Search results for "rfa"

showing 10 items of 11106 documents

Protected but Accessible: Oxygen Activation by a Calixarene-Stabilized Undecagold Cluster

2013

DFT computations show that calixarenes stabilize subnanometer Au11 clusters allowing access of small molecules like O2 to reactive metal sites in the core. Maximum of three dioxygen molecules can bind to the cluster, and they are activated to a superoxo O2(-) state. This study predicts that gold clusters could act as viable oxidation catalysts at ambient conditions based on similar principles as the metal centers in enzymes.

inorganic chemicalsta214ta114ChemistryInorganic chemistrychemistry.chemical_elementGeneral ChemistryPhotochemistryBiochemistrySmall moleculeOxygenCatalysisCatalysisMetalColloid and Surface Chemistryvisual_artUndecagoldCalixarenevisual_art.visual_art_mediumCluster (physics)MoleculeJournal of the American Chemical Society
researchProduct

Diastereomeric control of enantioselectivity: evidence for metal cluster catalysis

2014

Enantioselective hydrogenation of tiglic acid effected by diastereomers of the general formula [(μ-H)2Ru3(μ3-S)(CO)7(μ-P–P*)] (P–P* = chiral Walphos diphosphine ligand) strongly supports catalysis by intact Ru3 clusters. A catalytic mechanism involving Ru3 clusters has been established by DFT calculations. peerReviewed

intactLigandStereochemistryMetals and AlloysEnantioselective synthesisDiastereomerTiglic acidGeneral Chemistryhydrogenation catalysisCatalysisSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsCatalysisMetalchemistry.chemical_compoundchemistryvisual_artMaterials ChemistryCeramics and Compositesvisual_art.visual_art_mediumCluster (physics)triruthenium clustersta116Chemical Communications
researchProduct

Results on performance and ageing of solar modules based on Elkem Solar Silicon (ESS™) from installations at various locations

2014

Abstract The present study aims to present the current status of the results obtained using Elkem Solar Silicon (ESS™) as feedstock basis for solar cell and modules. It is shown that solar cells based on ESS™ are able to follow the development of the solar industry obtaining comparable efficiencies to standard polysilicon based cells. The characteristics of ESS™ based solar cells, having normally higher V oc and FF and lower I sc , seem to give clear advantages in the field for solar modules located at high irradiance areas. Results from several locations show enhanced electricity production of ESS™ based solar modules compared to polysilicon at increasing solar irradiance. This is explaine…

integumentary systemSiliconRenewable Energy Sustainability and the Environmentbusiness.industryHigh irradiancefood and beverageschemistry.chemical_elementSolar irradianceEngineering physicsSurfaces Coatings and FilmsElectronic Optical and Magnetic Materialslaw.inventionPhotovoltaic thermal hybrid solar collectorElectricity generationSolar cell efficiencyOpticschemistrySolar industrylawbiological sciencesSolar cellEnvironmental sciencebusinessSolar Energy Materials and Solar Cells
researchProduct

Melanin type and concentration determination using inverse model

2011

Abnormality of melanin production causes skin pigmentation disorders. Currently, assessment of treatment efficacy (under Physician's Global Assessment framework) only refers to visual conditions of skin surface and not the condition of the underlying skin layers and pigments. Albeit researches on models and simulations of light interaction with human skin have been reported, none has been specifically developed for pigmentation analysis of melanin types - eumelanin and pheomelanin. Therefore, our research objectives are to develop image analysis of skin pigmentation for classification and quantification of eumelanin and pheomelanin pigment types in human skin. In this research, the model is…

integumentary systembusiness.industryChemistryModel parametersHuman skinTreatment efficacyResearch objectivesClinical studyMelaninOpticsSkin Pigmentation DisorderSkin surfacesense organsBiological systembusiness2011 National Postgraduate Conference
researchProduct

Measurement of the Fluctuations in the Number of Muons in Extensive Air Showers with the Pierre Auger Observatory

