Three beta-decaying states in 128In and 130In resolved for the first time using Penning-trap techniques

2020

Isomeric states in 128In and 130In have been studied with the JYFLTRAP Penning trap at the IGISOL facility. By employing state-of-the-art ion manipulation techniques, three different beta-decaying states in 128In and 130In have been separated and their masses measured. JYFLTRAP was also used to select the ions of interest for identification at a post-trap decay spectroscopy station. A new beta-decaying high-spin isomer feeding the isomer in 128Sn has been discovered in 128In at 1797.6(20) keV. Shell-model calculations employing a CD-Bonn potential re-normalized with the perturbative G-matrix approach suggest this new isomer to be a 16⁺ spin-trap isomer. In 130In, the lowest-lying (10⁻) isom…

Hunt for θ13with LENA

2012

In a hunt for by far missing neutrino mixing angle ?13 the accelerator experiments have recently indicated non-zero value and the dedicated reactor neutrino experiments are moving towards the data-taking phase to confirm that. The small effect of ?13 to the neutrino oscillation probabilities can be also complementarily probed using artificially made source of mono-chromatic neutrinos with low energies originated from electron capture processes. Due to the small energy of neutrino and tiny interaction cross section, and the expected scale of ?13 support the use of large liquid scintillation detector. In this work, the estimated sensitivities for measurement of mixing angle ?13 is presented i…

Precision mass measurements on neutron-rich rare-earth isotopes at JYFLTRAP - reduced neutron pairing and implications for the $r$-process calculatio…

2018

The rare-earth peak in the $r$-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in $r$-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. $^{158}$Nd, $^{160}$Pm, $^{162}$Sm, and $^{164-166}$Gd have been measured for the first time and the precisions for $^{156}$Nd, $^{158}$Pm, $^{162,163}$Eu, $^{163}$Gd, and $^{164}$Tb have been improved considerably. Nuclear structure has been probed via two-neutron separation energies $S_{2n}$ and neutron pairing energy metrics…

Excited states in Br87 populated in β decay of Se87

2019

First isomeric yield ratio measurements by direct ion counting and implications for the angular momentum of the primary fission fragments

2018

We report the first experimental determination of independent isomeric yield ratios using direct ion counting with a Penning trap, which offered such a high resolution in mass that isomeric states could be separated. The measurements were performed at the Ion Guide Isotope Separator On-Line (IGISOL) facility at the University of Jyvaskyla. The isomer production ratios of Ge-81, Y-96,Y-97 Sn-128(,1)30, and Sb-129 in the 25-MeV proton-induced fission of U-na(t) and Th-232 were studied. Three isomeric pairs (Ge-81, Y-96, and Sb-129) were measured for the first time for the U-na(t)(p, f) reaction, while all the reported yield ratios for the Th-232(p, f) reaction were determined for the first ti…

β decay of Cd127 and excited states in In127

2019

A dedicated spectroscopic study of the β decay of 127Cd was conducted at the IGISOL facility at the University of Jyvaskyla. Following high-resolution mass separation in a Penning trap, β-γ-γ coincidences were used to considerably extend the decay scheme of 127In. The β-decaying 3/2+ and 11/2- states in 127Cd have been identified with the 127Cd ground state and the 283-keV isomer. Their respective half-lives have been measured to 0.45(+12-8)s and 0.36(4) s. The experimentally observed β feeding to excited states of 127In and the decay scheme of 127In are discussed in conjunction with large-scale shell-model calculations.

Precision Mass Measurements on Neutron-Rich Rare-Earth Isotopes at JYFLTRAP : Reduced Neutron Pairing and Implications for r-Process Calculations

2018

The rare-earth peak in the r-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step towards elucidating the nuclear structure and reducing the uncertainties in r-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. Nd158, Pm160, Sm162, and Gd164-166 have been measured for the first time, and the precisions for Nd156, Pm158, Eu162,163, Gd163, and Tb164 have been improved considerably. Nuclear structure has been probed via two-neutron separation energies S2n and neutron pairing energy metrics Dn. The data do not support the existence of…

