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showing 10 items of 2224 documents

ChemInform Abstract: Photoelectrochemical Characterization of Thin Anodic Oxide Films on Zirconium Metal.

2010

Abstract The effect of metal surface preparation on the properties of thin oxide films grown on zirconium in different electrolytes was investigated by photocurrent spectroscopy. Both passive layers grown by free corrosion of the samples in a solution and thin oxides grown anodically at a constant rate were investigated. The photoelectrochemical results give a complex picture of the interface, being influenced by the metal surface preparation, the solution pH and the electrode potential. A duplex structure of the films has been suggested on the basis of the photocurrent spectra, with an external hydrous layer (amorphous or strongly defective) having an optical gap ( E g 2 ~ 3 eV) lower resp…

PhotocurrentZirconiumchemistry.chemical_compoundchemistryInorganic chemistryOxidechemistry.chemical_elementGeneral MedicineElectrolyteThin filmCorrosionElectrode potentialAmorphous solidChemInform
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Photocurrent enhancement in thin a-Si:H solar cells via plasmonic light trapping

2014

Photocurrent enhancement in thin a-Si:H solar cells due to the plasmonic light trapping is investigated, and correlated with the morphology and the optical properties of the selfassembled silver nanoparticles incorporated in the cells' back reflector. © 2014 OSA.

Photocurrentanimal structuresMaterials sciencegenetic structuresbusiness.industryScanning electron microscopeTrappingSolar energySettore ING-INF/01 - ElettronicaAtomic and Molecular Physics and OpticsSettore FIS/03 - Fisica Della Materiaeye diseasesSilver nanoparticleSolar cell efficiencyOptoelectronicssense organsPlasmonic solar cellbusinessInstrumentationPlasmon
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Recent advances in photocurrent spectroscopy of passive films

2003

Abstract The quantitative application of photocurrent spectroscopy (PCS) for the in-situ determination of the composition of passive films and corrosion layers is reviewed in the light of recent theoretical advances, that have allowed to relate the measured optical gaps to the Pauling electronegativities of the film components. The correlations derived are tested versus recent experimental results regarding mixed oxides, anhydrous passive films on metallic alloys and hydroxide layers. The effect of the eventual long-range disorder into the passive film on the optical band gap values is also discussed. New experimental evidence reported for mixed d,d-metal oxides and passive films on sp,d-me…

Photocurrentbusiness.industryBand gapGeneral Chemical EngineeringMineralogyCorrosionMetalElectronegativitychemistry.chemical_compoundchemistryvisual_artElectrochemistryAnhydrousvisual_art.visual_art_mediumOptoelectronicsHydroxidebusinessSpectroscopyElectrochimica Acta
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Amorphous semiconductor-electrolyte junction

1987

Abstract The photoelectrochemical behaviour of amorphous anodic films on niobium (a-Nb 2 O 5 ) grown in a wide range of thicknesses (20 ⩽ d ox ⩽ 25 nm) is presented. The influence of the wavelength, light intensity and film thickness on the photocharacteristics of the a-Nb 2 O 5 /electrolyte junction is investigated. Expressions for the photocurrent curves under steady-state conditions are derived by assuming a variable efficiency of photocarrier generation and different distributions of the electrical potential inside the amorphous films. The influence of the light intensity on the photocharacteristics and the existence of a sub-band-gap photoresponse are explained by assuming a finite den…

Photocurrentbusiness.industryOxideNiobiumchemistry.chemical_elementElectrolyteAmorphous solidLight intensitychemistry.chemical_compoundWavelengthOpticschemistryDensity of statesOptoelectronicsbusinessJournal of Electroanalytical Chemistry and Interfacial Electrochemistry
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PV and magnetic field effects in poly(3-hexylthiophene)-fullerene cells doped with phthalocyanine soluble derivative

2007

An attempt was made to widen the photosensitivity spectral range of poly(3-hexylthiophene)-fullerene blend by adding an extra electron donor — a newly synthesized soluble phthalocyanine derivative (SnClPc) having the electron absorption band at 708 nm. As the electron acceptor, home-synthesised di(ethoxycarbonyl) methano-fullerene carboxylate (C 61 (CO 2 Et) 2 ) was used, and as the hole transporter — the regioregular poly 3-hexylthiophene (P3HT). The sandwich-type samples were prepared on an ITO glass substrate by coating it with a 30–50 nm thick PEDOT:PSS layer followed by a ~100 nm thick P3HT:C 61 (CO 2 Et) 2 :SnClPc blend. For the top electrodes In or Au were used. Spectral dependences …

Photocurrentchemistry.chemical_classificationChemistryDopingAnalytical chemistryElectron acceptorCondensed Matter PhysicsElectronic Optical and Magnetic Materialschemistry.chemical_compoundPhotosensitivityPEDOT:PSSAbsorption bandPhthalocyanineOrganic chemistryQuantum efficiencyInstrumentationThe European Physical Journal Applied Physics
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Electro- and photo-electrooxidation of 2,4,5-trichlorophenoxiacetic acid (2,4,5-T) in aqueous media with PbO2, Sb-doped SnO2, BDD and TiO2-NTs anodes…

