Search results for "Linear"
showing 10 items of 7165 documents
FIRST-PRINCIPLES LCAO CALCULATIONS ON 5D TRANSITION METAL OXIDES: ELECTRONIC AND PHONON PROPERTIES
2009
ABSTRACT First-principles quantum chemistry calculations within the periodic linear combination of atomic orbitals (LCAO) formalism have been used to probe electronic and phonon properties of crystalline 5d transition metal oxides ReO3, ZnWO4 and CaWO4. The obtained equilibrium crystal structure is in good agreement with known crystallographic data. Rhenium trioxide is correctly predicted to be a metal, whereas both tungstates—a wide gap insulating compounds. The phonon frequencies, calculated by the frozen phonon method, agree rather well with those obtained by infrared and Raman spectroscopies.
RADICAL DISTRIBUTIONS IN AMMONIUM TARTRATE SINGLE CRYSTALS EXPOSED TO PHOTON AND NEUTRON BEAMS
2014
The radiation therapy carried out by means of heavy charged particles (such as carbon ions) and neutrons is rapidly becoming widespread worldwide. The success of these radiation therapies relies on the high density of energy released by these particles or by secondary particles produced after primary interaction with matter. The biological damages produced by ionising radiations in tissues and cells depend more properly on the energy released per unit pathlength, which is the linear energy transfer and which determines the radiation quality. To improve the therapy effectiveness, it is necessary to grasp the mechanisms of free radical production and distribution after irradiation with these …
Enhanced photorefractive properties of Bi-doped Sn2P2S6
2008
International audience; Enhanced photorefractive properties of tin hypothiodiphosphate (Sn2P2S6) crystals as a result of Bi doping are presented. These new crystals were obtained by the vapor-transport technique using stoichiometric Sn2P2S6 composition with an additional amount of Bi up to 0.5 mol. % in the initial compound. The bandgap edges of the obtained crystals are located at ~750 nm and shift toward the red wavelengths with increasing Bi concentration. Sn2P2S6:Bi crystals are found to exhibit larger two-beam coupling gain coefficients (up to 17 cm−1 at a wavelength of 854 nm) as compared to (i) pure Sn2P2S6 (2.5 cm−1 at 854 nm), (ii) Sn2P2S6 crystals modified by the growth conditions…
First-principles LCAO study of the low and room temperature phases of CdPS$_3$
2020
A.K. is grateful to the Latvian Council of Science project no. lzp-2018/2-0353 for financial support. Institute of Solid State Physics, University of Latvia as the Center of Excellence has received funding from the European Union’s Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement No. 739508, project CAMART2.
Pre-determining the location of electromigrated gaps by nonlinear optical imaging
2014
In this paper we describe a nonlinear imaging method employed to spatially map the occurrence of constrictions occurring on an electrically-stressed gold nanowire. The approach consists at measuring the influence of a tightly focused ultrafast pulsed laser on the electronic transport in the nanowire. We found that structural defects distributed along the nanowire are efficient nonlinear optical sources of radiation and that the differential conductance is significantly decreased when the laser is incident on such electrically-induced morphological changes. This imaging technique is applied to pre-determined the location of the electrical failure before it occurs.
Determination of temperature by stimulated raman scattering of molecular nitrogen, oxygen, and carbon dioxide
1993
We have determined the temperature from SRS spectra of N2-N2, N2-CO2, O2-O2, and CO2-CO2 recorded in wide pressure and temperature ranges. The fitting procedure takes simultaneously into account the Dicke effect and motional narrowing. We have quantified the accuracy of the MEG and ECS-P models for rotational relaxation. The temperature extracted from each model is compared with thermocouple measurements. The influence of vibrational broadening and shifting is discussed in detail.
Flat supercontinuum generation pumped by amplified noise-like pulses from a figure-eight erbium-doped fiber laser
2017
The conditions to obtain noise-like pulses (NLPs) from a figure-eight fiber laser (F8L) and their application for supercontinuum (SC) generation in the anomalous dispersion regime are reported. The F8L is designed to remove the undesired low-intensity background radiation from pulse emission, generating NLPs with a 3 dB spectral bandwidth of 17.43 nm at the fundamental repetition frequency of 0.8 MHz. After amplification, NLPs reach a maximum average power of 9.2 mW and 123.32 nm spectral bandwidth. By controlling the amplifier pump power, flat SC generation is demonstrated through both a 800 m long spool of SMF-28 fiber and a piece of 5 m long highly nonlinear optical fiber. The results de…
Continuous-wave backward frequency doubling in periodically poled lithium niobate
2010
We report on backward second-harmonic-generation in bulk periodically poled congruent lithium niobate with a 3.2 microns period. A tunable continuous-wave Ti:sapphire laser allowed us exciting two resonant quasi-phase-matching orders in the backward configuration. The resonances were also resolved by temperature tuning and interpolated with standard theory to extract relevant information on the sample.
Theory of parabolic pulse propagation in nonlinear dispersion decreasing optical fiber amplifiers
2008
Optical fibers ; Nonlinear optics ; Optical fiber amplifiers ; Optical amplifier ; Optical solitons ; Electromagnetic wave propagation ; Pulse propagation ;; International audience; We show that pulse spectral broadening in normally dispersive nonlinear fiber amplifiers may be enhanced by introducing a suitable dispersion tapering. We obtain an analytical dispersion profile that permits one to reduce pulse propagation in a varying dispersion fiber to the case of an equivalent fiber with constant parameters.
Some considerations on the transmissivity of trirefringent metamaterials
2016
Nonlocal effects in metal–dielectric (MD) periodic nanostructures may typically be observed when the plasmonic particles and gaps are on the scale of a few tens of nanometers, enabling under certain conditions (succinctly for epsilon near zero) a collimated beam to split into three refracted signals. We developed a method for precisely evaluating the categorized transmissivity in an air/trirefringent metamaterial interface, which uses a fast one-dimensional Fourier transform and finite element solvers of Maxwell’s equations. In periodic arrays of MD nanofilms, it is proved a tunable transmissivity switch of the multirefracted beams under varying angle of incidence and wavelength, while keep…