Model independent determination of the spin of theTa180naturally occurring isomer

The hyperfine structures of the 33715.27 ${\mathrm{cm}}^{\ensuremath{-}1}$ and 33706.47 ${\mathrm{cm}}^{\ensuremath{-}1}$ transitions from the ground state of singly ionized Ta have been measured by collinear laser spectroscopy. The structures were found to contain a large second order contribution. From fitting the observed hyperfine components for both $^{181}\mathrm{Ta}$ and the $^{180}\mathrm{Ta}$ naturally occurring isomer it was possible to determine the first and second order hyperfine structure coefficients. As no model independent determination of the nuclear spin of the $^{180}\mathrm{Ta}$ isomer has been performed, fitting was attempted for a range of spins. A clear chi-squared m…

Evidence for Increased neutron and proton excitations between 51−63 Mn

The hyperfine structures of the odd-even 51−63Mnatoms (N=26 −38) were measured using bunched beam collinear laser spectroscopy at ISOLDE, CERN. The extracted spins and magnetic dipole moments have been compared to large-scale shell-model calculations using different model spaces and effective interactions. In the case of 61,63Mn, the results show the increasing importance of neutron excitations across the N=40subshell closure, and of proton excitations across the Z=28shell gap. These measurements provide the first direct proof that proton and neutron excitations across shell gaps are playing an important role in the ground state wave functions of the neutron-rich Mn isotopes. publisher: Els…

Evolution of nuclear structure in neutron-rich odd-Zn isotopes and isomers

Collinear laser spectroscopy was performed on Zn (Z=30) isotopes at ISOLDE, CERN. The study of hyperfine spectra of nuclei across the Zn isotopic chain, N=33–49, allowed the measurement of nuclear spins for the ground and isomeric states in odd-A neutron-rich nuclei up to N=50. Exactly one long-lived (&

Collinear laser spectroscopy of stable palladium isotopes at the IGISOL facility

AbstractCollinear laser spectroscopy on stable palladium isotopes was performed at the IGISOL facility in Jyväskylä in preparation for an experiment on its neutron-rich isotopes. Five transitions from different initial atomic states were tested, with the goal of finding the most spectroscopically efficient. The observed intensities afforded a comparison with atomic-level population predictions based on charge-exchange calculations. For some transitions hyperfine parameters of 105Pd were measured, which were found to be in good agreement with literature values. A King plot analysis was performed using the measured isotope shifts and known charge radii from literature to determine the atomic …

Nuclear mean-square charge radii of63,64,66,68−82Ga nuclei: No anomalous behavior atN=32

Collinear laser spectroscopy was performed on the ${}^{63,64,66,68\ensuremath{-}82}$Ga isotopes with neutron numbers from $N=32$ to $N=51$. These measurements were carried out at the ISOLDE radioactive ion beam facility at CERN. Here we present the nuclear mean-square charge radii extracted from the isotope shifts and, for the lighter isotopes, new spin and moment values. New ground-state nuclear spin and moments were extracted from the hyperfine spectra of ${}^{63,70}$Ga, measured on an atomic transition in the neutral atom. The ground-state spin of ${}^{63}$Ga is determined to be $I=3/2$. Analysis of the trend in the change in mean-square charge radii of the gallium isotopes demonstrates …

Upgrades to the collinear laser spectroscopy experiment at the IGISOL

Abstract We give an overview of recent changes to the collinear laser spectroscopy beamline in the IGISOL laboratory. We present a new data acquisition system, commissioning of a newly installed charge exchange cell, and cooler-voltage calibration measurements. Currently ongoing modifications to the RFQ cooler-buncher are also discussed.

Probing Sizes and Shapes of Nobelium Isotopes by Laser Spectroscopy

Until recently, ground-state nuclear moments of the heaviest nuclei could only be inferred from nuclear spectroscopy, where model assumptions are required. Laser spectroscopy in combination with modern atomic structure calculations is now able to probe these moments directly, in a comprehensive and nuclear-model-independent way. Here we report on unique access to the differential mean-square charge radii of ^{252,253,254}No, and therefore to changes in nuclear size and shape. State-of-the-art nuclear density functional calculations describe well the changes in nuclear charge radii in the region of the heavy actinides, indicating an appreciable central depression in the deformed proton densi…

High-resolution laser spectroscopy of Al27–32

Hyperfine spectra of $^\text{27-32}$Al ($Z=13$) have been measured at the ISOLDE-CERN facility via collinear laser spectroscopy using the $3s^23p\ ^2\text{P}^\text{o} _{3/2}\rightarrow 3s^24s\ ^2\text{S}_{1/2}$ atomic transition. For the first time, mean-square charge radii of radioactive aluminum isotopes have been determined alongside the previously unknown magnetic dipole moment of $^{29}$Al and electric quadrupole moments of $^{29,30}$Al. A potentially reduced charge radius at $N=19$ may suggest an effect of the $N=20$ shell closure, which is visible in the Al chain, contrary to other isotopic chains in the $sd$ shell. The experimental results are compared to theoretical calculations in…