2020

Abstract In this work, the 2,4,5-T degradation in aqueous media was studied by electro- (EC) and photoelectrochemical (PEC) oxidation methods, which are two of the most important advanced oxidation processes (AOPs) for wastewater treatment. Both EC and PEC experiments were carried out in a single compartment cell under galvanostatic conditions (30 mA cm−2) at 298 K by using 0.05 M Na2SO4 + 200 ppm 2,4,5-T at pH 3 and pH 9, as model solutions. EC oxidation was performed using Sb-doped SnO2, PbO2 and boron doped diamond (BDD) as anodic materials. Besides these anodes, TiO2 in a nanotubular structure (TiO2 NTs) with or without PbO2 dispersed nanoparticles (TiO2::PbO2) were also used for PEC ox…

Photocurrentchemistry.chemical_classificationElectrolysisAqueous solutionmedicine.diagnostic_testChemistryGeneral Chemical EngineeringCarboxylic acidInorganic chemistry02 engineering and technology010402 general chemistry021001 nanoscience & nanotechnology01 natural sciences0104 chemical sciencesAnalytical Chemistrylaw.inventionReaction rate constantlawSpectrophotometryElectrodeElectrochemistrymedicine0210 nano-technologyVoltammetryJournal of Electroanalytical Chemistry
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Synthesis and photovoltaic performance of asymmetric di-anchoring organic dyes

2015

Abstract Two novel metal-free organic dyes bearing two asymmetric double donor–acceptor segments were synthesized. Their physical, optical, electrochemical properties and photovoltaic performances were investigated. Compared with the mono-anchoring dye containing single donor–acceptor chain, these new dyes exhibited a broader and much stronger absorption in the light wavelength ranging from 400 to 600 nm, showed higher IPCE values and short-circuit current density, which led to more efficient photovoltaic performance. The dye with triphenylamine and phenothiazine as two electron donors and two cyanoacrylic acids as two electron acceptors exhibited an impressive power conversion efficiency o…

Photocurrentchemistry.chemical_classificationMaterials scienceProcess Chemistry and TechnologyGeneral Chemical EngineeringEnergy conversion efficiencyElectron acceptorPhotochemistryElectrochemistryTriphenylaminechemistry.chemical_compoundDye-sensitized solar cellchemistryPhenothiazineAbsorption (electromagnetic radiation)Dyes and Pigments
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Electrochemical Growth and Physico-Chemical Characterization in Organic Medium of Nb2O5 Thin Films

2008

Investigations about the energetics and the electrical properties of niobium thin film, electrochemically grown, were performed in an organic solution of acetonitrile and lithium perchlorate. The study of the energetics of the Nb2O5/organic solution interface was performed by means of a non-destructive optical technique, photocurrent spectroscopy. By means of this technique, it was possible estimating the value of the flat band potential and locating conduction and valence band. A more cathodic value of flat band potential in respect with acidic solution was found in organic medium. From impedance spectra, the electrical circuit that gives best fitting values is constituted by two resistanc…

Photocurrentchemistry.chemical_compoundMaterials sciencechemistryPhase (matter)ElectrodeNiobiumAnalytical chemistrychemistry.chemical_elementElectrolyteThin filmElectrochemistryLithium perchlorate2008 2nd ICTON Mediterranean Winter
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Nonadiabatic orientation, toroidal current, and induced magnetic field in BeO molecules.

2008

It is predicted that oriented BeO molecules would give rise to unprecedentedly strong, unidirectional electric ring current and an associated magnetic field upon excitation by a right or left circularly polarized laser pulse into the first excited degenerate singlet state. The strong toroidal electric ring current of this state is dominated by the ring current of the 1π± orbital about the molecular axis. Our predictions are based on the analysis of the orbital composition of the states involved and are substantiated by high level electronic structure calculations and wavepacket simulations of the laser-driven orientation and excitation dynamics. Luis.Serrano@uv.es

PhotoexcitationToroidMolecular electronic statesMolecule-photon collisionsMagnetic momentChemistryConfiguration interactionsExcited statesGeneral Physics and AstronomyElectronic structureMolecular orientationMagnetic fieldUNESCO::FÍSICA::Química físicaPhotoexcitationCoupled cluster calculationsBeryllium compoundsExcited stateMagnetic momentsPhysical and Theoretical ChemistryAtomic physics:FÍSICA::Química física [UNESCO]Beryllium compounds ; Configuration interactions ; Coupled cluster calculations ; Excited states ; Magnetic moments ; Molecular electronic states ; Molecular orientation ; Molecule-photon collisions ; PhotoexcitationRing currentExcitationThe Journal of chemical physics
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Silicon Photomultipliers Signal-to-Noise Ratio in the Continuous Wave Regime

2014

 Abstract— We report on Signal-to-Noise Ratio measurements carried out, in the continuous wave regime, at different bias voltages, frequencies and temperatures, on a class of silicon photomultipliers fabricated in planar technology on silicon p- type substrate. Signal-to-Noise Ratio has been measured as the ratio of the photogenerated current, filtered and averaged by a lock-in amplifier, and the Root Mean Square deviation of the same current. The measured noise takes into account the shot noise, resulting from the photocurrent and the dark current. We have also performed a comparison between our SiPMs and a photomultiplier tube in terms of Signal-to-Noise Ratio, as a function of the tempe…

PhotomultiplierMaterials sciencePhysics::Instrumentation and Detectorsbusiness.industryAmplifierElectrical engineeringShot noiseSettore ING-INF/02 - Campi ElettromagneticiNoise (electronics)Settore ING-INF/01 - ElettronicaAtomic and Molecular Physics and OpticsSignal-to-noise ratioOpticsSilicon photomultiplierSiPM SNR noise silicon detector photomultiplierContinuous waveElectrical and Electronic EngineeringbusinessDark current
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