2021

The successful installation, commissioning, and operation of the Pierre Auger Observatory would not have been possible without the strong commitment and effort from the technical and administrative staff in Malargue. We are very grateful to the following agencies and organizations for financial support: Argentina-Comision Nacional de Energia Atomica, Agencia Nacional de Promocion Cientifica y Tecnologica (ANPCyT), Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Gobierno de la Provincia de Mendoza, Municipalidad de Malargue, NDM Holdings and Valle Las Lenas; in gratitude for their continuing cooperation over land access; Australia-the Australian Research Council; Brazil…

interaction: modelPhysics::Instrumentation and DetectorsAstronomyHadronGeneral Physics and AstronomyUltra-high energy cosmic rays muons properties hadronic models01 natural sciencescosmic ray; particle interaction; astroparticle detectorsAugerHigh Energy Physics - ExperimentHigh Energy Physics - Experiment (hep-ex)ironsurface [detector]Observatory[PHYS.HEXP]Physics [physics]/High Energy Physics - Experiment [hep-ex]cosmic rayPhysics4. EducationPhysicsSettore FIS/01 - Fisica Sperimentalemeasured [fluctuation]model [interaction]Astrophysics::Instrumentation and Methods for Astrophysicsmodel: hadronicfluctuation: measured3. Good healthAugerobservatoryparticle interactionSciences exactes et naturellesatmosphere [showers]model [particle]airCherenkov counter: waterAstrophysics::High Energy Astrophysical PhenomenaUHE [cosmic radiation]FOS: Physical sciencesCosmic raydetector: fluorescenceNuclear physicsastroparticle detectorscosmic raysmuon0103 physical sciencescalorimeterddc:53014. Life underwatercosmic radiation: UHEHigh Energy Physicsdistribution functionelectromagnetic component010306 general physicsAstrophysiquePierre Auger Observatoryfluorescence [detector]Muonshowers: atmospherehep-exdetector: surfacewater [Cherenkov counter]particle: modelSmall deviationsFísicaASTROFÍSICAAir showerExperimental High Energy PhysicsElementary Particles and Fieldshadronic [model]High Energy Physics::Experiment
researchProduct

A Lightweight, User-Controlled System for the Home

2006

This paper explores how we designed, with input from some elderly persons, a multi-agent user-controlled network for the home. The system was designed to support the elderly in living longer at home with minimal support. We describe how our work attempts to tackle issues such as privacy, control of personal space, and enjoyment within the home. As the number of elderly individuals’ increases, a certain amount of information gathering or support may be required to assist the elderly in their homes. However, we strongly believe that we should preserve people’s privacy in their homes and ensure that any artifact we propose is seen as enjoyable, aesthetically pleasing and, most importantly, not…

interactive televisionubiquitous computinginformation interfaceelderly
researchProduct

Simulation of Fatigue Delamination Growth in Composites with Different Mode Mixtures

2007

A numerical model, obtained by implementing a cyclic damage model in the framework of an interface element, is here proposed to reproduce the crack growth in laminated composites subjected to cyclically repeated loads. This model, which differs from the few studies in the literature on the topic, applies not only to single fracture modes but also to mixed modes, and to constant or variable crack growth rates. The applied load (in terms of force or displacement) is assumed to oscillate between a minimum and a maximum constant value. The Paris curve can be reproduced with accuracy once some parameters in the numerical model are tuned with experiments. These parameters are preliminarily found…

interface elementMaterials scienceMechanical EngineeringDelaminationMode (statistics)Fracture mechanics02 engineering and technology021001 nanoscience & nanotechnologyCrack growth resistance curvedelaminationFinite element methodDisplacement (vector)020303 mechanical engineering & transports0203 mechanical engineeringMechanics of MaterialsMode couplingMaterials ChemistryCeramics and Compositesfinite element analysis (FEA)fatigueComposite materialSettore ING-IND/15 - Disegno E Metodi Dell'Ingegneria Industriale0210 nano-technologyConstant (mathematics)damageJournal of Composite Materials
researchProduct

Vers une assistance informatisée au diagnostic de la qualité ergonomique d'interfaces

