Search results for "Spins"

2019

Abstract In high sensitivity inductive electron spin resonance spectroscopy, superconducting microwave resonators with large quality factors are employed. While they enhance the sensitivity, they also distort considerably the shape of the applied rectangular microwave control pulses, which limits the degree of control over the spin ensemble. Here, we employ shaped microwave pulses compensating the signal distortion to drive the spins faster than the resonator bandwidth. This translates into a shorter echo, with enhanced signal-to-noise ratio. The shaped pulses are also useful to minimize the dead-time of our spectrometer, which allows to reduce the wait time between successive drive pulses.

Dynamics of a Ferromagnetic Particle Levitated Over a Superconductor

2018

Under conditions where the angular momentum of a ferromagnetic particle is dominated by intrinsic spin, applied torque is predicted to cause gyroscopic precession of the particle. If the particle is sufficiently isolated from the environment, a measurement of spin precession can potentially yield sensitivity to torque beyond the standard quantum limit. Levitation of a micron-scale ferromagnetic particle above a superconductor is a possible method of near frictionless suspension enabling observation of ferromagnetic particle precession and ultrasensitive torque measurements. We experimentally investigate the dynamics of a micron-scale ferromagnetic particle levitated above a superconducting …

Static and dynamic interaction betweenπanddelectrons in organic superconductorβ″-(BEDT-TTF)4[(H3O)Fe(C2O4)3]·C6H5Brstudied byC13NMR spectroscopy

2016

We present the results of $^{13}\mathrm{C}$ NMR experiments in an organic superconductor with localized Fe spins ${\ensuremath{\beta}}^{\ensuremath{''}}\ensuremath{-}{(\text{BEDT-}\mathrm{TTF})}_{4}[({\mathrm{H}}_{3}\mathrm{O})\mathrm{Fe}{({\mathrm{C}}_{2}{\mathrm{O}}_{4})}_{3}]\ifmmode\cdot\else\textperiodcentered\fi{}{\mathrm{C}}_{6}{\mathrm{H}}_{5}\mathrm{Br}$. We reveal the antiferromagnetic coupling between Fe $d$ spins and $\ensuremath{\pi}$ spins, which creates an exchange field antiparallel to the external field direction at the $\ensuremath{\pi}$ electrons. In addition to the static effects of Fe spins, we show from the nuclear spin-lattice relaxation rate measurement that the magn…

Self-Consistent Tilted-Axis-Cranking Study of Triaxial Strongly Deformed Bands inEr158at Ultrahigh Spin

2012

Stimulated by recent experimental discoveries, triaxial strongly deformed (TSD) states in $^{158}\mathrm{Er}$ at ultrahigh spins have been studied by means of the Skyrme-Hartree-Fock model and the tilted-axis-cranking method. Restricting the rotational axis to one of the principal axes---as done in previous cranking calculations---two well-defined TSD minima in the total Routhian surface are found for a given configuration: one with positive and another with negative triaxial deformation $\ensuremath{\gamma}$. By allowing the rotational axis to change direction, the higher-energy minimum is shown to be a saddle point. This resolves the long-standing question of the physical interpretation o…

Ultrafast amplification and non-linear magneto-elastic coupling of coherent magnon modes in an antiferromagnet

2021

We investigate the role of domain walls in the ultrafast magnon dynamics of an antiferromagnetic NiO single crystal in a pump-probe experiment with variable pump photon energy. Analysing the amplitude of the energy-dependent photo-induced ultrafast spin dynamics, we detect a yet unreported coupling between the material's characteristic THz- and a GHz-magnon modes. We explain this unexpected coupling between two orthogonal eigenstates of the corresponding Hamiltonian by modelling the magneto-elastic interaction between spins in different domains. We find that such interaction, in the non-linear regime, couples the two different magnon modes via the domain walls and it can be optically exploi…

Competition of Direct and Indirect Sources of Thermal Entanglement in a spin star network

2017

A spin star system consisting of three peripheral two-state systems and a central one is considered, with the peripheral spins assumed to interact with each other, as well as with the central one. It is shown that such two couplings, each one being a thermal entanglement source, can significantly compete in the formation of quantum correlations in the thermal state, to the point that they can destroy any thermal entanglement of the peripheral spins.

Finite Size Scaling Tools for the Study of Interfacial Phenomena and Wetting

2019

In this chapter, we use the word “interface” in the sense of a boundary between coexisting bulk phases (in thermal equilibrium). An example is the interface between liquid (e.g. water) and gas phases (water vapor) but also interfaces between fluid and solid phases (e.g. water and ice) can be considered, as well as interfaces between coexisting solid phases. The generic example are “domain walls” in magnets, separating domains with opposite orientation of the magnetization, a case that can already be studied in the framework of the simple Ising model (Chaps. 2 and 3) where one has spins on the sites of a rigid perfect lattice pointing up or down.

Electric Field Generation and Control of Bipartite Quantum Entanglement between Electronic Spins in Mixed Valence Polyoxovanadate [GeV14O40]8–

2017

As part of the search for systems in which control of quantum entanglement can be achieved, here we consider the paramagnetic mixed valence polyoxometalate K2Na6[GeV14O40]·10H2O in which two electrons are delocalized over the 14 vanadium ions. Applying a homogeneous electric field can induce an antiferromagnetic coupling between the two delocalized electronic spins that behave independently in the absence of the field. On the basis of the proposed theoretical model, we show that the external field can be used to generate controllable quantum entanglement between the two electronic spins traveling over a vanadium network of mixed valence polyoxoanion [GeV14O40]8–. Within a simplified two-lev…

MVPACK: a package to calculate energy levels and magnetic properties of high nuclearity mixed valence clusters.

2010

We present a FORTRAN code based on a new powerful and efficient computational approach to solve the double exchange problem for high-nuclearity MV clusters containing arbitrary number of localized spins and itinerant electrons. We also report some examples in order to show the possibilities of the program.

Modelling electric field control of the spin state in the mixed-valence polyoxometalate [GeV14O40]8−

2013

International audience; : The two-electron reduced mixed-valence polyoxometalate [GeV14O40](8-) presents an unusual paramagnetic behaviour as a consequence of the partial trapping of these electrons. The effect of applying an electric field is that of inducing antiferromagnetic coupling between the two delocalized electronic spins.