Impact of nuclear mass measurements in the vicinity of 132Sn on the r-process nucleosynthesis

2022

Nuclear masses are a key aspect in the modelling of nuclear reaction rates for the r-process nucleosynthesis. High precision mass measurements drastically reduce the associated uncertainties in the modelling of r-process nucleosynthesis. We investigate the impact of nuclear mass uncertainties on neutron-capture rates calculations using a Hauser – Feshbach statistical code in the vicinity of 132Sn. Finally, we study the impact of the propagated neutron-capture reaction rates uncertainties on the r-process nucleosynthesis. We find that mass measurements with uncertainties higher than 20 keV affect the calculation of reaction rates. We also note that modelling of reaction rates can differ for …

Single and Double Beta-DecayQValues among the TripletZr96,Nb96, andMo96

2016

The atomic mass relations among the mass triplet ^{96}Zr, ^{96}Nb, and ^{96}Mo have been determined by means of high-precision mass measurements using the JYFLTRAP mass spectrometer at the IGISOL facility of the University of Jyvaskyla. We report Q values for the ^{96}Zr single and double β decays to ^{96}Nb and ^{96}Mo, as well as the Q value for the ^{96}Nb single β decay to ^{96}Mo, which are Q_{β}(^{96}Zr)=163.96(13), Q_{ββ}(^{96}Zr)=3356.097(86), and Q_{β}(^{96}Nb)=3192.05(16)  keV. Of special importance is the ^{96}Zr single β-decay Q value, which has never been determined directly. The single β decay, whose main branch is fourfold unique forbidden, is an alternative decay path to the…

Fission studies at IGISOL/JYFLTRAP: Simulations of the ion guide for neutron-induced fission and comparison with experimental data

2020

For the production of exotic nuclei at the IGISOL facility, an ion guide for neutron-induced fission has been developed and tested in experiments. Fission fragments are produced inside the ion guide and collected using a helium buffer gas. Meanwhile, a GEANT4 model has been developed to simulate the transportation and stopping of the charged fission products. In a recent measurement of neutron-induced fission yields, implantation foils were located at different positions in the ion guide. The gamma spectra from these foils and the fission targets are compared to the results from the GEANT4 simulation. In order to allow fission yield measurements in the low yield regions, towards the tails a…

Study of radial motion phase advance during motion excitations in a Penning trap and accuracy of JYFLTRAP mass spectrometer

2021

Phase-imaging ion-cyclotron-resonance technique has been implemented at the Penning-trap mass spectrometer JYFLTRAP and is routinely employed for mass measurements of stable and short-lived nuclides produced at IGISOL facility. Systematic uncertainties that impose limitations on the accuracy of measurements are discussed. It was found out that the phase evolution of the radial motion of ions in a Penning trap during the application of radio-frequency fields leads to a systematic cyclotron frequency shift when more than one ion species is present in the trap during the cyclotron frequency measurement. An analytic expression was derived to correctly account for the shift. Cross-reference mass…

Recent developments for high-precision mass measurements of the heaviest elements at SHIPTRAP

2013

Abstract Atomic nuclei far from stability continue to challenge our understanding. For example, theoretical models have predicted an “island of stability” in the region of the superheavy elements due to the closure of spherical proton and neutron shells. Depending on the model, these are expected at Z = 114, 120 or even 126 and N = 172 or 184. Valuable information on the road to the island of stability is derived from high-precision mass measurements, which give direct access to binding energies of short-lived trans-uranium nuclei. Recently, direct mass measurements at SHIPTRAP have been extended to nobelium and lawrencium isotopes around the deformed shell gap N = 152. In order to further …

High-precision mass measurement of $^{168}$Yb for verification of nonlinear isotope shift

2020

The absolute mass value of $^{168}$Yb has been directly determined with the JYFLTRAP Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line (IGISOL) facility. A more precise value of the mass of $^{168}$Yb is needed to extract possible signatures of beyond standard model physics from high-precision isotope shift measurements of Yb atomic transition frequencies. The measured mass-excess value, ME($^{168}$Yb) = $-$61579.846(94) keV, is 12 times more precise and deviates from the Atomic Mass Evaluation 2016 value by 1.7$\sigma$. The impact on precision isotope shift studies of the stable Yb isotopes is discussed.

