Search results for "dextrin"

showing 10 items of 297 documents

Development of a coupled diffusion denuder system combined with gas chromatography/mass spectrometry for the separation and quantification of molecul…

2009

This study concerns the development of a coupled diffusion denuder system capable of separating and quantifying gaseous molecular iodine (I(2)) and two other highly reactive iodine species, ICl and HOI, which are collectively named activated iodine compounds (AIC). Both I(2) and AIC are key species in the atmospheric chemistry of iodine. 1,3,5-Trimethoxybenzene (1,3,5-TMB)- and alpha-cyclodextrin/(129)I(-) (alpha-CD/(129)I(-))-coated denuders proved to be suitable for the collection of gaseous AIC and I(2), respectively. The experimental collection efficiencies for AIC (tested as ICl) and I(2) agreed well with the theoretical values for gas flow rates in the range between 300 and 1800 mL mi…

alpha-CyclodextrinsAnalytical chemistryIodine Compoundschemistry.chemical_elementMass spectrometryIodineGas Chromatography-Mass SpectrometryAnalytical ChemistryDiffusionchemistry.chemical_compoundChloridesLimit of DetectionParticle SizeDetection limitAir PollutantsChromatographyAtmosphereEquipment DesignIodidesHypoiodous acidIodine monochloridechemistryAtmospheric chemistryGas chromatographyGasesGas chromatography–mass spectrometryVolatilizationIrelandIodineAnalytical chemistry
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Biochemical and structural features of a novel cyclodextrinase from cow rumen metagenome.

2007

A novel enzyme, RA.04, belonging to the alpha-amylase family was obtained after expression of metagenomic DNA from rumen fluid (Ferrer et al.: Environ. Microbiol. 2005, 7, 1996-2010). The purified RA.04 has a tetrameric structure (280 kDa) and exhibited maximum activity (5000 U/mg protein) at 70 degrees C and was active within an unusually broad pH range from 5.5 to 9.0. It maintained 80% activity at pH 5.0 and 9.5 and 75 degrees C. The enzyme hydrolyzed alpha-D-(1,4) bonds 13-fold faster than alpha-D-(1,6) bonds to yield maltose and glucose as the main products, and it exhibited transglycosylation activity. Its preferred substrates, in the descending order, were maltooligosaccharides (C3-C…

alpha-CyclodextrinsRumenGlycoside HydrolasesStarchAmylopectinOligosaccharidesApplied Microbiology and BiotechnologyCatalysisSubstrate Specificitychemistry.chemical_compoundBacterial ProteinsAmyloseCyclomaltodextrinaseAnimalsMaltoseGlucansChromatography High Pressure Liquidchemistry.chemical_classificationBinding Sitesbiologybeta-CyclodextrinsTemperatureActive sitePullulanStarchGeneral MedicineMaltoseHydrogen-Ion ConcentrationEnzymechemistryBiochemistryAmylopectinbiology.proteinMolecular MedicineCattleElectrophoresis Polyacrylamide GelAmylosegamma-CyclodextrinsBiotechnology journal
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Extensive Evaluation of a Diffusion Denuder Technique for the Quantification of Atmospheric Stable and Radioactive Molecular Iodine

2010

In this paper we present the evaluation and optimization of a new approach for the quantification of gaseous molecular iodine (I(2)) for laboratory- and field-based studies and its novel application for the measurement of radioactive molecular iodine. alpha-Cyclodextrin (alpha-CD) in combination with (129)I(-) is shown to be an effective denuder coating for the sampling of gaseous I(2) by the formation of an inclusion complex. The entrapped (127)I(2) together with the (129)I(-) spike in the coating is then released and derivatized to 4-iodo-N,N-dimethylaniline (4-I-DMA) for gas chromatography-mass spectrometry (GC-MS) analysis. The (127)I(2) collected can be differentiated from the (129)I(-…

