Search results for "perch"

showing 10 items of 1084 documents

Dinuclear alkoxo-bridged copper(II) coordination polymers: Syntheses, structural and magnetic properties

2010

Abstract The alkoxo-bridged dinuclear copper(II) complexes [Cu2(ap)2(NO2)2] (1), [Cu2(ap)2(C6H5COO)2] (2) and [Cu2(ap)2μ-1,3-C6H4(COO)2(dmso)2]·dmso (3) (ap = 3-aminopropanolato and dmso = dimethyl sulfoxide) have been synthesized via self-assembly from copper(II) perchlorate, 3-aminopropanol as main chelating ligand and nitrite and isophthalate anions as spacers and benzoate anion as auxiliary ligand. Complexes 1 and 3 crystallize as 2D and 1D coordination polymers, respectively, and their structures consist of dinuclear [Cu2(ap)2]2+ units connected with nitrite and isophthalate ligands. The adjacent dinuclear units of 2 and 1D polymers of 3 are further connected by hydrogen bonds resultin…

Hydrogen bondLigandStereochemistrychemistry.chemical_elementSulfoxideCopperInorganic ChemistryPerchloratechemistry.chemical_compoundCrystallographychemistryMaterials ChemistryAntiferromagnetismChelationPhysical and Theoretical ChemistryNitriteInorganica Chimica Acta
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Assembly and encapsulation of coordination tectons driven by hydrogen-bondingand space-filling

2001

[FR] Le composé ¿Fe(LI)3¿2¿Fe(H2O)6¿(ClO4)6 (2), LI = 1,10-phénanthroline-5,6-dione, a été synthétisé et caractérisé. La structure cristalline 2 est définie par un assemblage bidimensionnel non covalent, peu commun, constitué par des tectons chiraux ¿Fe(LI)3¿2+, assemblés par des cations ¿Fe(H2O)6¿2+ encapsulés dans des cages. Ces cages sont formées par 12 liaisons hydrogène établies entre les molécules d¿eau coordinées et les groupes dione appartenant à six molecules chirales ¿Fe(LI)3¿2+ ¿, ¿ alternées.

HydrogenIron(II) low-spin tectonsStereochemistrychemistry.chemical_elementSupramolecular interactionCrystal structureHydrogen bondsPerchloratechemistry.chemical_compoundChemical preparationMoleculeNon-Covalent assemblyInteraction supramoléculaireLigands alpha-diimineDiketoneChemistryHydrogen bondGeneral ChemistryOrthodiquinone ligandsLigands orthodiquinoneAssemblage non covalentCrystallographyFISICA APLICADALiaisons hydrogèneAlpha-Diimine ligandsFer(II) bas spin
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Electrochemistry of hydrotalcite-supported bis(2-mercapto-2,2-diphenyl-ethanoate) dioxomolybdate complexes.

1998

The redox properties of the hydrotalcite-intercalated bis(2-mercapto-2,2-diphenyl-ethanoate) dioxomolybdate(VI) complex are investigated by cyclic voltammetry by using modified carbon paste electrodes and clay-modified electrodes. The electrochemical data provide evidence that boundary-associated species involving the VI, V and IV oxidation states of molybdenum are responsible for the electroactivity.

HydrotalciteGeneral Chemical EngineeringInorganic chemistrychemistry.chemical_elementBuffer solutionSodium perchlorateElectrochemistryRedoxAnalytical Chemistrychemistry.chemical_compoundchemistryMolybdenumPolymer chemistryElectrochemistryCarboxylateCyclic voltammetryJournal of Electroanalytical Chemistry
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Impact of probiotics on risk factors for cardiovascular diseases. A review.

2014

International audience; Probiotic microorganisms have historically been used to rebalance disturbed intestinal microbiota and to diminish gastrointestinal disorders, such as diarrhea or inflammatory bowel diseases (e.g., Crohn's disease and ulcerative colitis). Recent studies explore the potential for expanded uses of probiotics on medical disorders that increase the risk of developing cardiovascular diseases and diabetes, such as obesity, hypercholesterolemia, arterial hypertension, and metabolic disturbances such as hyperhomocysteinemia and oxidative stress. This review aims at summarizing the proposed molecular and cellular mechanisms involved in probiotic-host interactions and to identi…