High-precision measurement of the mass difference between 102Pd and 102Ru

2019

The Q-value for the neutrinoless double electron capture on 102Pd, Qϵϵ(102Pd), is determined as the atomic mass difference between 102Pd and 102Ru. A precise measurement of the Qϵϵ(102Pd) at the SHIPTRAP Penning trap showed a more than 10σ deviation to the adopted Atomic Mass Evaluation (AME) value. The reliability of the SHIPTRAP measurement was challenged because the AME value was based on numerous experiments including β and electron capture decays and very precise (n, γ) data, all agreeing with each other. To solve the discrepancy, the Qϵϵ(102Pd) has now been determined with the JYFLTRAP Penning trap at the IGISOL facility in the Accelerator Laboratory of the University of Jyväskylä. Th…

Quantum-state-selective decay spectroscopy of Ra213

2017

An experimental scheme combining the mass resolving power of a Penning trap with contemporary decay spectroscopy has been established at GSI Darmstadt. The Universal Linear Accelerator (UNILAC) at GSI Darmstadt provided a $^{48}\mathrm{Ca}$ beam impinging on a thin $^{170}\mathrm{Er}$ target foil. Subsequent to velocity filtering of reaction products in the Separator for Heavy Ion reaction Products (SHIP), the nuclear ground state of the $5n$ evaporation channel $^{213}\mathrm{Ra}$ was mass-selected in SHIPTRAP, and the $^{213}\mathrm{Ra}$ ions were finally transferred into an array of silicon strip detectors surrounded by large composite germanium detectors. Based on comprehensive geant4 s…

High-precision mass measurements for the isobaric multiplet mass equation atA= 52

2017

Masses of $^{52}$Co, $^{52}$Co$^m$, $^{52}$Fe, $^{52}$Fe$^m$, and $^{52}$Mn have been measured with the JYFLTRAP double Penning trap mass spectrometer. Of these, $^{52}$Co and $^{52}$Co$^m$ have been experimentally determined for the first time and found to be more bound than predicted by extrapolations. The isobaric multiplet mass equation for the $T=2$ quintet at $A=52$ has been studied employing the new mass values. No significant breakdown (beyond the $3\sigma$ level) of the quadratic form of the IMME was observed ($\chi^2/n=2.4$). The cubic coefficient was 6.0(32) keV ($\chi^2/n=1.1$). The excitation energies for the isomer and the $T=2$ isobaric analogue state in $^{52}$Co have been d…

High-precision measurement of the mass difference between 102Pd and 102Ru

2019

Abstract The Q-value for the neutrinoless double electron capture on 102Pd, Qϵϵ(102Pd), is determined as the atomic mass difference between 102Pd and 102Ru. A precise measurement of the Qϵϵ(102Pd) at the SHIPTRAP Penning trap showed a more than 10σ deviation to the adopted Atomic Mass Evaluation (AME) value. The reliability of the SHIPTRAP measurement was challenged because the AME value was based on numerous experiments including β and electron capture decays and very precise (n, γ) data, all agreeing with each other. To solve the discrepancy, the Qϵϵ(102Pd) has now been determined with the JYFLTRAP Penning trap at the IGISOL facility in the Accelerator Laboratory of the University of Jyva…

Precision mass measurements of Fe67 and Co69,70 : Nuclear structure toward N=40 and impact on r -process reaction rates

2020

Accurate mass measurements of neutron-rich iron and cobalt isotopes $^{67}\mathrm{Fe}$ and $^{69,70}\mathrm{Co}$ have been realized with the JYFLTRAP double Penning-trap mass spectrometer. With novel ion-manipulation techniques, the masses of the $^{69,70}\mathrm{Co}$ ground states and the $1/{2}^{\ensuremath{-}}$ isomer in $^{69}\mathrm{Co}$ have been extracted for the first time. The measurements remove ambiguities in the previous mass values and yield a smoother trend on the mass surface, extending it beyond $N=40$. The moderate $N=40$ subshell gap has been found to weaken below $^{68}\mathrm{Ni}$, a region known for shape coexistence and increased collectivity. The excitation energy for…

Precision Ga71–Ge71 mass-difference measurement

2016

Abstract The Ga 71 ( ν e , e − ) Ge 71 reaction Q value has been measured with the JYFLTRAP mass spectrometer at the IGISOL facility of the University of Jyvaskyla to Q  = 232.443(93) keV. This value agrees with previous measurements, though it features a much higher accuracy. The Q value is being discussed in the context of the solar neutrino capture rate in Ga 71 .