2000

International audience; Notre objectif ici est d'encourager les concepteurs à s'intéresser aux usages de leur produit en prenant davantage en compte les facteurs humains dans la phase de test qui est souvent focalisée sur les aspects techniques. L'idée dans cette étude est donc de faciliter le recours aux utilisateurs comme source d'évaluation lors des tests de conception en apportant aux concepteurs un environnement logiciel de test pratique à mettre en œuvre pour faire évaluer leurs propres produits par des utilisateurs. Nous avons mené deux expériences de nature à explorer la faisabilité de ce projet.

interface homme-machineévaluation par l'utilisateur[SCCO.COMP] Cognitive science/Computer scienceévaluation par inspection[SHS.INFO]Humanities and Social Sciences/Library and information sciences[ SCCO.COMP ] Cognitive science/Computer sciencedocument numérique[ SHS.INFO ] Humanities and Social Sciences/Library and information sciences[SCCO.COMP]Cognitive science/Computer scienceméthode d'évaluation ergonomique assistée par ordinateurcritères de qualité ergonomique[SHS.INFO] Humanities and Social Sciences/Library and information sciencesdocument électronique
researchProduct

Il calcestruzzo poroso per il miglioramento delle condizioni di stabilità dei pendii sede di falda idrica

2022

Reduction of pore water pressures is a useful strate-gy to improve the stability conditions of slopes. Deep draining trenches can be used for this scope. For the realisation of deep trenches, the usual con-ventional construction techniques are not adequate and the use of adjacent vertical panels, built by means of the methods well established for dia-phragm walls, is necessary. However, unbonded ma-terials (i.e. gravels) cannot be used, since the excava-tion of a panel adjacent to already built ones will cause instability. For this scope a bonded material such as the pervious concrete can be used. It must have high permeability, filtering capacity in order to prevent the internal erosion of…

interface shear strengthPervious concreteSettore ICAR/07 - Geotecnicashear keys effect.
researchProduct

La resistenza di interfaccia calcestruzzo poroso-terreni a grana fina per il consolidamento di pendii mediante trincee drenanti profonde

2022

Le trincee drenanti profonde rappresentano uno dei metodi più efficaci per la mitigazione del rischio da frana, in pendii con falda idrica. Esse sono realizzate mediante pannelli o pali secanti. Il riempimento è costituito di calcestruzzo poroso o materiale granulare. Se le trincee sono adeguatamente “innestate” nel terreno stabile e il materiale di riempimento ha sufficiente resistenza e rigidezza come il calcestruzzo poroso, si ha ulteriore in-cremento di resistenza a taglio per effetto shear keys, oltre a quello derivante dalla riduzione delle pressioni in-terstiziali. L’incremento di resistenza è dovuto sia alla resistenza all’interfaccia calcestruzzo–terreni sia a quella intrinseca del…

interface shear strengthPervious concreteSettore ICAR/07 - Geotecnicashear keys effect. Pervious concrete for deep trench drains used to stabilise slopes must simultaneously satisfy many requirements namely adequate hydraulic conductiv-ity adequate shear strength a few days after pour-ing capacity to act as a protective filter for soils in which the drain is installed good resistance to clog-ging and adequate residual hydraulic conductivity. The pervious concrete with appropriated mix-design can effectively satisfy all the abovementioned requirements. If the trenches depth is such that they intersect the sliding surface and if the trenches are adequate-ly "socket" in the layers of stable soil there is a fur-ther increase in shear strength due to the shear keys effect. This latter is in addition to the increase in shear strength resulting from the reduction of inter-stitial pressures that remains the principal scope of the draining trenches. Obviously the increase of shear strength due to the shear keys effect occurs if the trenches are filled with material that have enough strength and stiffness such as the porous concrete. In this case the beneficial effects of the draining trenches on stability are also due to the resistance at the concrete interface of the trench - soils and to the intrinsic resistance of the concrete at the area of the trench intersected by the sliding surface taken into consideration.The increase in resistance due to the shear keys effect can be very significant in relation to the thickness and interspace of the trenches. Results reported in the paper demonstrated that the interface fine grained soil-pervious concrete is higher than the residual shear strength of the soil.
researchProduct