HypercholesterolemiaHyperhomocysteinemiaDiseaseBiologyIndustrial and Manufacturing Engineeringlaw.invention03 medical and health sciencesProbioticImmune systemRisk Factors[ CHIM.ORGA ] Chemical Sciences/Organic chemistrylawImmunityDiabetes mellitusDiabetes MellitusmedicineAnimalsHumansObesity030304 developmental biology0303 health sciences030306 microbiology[CHIM.ORGA]Chemical Sciences/Organic chemistryMicrobiotaProbioticsImmunityGeneral MedicineLipid Metabolismmedicine.diseaseObesityUlcerative colitisEnzymes3. Good healthIntestinesOxidative StressDiarrheaCardiovascular DiseasesHypertensionImmunologymedicine.symptomFood Science
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An Unexplained Congenital Disorder of Glycosylation-II in a Child with Neurohepatic Involvement, Hypercholesterolemia and Hypoceruloplasminemia

2017

We report on a 12-year-old adopted boy with psychomotor disability, absence seizures, and normal brain MRI. He showed increased (but initially, at 5 months, normal) serum cholesterol, increased alkaline phosphatases, transiently increased transaminases and hypoceruloplasminemia with normal serum and urinary copper. Blood levels of immunoglobulins, haptoglobin, antithrombin, and factor XI were normal. A type 2 serum transferrin isoelectrofocusing and hypoglycosylation of apoCIII pointed to a combined N- and O-glycosylation defect. Neither CDG panel analysis with 79 CDG-related genes, nor whole exome sequencing revealed the cause of this CDG. Whole genome sequencing was not performed since th…

Hypoceruloplasminemiacongenital hereditary and neonatal diseases and abnormalitiesmedicine.medical_specialtySettore MED/09 - Medicina InternaUrinary systemHypercholesterolemiaArticleInternal medicineNeurohepatic involvementmedicineCDG-IIGlycomicsExome sequencingWhole genome sequencingchemistry.chemical_classificationbiologybusiness.industryHaptoglobinAntithrombinmedicine.diseaseDisorders of movement Donders Center for Medical Neuroscience [Radboudumc 3]EndocrinologyMALDI TOFchemistryTransferrinbiology.proteinCDGAntibodybusinessCongenital disorder of glycosylationmedicine.drug
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Elaboration of ammonia gas sensors based on electrodeposited polypyrrole - cobalt phthalocyanine hybrid films

2013

The electrochemical incorporation of a sulfonated cobalt phthalocyanine (sCoPc) in conducting polypyrrole (PPy) was done, in the presence or absence of LiClO4, in order to use the resulting hybrid material for the sensing of ammonia. After electrochemical deposition, the morphological features and structural properties of polypyrrole/phthalocyanine hybrid films were investigated and compared to those of polypyrrole films. A gas sensor consisting in platinum microelectrodes arrays was fabricated using silicon microtechnologies, and the polypyrrole and polypyrrole/phthalocyanine films were electrochemically deposited on the platinum microelectrodes arrays of this gas sensor. When exposed to a…

IndolesSiliconPolymersInorganic chemistrychemistry.chemical_element02 engineering and technology010402 general chemistryElectrochemistryPolypyrroleSensitivity and Specificity01 natural sciencesAnalytical Chemistrychemistry.chemical_compoundAmmoniaOrganometallic CompoundsPyrrolesComputingMilieux_MISCELLANEOUSPlatinumchemistry.chemical_classificationAir PollutantsPerchloratesElectric ConductivityReproducibility of ResultsPolymer021001 nanoscience & nanotechnologyElectroplating0104 chemical sciencesMicroelectrodechemistryLithium CompoundsPhthalocyanine0210 nano-technologyPlatinumHybrid materialMicroelectrodes
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The first authenticated example of triorganotin(IV) perchlorate complexes of some heterocyclic bases

1993

Abstract A convenient method is reported for the synthesis of some novel complexes of composition (R 3 SnL 2 ) ClO 4 where L represents pyridine, γ-picoline, 2,2′-bipyridine and 1,10-phenanthroline; and R  n Bu or Ph. All of the new ionic complexes have been characterized by elemental analysis, molar conductance, infrared, multinuclear nuclear magnetic resonance ( 1 H, 13 C and 119 Sn) and 119 Sn Mossbauer spectroscopies. The complexes of composition (R 3 SnL 2 )ClO 4 exist both in solution and in the solid state with trans -trigonal bipyramidal structure where the R-groups occupy the equatorial positions while the ligands are in the axial position.