Double-βtransformations in isobaric triplets with mass numbersA=124, 130, and 136

2012

The Q values of double-electron capture in ${}^{124}$Xe, ${}^{130}$Ba, and ${}^{136}$Ce and double-beta decay of ${}^{124}$Sn and ${}^{130}$Te have been determined with the Penning-trap mass spectrometer SHIPTRAP with a few hundred eV uncertainty. These nuclides are members of three isobaric triplets with common daughter nuclides. The main goal of this work was to investigate the existence of the resonant enhancement of the neutrinoless double-electron-capture rates in ${}^{124}$Xe and ${}^{130}$Ba in order to assess their suitability for the search for neutrinoless double-electron capture. Based on our results, in neither of these cases is the resonance condition fulfilled.

High-Precision Q -Value Measurement Confirms the Potential of Cs135 for Absolute Antineutrino Mass Scale Determination

2020

The ground-state-to-ground-state $\ensuremath{\beta}$-decay $Q$ value of $^{135}\mathrm{Cs}(7/{2}^{+})\ensuremath{\rightarrow}^{135}\mathrm{Ba}(3/{2}^{+})$ has been directly measured for the first time. The measurement was done utilizing both the phase-imaging ion-cyclotron resonance technique and the time-of-flight ion-cyclotron resonance technique at the JYFLTRAP Penning-trap setup and yielded a mass difference of 268.66(30) keV between $^{135}\mathrm{Cs}(7/{2}^{+})$ and $^{135}\mathrm{Ba}(3/{2}^{+})$. With this very small uncertainty, this measurement is a factor of 3 more precise than the currently adopted $Q$ value in the Atomic Mass Evaluation 2016. The measurement confirms that the f…

β Decay of 127Cd and Excited States in 127In

2019

A dedicated spectroscopic study of the β decay of 127Cd was conducted at the IGISOL facility at the University of Jyväskylä. Following high-resolution mass separation in a Penning trap, β−γ−γcoincidences were used to considerably extend the decay scheme of 127In. The β-decaying 3/2+ and 11/2− states in 127Cd have been identified with the 127Cd ground state and the 283-keV isomer. Their respective half-lives have been measured to 0.45(128)s and 0.36(4) s. The experimentally observed βfeeding to excited states of 127In and the decay scheme of 127In are discussed in conjunction with large-scale shell-model calculations. peerReviewed

Exploring the mass surface near the rare-earth abundance peak via precision mass measurements at JYFLTRAP

2019

The JYFLTRAP double Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility has been used to measure the atomic masses of 13 neutron-rich rare-earth isotopes. Eight of the nuclides, $^{161}$Pm, $^{163}$Sm, $^{164,165}$Eu, $^{167}$Gd, and $^{165,167,168}$Tb, were measured for the first time. The systematics of the mass surface has been studied via one- and two-neutron separation energies as well as neutron pairing-gap and shell-gap energies. The proton-neutron pairing strength has also been investigated. The impact of the new mass values on the astrophysical rapid neutron capture process has been studied. The calculated abundance distribution results in a better agreement w…

Mass Measurements for the rp Process

2017

One of the key parameters for the reaction network calculations for the rapid proton capture (rp) process, occurring e.g., in type I X-ray bursts, are the masses of the involved nuclei. Nowadays, masses of even rather exotic nuclei can be measured very precisely employing Penning-trap mass spectrometry. With the JYFLTRAP Penning trap at the IGISOL facility, masses of around 100 neutron-deficient nuclei have been determined with a typical precision of a few keV. Most recently, 25Al, 30P, 31Cl, and 52Co have been measured. Of these, the precision of the mass-excess value of 31Cl was improved from 50 to 3.4 keV, and the mass of 52Co was experimentally determined for the first time. The mass of…