alpha-CyclodextrinsTime FactorsAnalytical chemistrychemistry.chemical_elementIodineMass spectrometryGas Chromatography-Mass SpectrometryDiffusionIodine Radioisotopeschemistry.chemical_compoundGermanyEnvironmental ChemistryDerivatizationDetection limitAir PollutantsChromatographyAtmosphereChemistryReproducibility of ResultsGeneral ChemistryIodine RadioisotopesVolumetric flow rateAir Pollutants RadioactiveGasesGas chromatographyGas chromatography–mass spectrometryIrelandEnvironmental MonitoringEnvironmental Science & Technology
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Enantiodifferentiation of N-benzyloxycarbonylaminophosphonic and phosphinic acids and their esters using cyclodextrins by means of capillary electrop…

2005

Capillary electrophoresis was successfully applied for separation of the enantiomers of N-benzyloxycarbonyl-alpha-aminophosphonic and alpha-aminophosphinic acids as well as their ethyl and phenyl monoesters with the use of a range of commercially available cyclodextrins (alpha, beta and hydroxypropyl-gamma-cyclodextrins) as chiral selectors. The dependence of effectiveness of separation on type and concentration of these chiral selectors as well as on pH of background electrolyte was examined in some detail.

aminophosphinatesaminophosphonatesOrganophosphonatescapillary electrophoresisElectrolyteBiochemistryAnalytical ChemistryInclusion compoundchemistry.chemical_compoundCapillary electrophoresisOrganic chemistrychemistry.chemical_classificationChromatographycyclodextrinsMolecular StructureCyclodextrinChemistryOrganic ChemistryenantiodiscriminationElectrophoresis CapillaryReproducibility of ResultsEstersStereoisomerismGeneral MedicineHydrogen-Ion ConcentrationPhosphinic AcidsPhosphinic AcidsPhase compositionEnantiomerJournal of Chromatography A
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Separation of aminoalkanephosphonic acid enantiomers by indirect UV detection capillary electrophoresis with application of cyclodextrins.

2003

Indirect UV detection capillary electrophoresis (CE) was used for the separation of aminoalkanephosphonic acid (AP) enantiomers by applying commercially available cyclodextrins as chiral discriminators. The results show that the separation of the enantiomers depends on pH of the background electrolyte, the molar ratio of cyclodextrin to aminophosphonic acid, and on the type of the applied chiral selector. Optimization of process conditions allowed enantiomeric baseline separation or partial separation of 12 out of 14 alpha-aminophosphonic acids studied. This type of CE might therefore be successfully used for routine determination of enantiomeric purity of aminophosphonic acids.

aminophosphonic acidsClinical Biochemistrycapillary electrophoresisOrganophosphonatesElectrolyteBiochemistryindirect UV detectionAnalytical ChemistryCapillary electrophoresisMolar ratiopolycyclic compoundsheterocyclic compoundsAmineschemistry.chemical_classificationCyclodextrinsChromatographyCyclodextrinorganic chemicalsElectrophoresis CapillaryStereoisomerismHydrogen-Ion ConcentrationProcess conditionschemistrycyclodextrinUv detectionEnantiomerenantiomer separationElectrophoresis
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Thermodynamics of binding between α- and β-cyclodextrins and some p-nitro-aniline derivatives: reconsidering the enthalpy–entropy compensation effect

2004

Abstract The thermodynamics of binding between native α- and β-cyclodextrin towards several p -nitro-aniline derivatives was examined, in order to gain further insights about the occurrence of different interaction modes for the two hosts. Valuable information was achieved regarding the ‘expanded hydrophobic sphere’ of α-cyclodextrin. Furthermore, very interesting and unexpected aspects of the behavior of β-cyclodextrin were enlightened, such as the crucial role played by hydrogen bond interactions. Experimental data were examined under the perspective of the ‘enthalpy–entropy compensation effect’, and some ideas about this topic are discussed.

binding equlibria cyclodextrinchemistry.chemical_compoundAnilinechemistryEnthalpy–entropy compensationHydrogen bondOrganic ChemistryDrug DiscoveryNitroThermodynamicsSettore CHIM/06 - Chimica Organicaβ cyclodextrinsBiochemistryTetrahedron
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CCDC 1899329: Experimental Crystal Structure Determination