Laser spectroscopy with an electrostatic ConeTrap

A compact electrostatic trap has been designed and installed as part of the recent upgrades to the IGISOL IV facility. The ConeTrap provides an in vacuo optical pumping site for low energy (800 eV) ionic ensembles available for interaction periods of 10-100 ms. At present, 6.7(3) % of injected mass A=98 ions can be trapped, stored for 5 ms, extracted and transported to a laser-ion interaction region. This fraction represents those ions for which no perturbation to total energy or energy spread is observed. Proposed enhancements to the trap are designed to improve the trapping efficiency by up to a factor of 5. Differential pumping and reduction in background pressure below the present 10−6 …

An ion cooler-buncher for high-sensitivity collinear laser spectroscopy at ISOLDE

International audience; A gas-filled segmented linear Paul trap has been installed at the focal plane of the high-resolution separator (HRS) at CERN-ISOLDE. As well as providing beams with a reduced transverse emittance, this device is also able to accumulate the ions and release the sample in bunches with a well-defined time structure. This has recently permitted collinear laser spectroscopy with stable and radioactive bunched beams to be demonstrated at ISOLDE. Surface-ionized 39, 44, 46K and 85Rb beams were accelerated to 30keV, mass separated and injected into the trap for subsequent extraction and delivery to the laser setup. The ions were neutralized in a charge exchange cell and exci…

Nuclear Spins and Magnetic Moments ofCu71,73,75: Inversion ofπ2p3/2andπ1f5/2Levels inCu75

We report the first confirmation of the predicted inversion between the pi2p3/2 and pi1f5/2 nuclear states in the nu(g)9/2 midshell. This was achieved at the ISOLDE facility, by using a combination of in-source laser spectroscopy and collinear laser spectroscopy on the ground states of 71,73,75Cu, which measured the nuclear spin and magnetic moments. The obtained values are mu(71Cu)=+2.2747(8)mu(N), mu(73Cu)=+1.7426(8)mu(N), and mu(75Cu)=+1.0062(13)mu(N) corresponding to spins I=3/2 for 71,73Cu and I=5/2 for 75Cu. The results are in fair agreement with large-scale shell-model calculations.

Simple Nuclear Structure inCd111–129from Atomic Isomer Shifts

Isomer shifts have been determined in ^{111-129}Cd by high-resolution laser spectroscopy at CERN-ISOLDE. The corresponding mean square charge-radii changes, from the 1/2^{+} and the 3/2^{+} ground states to the 11/2^{-} isomers, have been found to follow a distinct parabolic dependence as a function of the atomic mass number. Since the isomers have been previously associated with simplicity due to the linear mass dependence of their quadrupole moments, the regularity of the isomer shifts suggests a higher order of symmetry affecting the ground states in addition. A comprehensive description assuming nuclear deformation is found to accurately reproduce the radii differences in conjunction wi…

Ground-state spins and moments of72,74,76,78Ga nuclei

Laser spectroscopy was performed on the ${}^{72,74,76,78}$Ga isotopes at On-Line Isotope Mass Separator (ISOLDE) facility, CERN. Ground-state nuclear spins and moments were extracted from the measured hyperfine spectra. The results are compared to shell-model calculations, which provide a detailed probe of the nuclear wave function. The spin is established from the shape of the hyperfine structure and the parity inferred from a comparison of shell-model calculations with the measured nuclear moments. The ground states of ${}^{76,78}$Ga are both assigned a spin and parity of ${I}^{\ensuremath{\pi}}={2}^{\ensuremath{-}}$, while ${}^{74}$Ga is tentatively assigned as ${I}^{\ensuremath{\pi}}={3…

Proton-neutron pairing correlations in the self-conjugate nucleus 42Sc

Collinear laser spectroscopy of the N=Z=21 self-conjugate nucleus 42Sc has been performed at the JYFL IGISOL IV facility in order to determine the change in nuclear mean-square charge radius between the Iπ=0+ ground state and the Iπ=7+ isomer via the measurement of the 42g,42mSc isomer shift. New multi-configurational Dirac-Fock calculations for the atomic mass shift and field shift factors have enabled a recalibration of the charge radii of the 42−46Sc isotopes which were measured previously. While consistent with the treatment of proton-neutron, proton-proton and neutron-neutron pairing on an equal footing, the reduction in size for the isomer is observed to be of a significantly larger m…

Investigating the large deformation of the 5/2+ isomeric state in Zn73 : An indicator for triaxiality

Nuclear moments, charge radii and spins of the ground and isomeric states in175Yb and177Yb

This paper reports static moments and changes in mean-square charge radii of 175, 177, 177mYb measured using collinear laser spectroscopy at the IGISOL facility. The moments are compared to predictions made using the Nilsson model to determine the purity of the multi-quasiparticle T1/2 = 11.4 s, Iπ = 8− state of 176Yb and the ground state of 177Yb. The ground-state spins of 175, 177Yb and the T1/2 = 6.41 s, E = 331.5 keV isomeric state in 177Yb, have been measured from the hyperfine structure to be 7/2, 9/2 and 1/2 respectively.