Phase-Imaging Ion-Cyclotron-Resonance Measurements for Short-Lived Nuclides

2013

A novel approach based on the projection of the Penning-trap ion motion onto a position-sensitive detector opens the door to very accurate mass measurements on the ppb level even for short-lived nuclides with half-lives well below a second. In addition to the accuracy boost, the new method provides a superior resolving power by which low-lying isomeric states with excitation energy on the 10-keV level can be easily separated from the ground state. A measurement of the mass difference of ^{130}Xe and ^{129}Xe has demonstrated the great potential of the new approach.

Impact of nuclear mass measurements in the vicinity of 132Sn on the r-process nucleosynthesis

2022

Nuclear masses are a key aspect in the modelling of nuclear reaction rates for the r-process nucleosynthesis. High precision mass measurements drastically reduce the associated uncertainties in the modelling of r-process nucleosynthesis. We investigate the impact of nuclear mass uncertainties on neutron-capture rates calculations using a Hauser – Feshbach statistical code in the vicinity of 132Sn. Finally, we study the impact of the propagated neutron-capture reaction rates uncertainties on the r-process nucleosynthesis. We find that mass measurements with uncertainties higher than 20 keV affect the calculation of reaction rates. We also note that modelling of reaction rates can differ for …

A new off-line ion source facility at IGISOL

2019

An off-line ion source station has been commissioned at the IGISOL (Ion Guide Isotope Separator On-Line) facility. It offers the infrastructure needed to produce stable ion beams from three off-line ion sources in parallel with the radioactive ion beams produced from the IGISOL target chamber. This has resulted in improved feasibility for new experiments by offering reference ions for Penning-trap mass measurements, laser spectroscopy and atom trap experiments.

High-precision mass measurements and production of neutron-deficient isotopes using heavy-ion beams at IGISOL

2019

An upgraded ion-guide system for the production of neutron-deficient isotopes with heavy-ion beams has been commissioned at the IGISOL facility with an $^{36}\mathrm{Ar}$ beam on a $^{\mathrm{nat}}\mathrm{Ni}$ target. It was used together with the JYFLTRAP double Penning trap to measure the masses of $^{82}\mathrm{Zr}, ^{84}\mathrm{Nb}, ^{86}\mathrm{Mo}, ^{88}\mathrm{Tc}$, and $^{89}\mathrm{Ru}$ ground states and the isomeric state $^{88}\mathrm{Tc}^{m}$. Of these, $^{89}\mathrm{Ru}$ and $^{88}\mathrm{Tc}^{m}$ were measured for the first time. The precision of measurements of $^{82}\mathrm{Zr}, ^{84}\mathrm{Nb}$, and $^{88}\mathrm{Tc}$ was significantly improved. The literature value for $^…

Fission studies at IGISOL/JYFLTRAP: Simulations of the ion guide for neutron-induced fission and comparison with experimental data

2020

For the production of exotic nuclei at the IGISOL facility, an ion guide for neutron-induced fission has been developed and tested in experiments. Fission fragments are produced inside the ion guide and collected using a helium buffer gas. Meanwhile, a GEANT4 model has been developed to simulate the transportation and stopping of the charged fission products. In a recent measurement of neutron-induced fission yields, implantation foils were located at different positions in the ion guide. The gamma spectra from these foils and the fission targets are compared to the results from the GEANT4 simulation. In order to allow fission yield measurements in the low yield regions, towards the tails a…

First β -decay scheme of Nb107 : New insight into the low-energy levels of Mo107

2019

Monoisotopic samples of $^{107}\mathrm{Nb}$ nuclei, produced in the proton-induced fission of $^{238}\mathrm{U}$ and separated using the IGISOL mass separator coupled to a Penning trap, were used to perform $\ensuremath{\beta}$- and $\ensuremath{\gamma}$-coincidence spectroscopy of $^{107}\mathrm{Mo}$. Gamma transitions and excited levels in $^{107}\mathrm{Mo}$ were observed in $\ensuremath{\beta}$ decay for the first time. Spin and parity $1/{2}^{+}$ for the ground state of $^{107}\mathrm{Mo}$ is proposed, to replace the previous $5/{2}^{+}$ assignment. The experimental $\ensuremath{\beta}$-decay half-life of $^{107}\mathrm{Nb}$ was estimated to be $0.27\ifmmode\pm\else\textpm\fi{}0.02$ s.