2020

Related Article: Ondřej Jurček, Rakesh Puttreddy, Filip Topić, Pia Jurček, Pezhman Zarabadi-Poor, Hendrik V. Schröder, Radek Marek, Kari Rissanen|2020|Cryst.Growth Des.|20|4193|doi:10.1021/acs.cgd.0c00532

bis(mu-hexakis(23-di-O-methyl)-alpha-cyclodextrin)-hexakis(mu-aqua)-nona-silver nona-hexafluorophosphate unknown solvateSpace GroupCrystallographyCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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Docetaxel-Loaded Nanoparticles Assembled from β-Cyclodextrin/Calixarene Giant Surfactants: Physicochemical Properties and Cytotoxic Effect in Prostat…

2017

Giant amphiphiles encompassing a hydrophilic β-cyclodextrin (βCD) component and a hydrophobic calix[4]arene (CA4) module undergo self-assembly in aqueous media to afford core-shell nanospheres or nanocapsules, depending on the nanoprecipitation protocol, with high docetaxel (DTX) loading capacity. The blank and loaded nanoparticles have been fully characterized by dynamic light scattering (DLS), ζ-potential measurements and cryo-transmission electron microscopy (cryo-TEM). The data are compatible with the distribution of the drug between the nanoparticle core and the shell, where it is probably anchored by inclusion of the DTX aromatic moieties in βCD cavities. Indeed, the release kinetics …

calixarenesSupramolecular chemistryNanoparticle02 engineering and technology010402 general chemistry01 natural sciencesNanocapsulesDynamic light scatteringCalixareneAmphiphiledocetaxelPharmacology (medical)Original Researchchemistry.chemical_classificationPharmacologycyclodextrinsCyclodextrinlcsh:RM1-950glioblastoma021001 nanoscience & nanotechnologyprostate cancerCombinatorial chemistry0104 chemical scienceslcsh:Therapeutics. PharmacologychemistryDrug delivery0210 nano-technologyFrontiers in pharmacology
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CCDC 1899331: Experimental Crystal Structure Determination

2020

Related Article: Ondřej Jurček, Rakesh Puttreddy, Filip Topić, Pia Jurček, Pezhman Zarabadi-Poor, Hendrik V. Schröder, Radek Marek, Kari Rissanen|2020|Cryst.Growth Des.|20|4193|doi:10.1021/acs.cgd.0c00532

catena-[triaqua-(mu-hexakis(23-O-methyl)-alpha-cyclodextrin)-silver tetrafluoroborate unknown solvate tetrahydrate]Space GroupCrystallographyCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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Water Adsorption Properties of Free and Dehydrated β-Cyclodextrin Studied by near Infrared Spectroscopy and Gravimetry

2016

β-cyclodextrin, like other carbohydrates has a tendency to adsorb water molecules and the properties are attributed to the hydroxyl groups in the molecules. β-cyclodextrin, the cyclic oligomer of glucose has a hydrophobic interior and hydrophilic exterior. The cyclic structure favours the formation of hydrogen bonds between the OH groups on the adjacent glucose units and affects the formation of hydrogen bonds with water molecules. The hydoxyl groups engaged in hydrogen bondings can be eliminated at high temperatures and the adsorption properties of the dehydrated β-cyclodextrin will depend on the new functional groups formed. The aim of the report is to discuss the issue of the water adsor…

chemistry.chemical_classification010304 chemical physicsHydrogenCyclodextrinChemistryHydrogen bondMechanical Engineering05 social sciencesInorganic chemistrychemistry.chemical_elementHumiditymedicine.disease01 natural sciencesOligomerchemistry.chemical_compoundAdsorptionMechanics of Materials0502 economics and business0103 physical sciencesmedicineOrganic chemistryMoleculeGeneral Materials ScienceDehydration050203 business & managementKey Engineering Materials
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