Search results for "Kerr effect"
showing 10 items of 107 documents
Molecular structure and electric properties of N -methyl- N -nitroaniline and its derivatives
2001
A comparative study of the molecular structure of N-methyl-N-nitroaniline and its derivatives is carried out employing the Kerr effect and dipole moments methods in combination with the crystallographic analysis. The obtained experimental structural data agree with the quantum-chemical calculations by the B3LYP/6-31G p and MP2/3-21G p methods. The measurement and calculation results are used to draw conclusions about the mutual interaction and role of various substituents to the Nmethyl-N-nitroaniline molecule. q 2001 Elsevier Science B.V. All rights reserved.
Study of Structure–Third-Order Susceptibility Relation of Indandione Derivatives
2016
By using the Z-scan method we studied the third-order nonlinear optical parameters of several aminobenziliden-1,3-indandione (ABI) derivatives that have previously been shown to own second-order nonlinear optical properties. Measurements were carried out using two 1064 nm Nd:YAG lasers with picosecond (ps) and nanosecond (ns) pulse widths, respectively. When ns laser was employed in the Z-scan setup, a strong thermal lensing took place resulting in severe overestimation of optical Kerr coefficients. Due to this reason the ps laser was employed to evaluate correct magnitude of Kerr effect. For investigated organic molecules, experimental results show that two-photon absorption at 1064 nm is …
Higher-order Kerr terms allow ionization-free filamentation in gases.
2010
We show that higher-order nonlinear indices ($n_4$, $n_6$, $n_8$, $n_{10}$) provide the main defocusing contribution to self-channeling of ultrashort laser pulses in air and Argon at 800 nm, in contrast with the previously accepted mechanism of filamentation where plasma was considered as the dominant defocusing process. Their consideration allows to reproduce experimentally observed intensities and plasma densities in self-guided filaments.
Field-free two-direction alignment alternation of linear molecules by elliptic laser pulses
2005
We show that a linear molecule subjected to a short specific elliptically polarized laser field yields postpulse revivals exhibiting alignment alternatively located along the orthogonal axis and the major axis of the ellipse. The effect is experimentally demonstrated by measuring the optical Kerr effect along two different axes. The conditions ensuring an optimal field-free alternation of high alignments along both directions are derived.
Electrical control of 2D magnetism in bilayer CrI3
2018
The challenge of controlling magnetism using electric fields raises fundamental questions and addresses technological needs such as low-dissipation magnetic memory. The recently reported two-dimensional (2D) magnets provide a new system for studying this problem owing to their unique magnetic properties. For instance, bilayer chromium triiodide (CrI3) behaves as a layered antiferromagnet with a magnetic field-driven metamagnetic transition. Here, we demonstrate electrostatic gate control of magnetism in CrI3 bilayers, probed by magneto-optical Kerr effect (MOKE) microscopy. At fixed magnetic fields near the metamagnetic transition, we realize voltage-controlled switching between antiferroma…
Integrated Optical Technique for Detection of Electro-Optical Non-Linearities in Thin Films
1976
A simple method for detection of electro-optical non-linearities in thin films is presented. The method involves an easily fabricated structure and a little practice in integrated optical techniques. It is also possible to detect small induced variations of refractive index, using lower voltage with respect to those applied in a conventional Kerr cell. We have sucessfully tested our method using two different polymer materials as thin films. In both of these we have observed an induced ?n ? 3 10?5 with an electric field of 60 V/?, with a response time round about 300 nsec. The experimental values of induced ?n versus electric field fit very well a parabola, proving the quadratic behavior of…
Measurement of high order Kerr refractive index of major air components
2009
International audience; We measure the instantaneous electronic nonlinear refractive index of N2 , O2 , and Ar at room temperature for a 90 fs and 800 nm laser pulse. Measurements are calibrated by post-pulse molecular alignment through a polarization technique. At low intensity, quadratic coefficients n2 are determined. At higher intensities, a strong negative contribution with a higher nonlinearity appears, which leads to an overall negative nonlinear Kerr refractive index in air above 26 TW/cm2 .
Measurement of laser-induced alignment of molecules by cross defocusing
2005
0146-9592; The field-free alignment of CO2 produced in response to the excitation of a molecule by a high-intensity femtosecond pump pulse is measured with a simple coronography-like technique. The technique is based on the defocusing of a time-delayed probe pulse produced by the spatial distribution of aligned molecules. In the intensity regime explored here, the technique is shown to give valuable information about dynamic alignment. With the help of simulations, the degree of alignment is extracted from the data. (C) 2005 Optical Society of America.
Theory of spontaneous polarization and birefringence in the tetragonal phase of KNbO3
1995
Abstract The microscopic mechanism of optical anisotropy in the tetragonal phase of KNbO3 is discussed taking account of the dipole-dipole effect due to the ionic and electronic polarizations of the crystal and the spontaneous Kerr effect. The last effect is a cause of the strong local field acting on the constituent ions. For the spontaneous polarization we use only the first effect. It is found that the birefringence and the spontaneous polarization are in good agreement with the experimental data.
Incoherent solitons and condensation processes
2006
International audience; We study the nonlinear interaction of partially incoherent nonlinear optical waves. We show that, in spite of the incoherence of the waves, coherent phase effects may play a relevant role during the propagation, in contrast with the usual wave turbulence description of the interaction. These nonlinear phase effects may lead the system to unexpected processes of self-organization, such as condensation, or incoherent soliton generation in instantaneous response nonlinear media. Such self-organization processes may be characterized by a reduction of the non-equilibrium entropy, which violates the Boltzmann's H-theorem of entropy growth inherent to the wave turbulence th…