Investigation of the magnetic field fluctuation and implementation of a temperature and pressure stabilization at SHIPTRAP

2011

Abstract Penning traps have proven to be powerful tools for the determination of nuclear masses with high accuracy. A crucial parameter for precision mass measurements in Penning traps is the accurate determination of the magnetic-field strength. However, the magnetic field of a superconducting magnet is not constant in time, but changes due to intrinsic effects of the solenoid and external perturbations. These effects have been investigated for SHIPTRAP. Furthermore, a stabilization of the temperature in the magnet bore as well as of the pressure in the liquid-helium cryostat has been implemented. Thus, the magnetic-field related uncertainties have been reduced to 7(6)×10−11/h.

Mass of astrophysically relevantCl31and the breakdown of the isobaric multiplet mass equation

2016

The mass of $^{31}\mathrm{Cl}$ has been measured with the JYFLTRAP double-Penning-trap mass spectrometer at the Ion Guide Isotope Separator On-Line (IGISOL) facility. The determined mass-excess value, $\ensuremath{-}7034.7(34)$ keV, is 15 times more precise than in the Atomic Mass Evaluation 2012. The quadratic form of the isobaric multiplet mass equation for the $T=3/2$ quartet at $A=31$ fails $({\ensuremath{\chi}}_{n}^{2}=11.6)$ and a nonzero cubic term, $d=\ensuremath{-}3.5(11)$ keV, is obtained when the new mass value is adopted. $^{31}\mathrm{Cl}$ has been found to be less proton-bound, with a proton separation energy of ${S}_{p}=264.6(34)$ keV. Energies for the excited states in $^{31…

Production of Sn and Sb isotopes in high-energy neutron induced fission of natU

2018

The first systematic measurement of neutron-induced fission yields has been performed at the upgraded IGISOL-4 facility at the University of Jyväskylä, Finland. The fission products from high-energy neutron-induced fission of nat U were stopped in a gas cell filled with helium buffer gas, and were online separated with a dipole magnet. The isobars, with masses in the range A = 128-133 , were transported to a tape-implantation station and identified using γ -spectroscopy. We report here the relative cumulative isotopic yields of tin (Z = 50) and the relative independent isotopic yields of antimony (Z = 51). Isomeric yield ratios were also obtained for five nuclides. The yields of tin show a …

Evidence of a sudden increase in the nuclear size of proton-rich silver-96

2021

Understanding the evolution of the nuclear charge radius is one of the long-standing challenges for nuclear theory. Recently, density functional theory calculations utilizing Fayans functionals have successfully reproduced the charge radii of a variety of exotic isotopes. However, difficulties in the isotope production have hindered testing these models in the immediate region of the nuclear chart below the heaviest self-conjugate doubly-magic nucleus 100Sn, where the near-equal number of protons (Z) and neutrons (N) lead to enhanced neutron-proton pairing. Here, we present an optical excursion into this region by crossing the N = 50 magic neutron number in the silver isotopic chain with th…

Extending Penning trap mass measurements with SHIPTRAP to the heaviest elements

2013

Penning-trap mass spectrometry of radionuclides provides accurate mass values and absolute binding energies. Such mass measurements are sensitive indicators of the nuclear structure evolution far away from stability. Recently, direct mass measurements have been extended to the heavy elements nobelium (Z=102) and lawrencium (Z=103) with the Penning-trap mass spectrometer SHIPTRAP. The results probe nuclear shell effects at N=152. New developments will pave the way to access even heavier nuclides.

