Search results for "raman scattering"
showing 10 items of 284 documents
Multiple four-wave mixing-induced modulational instability in highly birefringent fibers.
2001
Theoretical and experimental results are presented that illustrate efficient generation of new optical frequencies by means of induced modulational instability in birefringent fibers for an initially highly phase-mismatched process. Modulational instability is assisted by multiple four-wave mixing interactions. This technique relaxes the strict spectral limitations imposed by the phase-matching conditions on the signal used for frequency conversion by means of modulational instability.
Magnetic-field-enhanced outgoing excitonic resonance in multi-phonon Raman scattering from polar semiconductors
1996
A combined scattering mechanism involving the states of free electron-hole pairs (exciton continuum) and discrete excitons as intermediate states in the multi-phonon Raman scattering leads to (1) a strong increase of the scattering efficiency in the presence of a high magnetic field and to (2) an outgoing excitonic resonance: the two features are not compatible when only free pairs (leading to a strong increase of the scattering efficiency under the applied magnetic field) or discrete excitons (resulting in the outgoing resonance at the excitonic gap) are taken into account.
Anomalous thermalization of nonlinear optical waves
2010
We report theoretically and experimentally an anomalous thermalization process characterized by an irreversible evolution of the waves towards a novel family of equilibrium states of a fundamental different nature than the standard thermodynamic equilibrium state.
Resonant Raman scattering in self-assembledGaN∕AlNquantum dots
2006
Self-assembled $\mathrm{Ga}\mathrm{N}∕\mathrm{Al}\mathrm{N}$ quantum dots have been investigated by means of Raman scattering. A resonant enhancement of the Raman peaks has been observed when the excitation is tuned above the GaN band-gap energy. The polar mode nature, either quasiconfined or interfacial, has been assigned after comparing with the polar optical modes of spheroidal dots calculated within the framework of the anisotropic dielectric continuum model. The built-in strain of the GaN dots induced a substantial blueshift of the nonpolar ${E}_{2H}$ Raman mode frequency. A theoretical model that analyzes the three-dimensional strain distribution in the quantum dots has been employed …
Resonant hyper-Raman scattering in semiconductors: Excitonic effects
1999
Abstract A theoretical model of resonant hyper-Raman scattering involving two incident photons of frequency ωL is developed. The model is valid for energies 2ℏωL around the absorption edge of the semiconductor, and takes into account Wannier excitons as intermediate states in the scattering process. Both deformation potential and Frohlich interaction are included in the model: It is found that Frohlich-mediated scattering is a dipole-allowed process, in contrast to one-phonon Raman scattering, where the Frohlich mechanism is dipole-forbidden. We have performed numerical calculations of the resonance profile (hyper-Raman cross-section versus 2ℏωL) and applied our model to materials with dipo…
Excitonic model for second-order resonant Raman scattering.
1994
A theoretical model for second-order resonant Raman scattering is presented. The effect of Coulomb interaction between electrons and holes is fully taken into account in the framework of the effective-mass approximation. By introducing discrete and continuous excitonic intermediate states in the Raman process, an explicit expression for the Raman scattering efficiency is given for long-range Fr\"ohlich electron-phonon interaction. The model developed can be used to evaluate Raman profiles around the resonant region. A closed-form expression for all matrix elements of the exciton-phonon interaction is obtained once the Coulomb problem for the relative electron-hole motion is separated in sph…
Electronic and acoustic-phonon inter-Landau-level Raman scattering in GaAs/AlxGa1−xAs multiple quantum wells
1995
We present an experimental study of inter-Landau-level excitations in undoped GaAs/${\mathrm{Al}}_{\mathit{x}}$${\mathrm{Ga}}_{1\mathrm{\ensuremath{-}}\mathit{x}}$As multiple quantum wells in high magnetic fields by means of Raman scattering. The experiments were performed in Faraday backscattering geometry with the field along the growth axis, using circularly polarized light for resonant excitation of low-index magneto-optical transitions between Landau levels. We observe two types of peaks. One of them, present in both Stokes and anti-Stokes regions at a constant Raman shift, corresponds to the electron cyclotron energy. We attribute it to electronic Raman scattering from a quasistationa…
Strong Exciton-Coherent Phonon Coupling in Single-Layer MoS2
2020
Broadband transient absorption with sub-20fs temporal resolution, supported by ab-initio calculations, quantitatively provides the strength of exciton-coherent phonon coupling in 1L-MoS2, showing a resonant profile around the C exciton.
Elastic light scattering from semiconductor structures: Localized versus propagating intermediate electronic excitations
1995
We present a theoretical study of the relative role of localized and propagating intermediate electronic states in the processes of elastic scattering of light. Only localized excitations lead to isotropic scattering in lowest-order perturbation theory. Inhomogeneous broadening of the optical transition affects the scattering efficiency from the ordered and disordered array of localized states in a qualitatively different way. The propagating electronic excitations may only contribute to elastic light scattering via higher-order processes. The scattering of excitons by impurities or the interface roughness potential is suggested as a mechanism for the contribution of propagating excitations…
Spatiotemporal Complexity in Step-Index Multimode Fibers
2016
We study supercontinuum generation in step-index fibers with a varying number of modes. We observe new spatiotemporal effects, including evidence of multimode spectral incoherent solitons, and a universal transition to spatiotemporal complexity.