InfraredChemistryStereochemistryOrganic ChemistryIonic bondingNuclear magnetic resonance spectroscopyBiochemistryInorganic ChemistryTrigonal bipyramidal molecular geometryPerchloratechemistry.chemical_compoundCrystallographyElemental analysisMössbauer spectroscopyPyridineMaterials ChemistryPhysical and Theoretical ChemistryJournal of Organometallic Chemistry
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Indicaciones de los inhibidores de PCSK9 en la práctica clínica. Recomendaciones de la Sociedad Española de Arteriosclerosis (SEA), 2019

2019

Resumen Un grupo de expertos convocado por la Sociedad Espanola de Arteriosclerosis (SEA) se ha encargado de actualizar el documento de la SEA sobre las indicaciones de los inhibidores de PCSK9 (iPCSK9) en la practica clinica publicadas en 2016. Esta actualizacion es necesaria porque en el periodo transcurrido hasta la actualidad se han publicado los resultados de los ensayos clinicos realizados a gran escala con iPCSK9 que demuestran que, ademas de su alta potencia para disminuir el colesterol aterogenico, disminuyen el riesgo de presentar episodios de enfermedad cardiovascular aterosclerotica en los pacientes con enfermedad tanto estable como reciente, y con un alto grado de seguridad. La…

Inhibidores de la proproteína convertasa subtilisina kexina 9ArteriosclerosisEnfermedad cardiovascularFamilial hypercholesterolemiaClinical indicationsLow density lipoprotein030204 cardiovascular system & hematologyArteriosclerosi03 medical and health sciencesLipoproteínas de baja densidad0302 clinical medicineIndicaciones clínicasTratamientoPharmacology (medical)030212 general & internal medicineConsensus documentHipercolesterolemia familiarNumber needed to treatCardiovascular diseaseDocumento de consensoTreatmentArterioesclerosiCholesterolProprotein convertase subtilisin kexin 9 inhibitorsCardiology and Cardiovascular MedicineColesterolNúmero necesario a tratar
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Schiff-Base Podates – X-ray, NMR and Ab Initio Molecular-Orbital Studies of the Cadmium(II) Complexes of Linear and Three-Armed Podands in Solution a…

1998

Cadmium(II) complexes of two Schiff bases, 1,3-di(pyridine-2-carboxaldimino)propane (C15H16N4, L1)[1] and tris[4-(2′-pyridyl)-3-aza-3-butenyl]amine (C24H27N7, L2)[2] are described. An efficient route utilising molecular sieves for the synthesis of Schiff bases is presented. The ligands L1 and L2 can be described as linear and three-armed podands, respectively, L1 being conformationally flexible and L2 preorganised. Cadmium perchlorate in methanol with L1 yields a crystalline complex [Cd(L1)2](ClO4)2 (1), the structure of which was determined by X-ray structure analysis. The complex 1 has an unusual nonsymmetrical 8-coordinated helical structure and crystallizes in an acentric space group (C…

Inorganic ChemistryCrystallographychemistry.chemical_compoundPerchlorateSchiff baseChemistryComputational chemistryAb initio quantum chemistry methodsAb initioMolecular orbitalNuclear magnetic resonance spectroscopyEnantiomerHEXAEuropean Journal of Inorganic Chemistry
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Synthesis, crystal structure, EXAFS, and magnetic properties of catena [mu-tris(1,2-bis(tetrazol-1-yl)propane-N1,N1')iron(II)] bis(perchlorate). Firs…

2000

[Fe(btzp)3](ClO4)2 (btzp = 1,2-bis(tetrazol-1-yl)propane) represents the first structurally characterized Fe(II) linear chain compound exhibiting thermal spin crossover. It shows a very gradual spin transition (T1/2 = 130 K) which has been followed by magnetic susceptibility measurements and 57Fe Mössbauer spectroscopy. The structure has been solved at 200 and 100 K by single-crystal X-ray analysis. It crystallizes in the trigonal space group P3c1 with Z = 2 Fe(II) units at both temperatures. The molecular structure consists of chains running along the c axis in which the Fe(II) ions are linked by three N4,N4' coordinating bis(tetrazole) ligands. The main difference between the two forms ap…

Inorganic ChemistryPerchloratechemistry.chemical_compoundCrystallographychemistrySpin statesExtended X-ray absorption fine structureOctahedronSpin crossoverSpin transitionCrystal structurePhysical and Theoretical ChemistryMagnetic susceptibilityInorganic chemistry
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