Precision 71Ga – 71Ge mass-difference measurement

2016

The 71Ga(νe, e−) 71Ge reaction Q value has been measured with the JYFLTRAP mass spectrometer at the IGISOL facility of the University of Jyv¨askyl¨a to Q = 232.443(93) keV. This value agrees with previous measurements, though it features a much higher accuracy. The Q value is being discussed in the context of the solar neutrino capture rate in 71Ga. peerReviewed

Direct Mapping of Nuclear Shell Effects in the Heaviest Elements

2014

Quantum-mechanical shell effects are expected to strongly enhance nuclear binding on an "island of stability" of superheavy elements. The predicted center at proton number $Z=114,120$, or $126$ and neutron number $N=184$ has been substantiated by the recent synthesis of new elements up to $Z=118$. However the location of the center and the extension of the island of stability remain vague. High-precision mass spectrometry allows the direct measurement of nuclear binding energies and thus the determination of the strength of shell effects. Here, we present such measurements for nobelium and lawrencium isotopes, which also pin down the deformed shell gap at $N=152$.

Phase-Imaging Ion-Cyclotron-Resonance technique at the JYFLTRAP double Penning trap mass spectrometer

2018

The Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique has been commissioned at the JYFLTRAP double Penning trap mass spectrometer. This technique is based on projecting the ion motion in the Penning trap onto a position-sensitive multichannel-plate ion detector. Mass measurements of stable 85 Rb $ ^{+}$ and 87 Rb $ ^{+}$ ions with well-known mass values show that relative uncertainties $ \Delta m/m \leq 7\cdot 10^{-10}$ are possible to reach with the PI-ICR technique at JYFLTRAP. The significant improvement both in resolving power and in precision compared to the conventional Time-of-Flight Ion Cyclotron Resonance technique will enable measurements of close-lying isomeric states and …

Direct measurement of the mass difference of As72−Ge72 rules out As72 as a promising β -decay candidate to determine the neutrino mass

2021

We report the first direct determination of the ground-state to ground-state electron-capture $Q$ value for the $^{72}\mathrm{As}$ to $^{72}\mathrm{Ge}$ decay by measuring their atomic mass difference utilizing the double Penning trap mass spectrometer, JYFLTRAP. The $Q$ value was measured to be 4343.596(75) keV, which is more than a fiftyfold improvement in precision compared to the value in the most recent Atomic Mass Evaluation 2020. Furthermore, the new $Q$ value was found to be 12.4(40) keV (3.1 $\ensuremath{\sigma}$) lower. With the significant reduction of the uncertainty of the ground-state to ground-state $Q$ value combined with the level scheme of $^{72}\mathrm{Ge}$ from $\ensurem…

Isomeric fission yield ratios for odd-mass Cd and In isotopes using the Phase-Imaging Ion-Cyclotron-Resonance technique

2018

Isomeric yield ratios for the odd-$A$ isotopes of $^{119-127}$Cd and $^{119-127}$In from 25-MeV proton-induced fission on natural uranium have been measured at the JYFLTRAP double Penning trap, by employing the Phase-Imaging Ion-Cyclotron-Resonance technique. With the significantly improved mass resolution of this novel method isomeric states separated by 140 keV from the ground state, and with half-lives of the order of 500 ms, could be resolved. This opens the door for obtaining new information on low-lying isomers, of importance for nuclear structure, fission and astrophysics. In the present work the experimental isomeric yield ratios are used for the estimation of the root-mean-square a…

Measurement of the 2+→0+ ground-state transition in the β decay of F20

2019

We report the first detection of the second-forbidden, nonunique, 2+→0+, ground-state transition in the β decay of F20. A low-energy, mass-separated F+20 beam produced at the IGISOL facility in Jyvaskyla, Finland, was implanted in a thin carbon foil and the β spectrum measured using a magnetic transporter and a plastic-scintillator detector. The β-decay branching ratio inferred from the measurement is bβ=[0.41±0.08(stat)±0.07(sys)]×10-5 corresponding to logft=10.89(11), making this one of the strongest second-forbidden, nonunique β transitions ever measured. The experimental result is supported by shell-model calculations and has significant implications for the final evolution of stars tha…