significant differences in electron injection dynamics for these dyes and some results have indicated that aggregation of the sensitizer may lead to slow injection. By measuring transient absorption spectra and kinetics of RuN3 and RuN3-TBA in solution and attached to TiO2 film we show that the electron injection dynamics are very similar for the two forms of the dye and that aggregation has only moderate effects on the electron transfer dynamics. (c) 2008…
Mode cleaning in graphene oxide-doped polymeric whispering gallery mode microresonators
2020
The strategy to incorporate graphene oxide (GO) in a composite material offers significant opportunities to realize compact photonic devices, such as saturable absorbers and polarization selective devices. However, the processing of GO-based composites by direct laser writing, which would afford vast patterning and material flexibility in a single step process, has been little addressed. In this work, we investigated the mechanisms underlying a mode cleaning effect in polymeric whispering gallery mode microresonators containing GO, aiming at the development of on-chip integrable photonic devices. We fabricated the microresonators (cavity loaded Q-factor of 20 000 at 1550 nm) in a single ste…
Multiphoton process investigation in silica by UV femtosecond laser
2022
We investigated the interaction processes between high intensity femtosecond ultraviolet laser pulses and amorphous silica, leading to permanent refractive-index changes that are at the basis of advanced manufacturing for photonics devices. The experiment, carried out as a function of the laser power, improves our understanding on the strong-field ionization process by the monitoring of the 1.9 eV and 2.65 eV emissions, related to nonbridging oxygen hole centers and self-trapped exciton, respectively, induced in the exposed glass region. Our results clearly proved that the UV laser light band-to-band absorption is allowed in the multiphoton ionization limit, whose consecutive relaxation lea…
Ultrafast ionization and rotational dynamics of molecules in strong laser fields
2021
The investigation of ultrafast molecular dynamics is of great importance towards the understanding of a variety of natural phenomena in physical and chemical sciences. With the rapid development of femtosecond laser systems and precision detection technologies, it is possible now to visualize and steer the motion of molecules in matter as well as the ultrafast dynamics of electrons and nuclei in molecules on a microscopic timescale. When a molecule is exposed to a strong laser field, its electrons can be freed or excited, which often triggers a rapid dissociation of the system, in which the released electrons and nuclei exhibit a strong correlation, while the electronic motion on attosecond…
Emission of real phonons due to electron's self-dressing in a covalent crystal
2011
A slow monoelectronic excitation in a covalent crystal at the temperature T=0 is analyzed. The interaction with zero-point longitudinal acoustic phonons leads to the formation of a dressed electronic state at an energy level lower than that of the initial bare state. This aspect of the dressing process is described here by hypothesizing that the excess of energy is released with the emission of real phonons. Specifically, this paper considers the transition probability from the bare monoelectronic state to a dressed state of the electron accompanied by real phonons and a deformation field. The spectrum of the real phonons emitted during the electronic self-dressing is calculated by applying…
High spatiotemporal resolution in multifocal processing with femtosecond laser pulses.
2006
We report spatial and temporal dispersion compensation for fan-out of femtosecond pulses with a low-frequency diffraction grating by means of a hybrid diffractive-refractive lens triplet. In this way, we achieve a multifocal light structure with nearly diffraction-limited light spots even for 20 fs pulse duration. The spatial chromatic compensation, which drastically reduces the lateral walk-off of the various spectral components, also allows us to improve the available bandwidth at the dispersion-compensated diffraction orders. In fact, the temporal width of the output pulse is essentially limited by the group-delay dispersion term, which is shown to be small. The high spatiotemporal resol…
All-fibered high-quality 1.5–2 THz femtosecond pulse sources
2009
Generation of high-quality ultra-high repetition rate optical pulse trains around 1.55µm has become increasingly interesting for many scientific applications such as optical sampling, ultra-high capacity transmission systems, component testing or nonlinear phenomena studies. Unfortunately, the current bandwidth limitations of optoelectronic devices do not enable the direct generation of pulses with repetition rate higher than 80GHz and a temporal width below a few ps.
Diffractive optics for quasi-direct space-to-time pulse shaping.
2008
The strong chromatic behavior associated with a conventional diffractive lens is fully exploited to propose a novel optical device for pulse shaping in the femtosecond regime. This device consists of two optical elements: a spatially patterned circularly symmetric mask and a kinoform diffractive lens, which are facing each other. The system performs a mapping between the spatial position of the masking function expressed in the squared radial coordinate and the temporal position in the output waveform. This space-to-time conversion occurs at the chromatic focus of the diffractive lens, and makes it possible to tailor the output central wavelength along the axial location of the output point…
Fiber-based device for the detection of low-intensity fluctuations of ultrashort pulses
2012
International audience; We describe a fiber-based device that can significantly enhance the low intensity fluctuations of an ultrashort pulse train to detect them more easily than with usual direct detection systems. Taking advantage of the Raman intrapulse effect that progressively shifts the central frequency of a femtosecond pulse propagating in an anomalous dispersion fiber, a subsequent spectral filtering can efficiently increase the level of fluctuations by more than one order of magnitude. We show that attention has to be paid to maintain the shape of the statistical distribution unaffected by the nonlinear process.