Search results for "Phosphoramidite"

showing 3 items of 3 documents

A modified guanosine phosphoramidite for click functionalization of RNA on the sugar edge

2012

A propargyl containing guanosine phosphoramidite was synthesized and incorporated into siRNA, enabling click-ligation with an azido fluorophore onto the nucleobase sugar edge. Duplex stability was not affected by labeling at this new site, which allowed deconvolution of the effects of label, structure and attachment site on RNAi activity.

PhosphoramiditeFluorophoreGuanosineMolecular StructureCarbohydratesMetals and AlloysGuanosineRNAGeneral ChemistryCombinatorial chemistryCatalysisSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsNucleobasechemistry.chemical_compoundOrganophosphorus CompoundschemistryDuplex (building)PropargylMaterials ChemistryCeramics and CompositesRNASurface modificationClick ChemistryRNA Small InterferingChemical Communications
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Pathogen-Mimicking MnO Nanoparticles for Selective Activation of the TLR9 Pathway and Imaging of Cancer Cells

2009

Here, design of the first pathogen-mimicking metal oxide nanoparticles with the ability to enter cancer cells and to selectively target and activate the TLR9 pathway, and with optical and MR imaging capabilities, is reported. The immobilization of ssDNA (CpG ODN 2006) on MnO nanoparticles is performed via the phosphoramidite route using a multifunctional polymer. The multifunctional polymer used for the nanoparticle surface modification not only affords a protective organic biocompatible shell but also provides an efficient and convenient means for loading immunostimulatory oligonucleotides. Since fluorescent molecules are amenable to photodetection, a chromophore (Rhodamine) is introduced …

PhosphoramiditeMaterials scienceOligonucleotideNanoparticleNanotechnology02 engineering and technology010402 general chemistry021001 nanoscience & nanotechnologyCondensed Matter Physics01 natural sciences0104 chemical sciencesElectronic Optical and Magnetic MaterialsBiomaterialsRhodaminechemistry.chemical_compoundchemistryCancer cellElectrochemistryBiophysicsSurface modification0210 nano-technologyDrug carrierBiosensorAdvanced Functional Materials
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Straightforward synthesis of bioconjugatable azo dyes. Part 1: Black Hole Quencher-​1 (BHQ-​1) scaffold

2014

Abstract Azo dyes are currently used to quench the fluorescence of energy donors in bioassays through Forster resonance energy transfer (FRET) phenomenon. Common examples of such dark quenchers are DABCYL and the three members of Black Hole Quencher® (BHQ) family. Yet, only carboxylic acid and phosphoramidite derivatives of such azo dyes are presently commercially available. This Letter presents a straightforward synthesis method to novel bioconjugatable quenchers derived from BHQ-1 scaffold and equipped with a reactive group being either azido, terminal alkyne, or maleimide. The potential utility of the ‘clickable’ azido and thiol-reactive derivatives was notably demonstrated through the p…

chemistry.chemical_classificationPhosphoramiditeBioconjugation[CHIM.ORGA]Chemical Sciences/Organic chemistryCarboxylic acidOrganic ChemistryAlkyneBlack Hole Quencher-1[CHIM.CATA]Chemical Sciences/Catalysis[CHIM.THER]Chemical Sciences/Medicinal ChemistryPhotochemistry7. Clean energyBiochemistryFluorescence[CHIM.THEO]Chemical Sciences/Theoretical and/or physical chemistrychemistry.chemical_compoundFörster resonance energy transferchemistry[CHIM.ANAL]Chemical Sciences/Analytical chemistryDrug DiscoveryMaleimideComputingMilieux_MISCELLANEOUS[CHIM.CHEM]Chemical Sciences/Cheminformatics
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