The shape transition in the neutron-rich yttrium isotopes and isomers

Abstract Laser spectroscopy has been used to study 86–90,92–102Y and isomeric states of 87–90,93,96,97,98Y. Nuclear charge radii differences, magnetic dipole and electric quadrupole moments have been obtained. Information on the nature of the Z ≈ 40 , N ≈ 60 sudden onset of deformation has been derived from all three parameters. It is seen that with increasing neutron number from the N = 50 shell closure that the nuclear deformation becomes increasingly oblate and increasingly soft. At N = 60 a transition to a strongly deformed rigid prolate shape occurs but prior to this, although the nuclear deformation is increasing with N, a proportionate increase in softness is also observed.

Developments for resonance ionization laser spectroscopy of the heaviest elements at SHIP

Abstract The experimental determination of atomic levels and the first ionization potential of the heaviest elements ( Z ⩾ 100 ) is key to challenge theoretical predictions and to reveal changes in the atomic shell structure. These elements are only artificially produced in complete-fusion evaporation reactions at on-line facilities such as the GSI in Darmstadt at a rate of, at most, a few atoms per second. Hence, highly sensitive spectroscopic methods are required. Laser spectroscopy is one of the most powerful and valuable tools to investigate atomic properties. In combination with a buffer-gas filled stopping cell, the Radiation Detected Resonance Ionization Spectroscopy (RADRIS) techniq…

Ground state properties of manganese isotopes across the N=28 shell closure

Abstract The first optical study of the N = 28 shell closure in manganese is reported. Mean-square charge radii and quadrupole moments, obtained for ground and isomeric states in 50–56 Mn, are extracted using new calculations of atomic factors. The charge radii show a well defined shell closure at the magic number. The behaviour of the charge radii is strikingly different to that of the neutron separation energies where no shell effect can be observed. The nuclear parameters can be successfully described by large scale shell model calculations using the GXPF1A interaction.

Spins and magnetic moments ofMn58,60,62,64ground states and isomers

The odd-odd $^{54,56,58,60,62,64}\mathrm{Mn}$ isotopes ($Z=25$) were studied using bunched-beam collinear laser spectroscopy at ISOLDE, CERN. From the measured hyperfine spectra the spins and magnetic moments of Mn isotopes up to $N=39$ were extracted. The previous tentative ground state spin assignments of $^{58,60,62,64}\mathrm{Mn}$ are now firmly determined to be $I=1$ along with an $I=4$ assignment for the isomeric states in $^{58,60,62}\mathrm{Mn}$. The $I=1$ magnetic moments show a decreasing trend with increasing neutron number while the $I=4$ moments remain quite constant between $N=33$ and $N=37$. The results are compared to large-scale shell-model calculations using the GXPF1A and…

Laser Spectroscopy of Neutron-Rich Tin Isotopes: A Discontinuity in Charge Radii across the N=82 Shell Closure

Physical review letters 122(19), 192502 (2019). doi:10.1103/PhysRevLett.122.192502

From Calcium to Cadmium: Testing the Pairing Functional through Charge Radii Measurements of Cd100−130

Differences in mean-square nuclear charge radii of $^{100--130}\mathrm{Cd}$ are extracted from high-resolution collinear laser spectroscopy of the $5s\text{ }{^{2}S}_{1/2}\ensuremath{\rightarrow}5p\text{ }{^{2}P}_{3/2}$ transition of the ion and from the $5s5p\text{ }{^{3}P}_{2}\ensuremath{\rightarrow}5s6s\text{ }{^{3}S}_{1}$ transition in atomic Cd. The radii show a smooth parabolic behavior on top of a linear trend and a regular odd-even staggering across the almost complete $sdgh$ shell. They serve as a first test for a recently established new Fayans functional and show a remarkably good agreement in the trend as well as in the total nuclear charge radius.

Nuclear spin determination of100mY by collinear laser spectroscopy of optically pumped ions

The nuclear spin of the τ1/2 = 0.94 s isomer in 100Y has been determined by collinear laser spectroscopy of optically pumped yttrium fission fragments at the IGISOL facility, JYFL. The isotopes 96, 98, 99, 100Y were produced by the proton-induced fission of natural uranium, and studied on the 4d5s 3D2 (1045 cm−1) → 4d5p 3P1 (32 124 cm−1) transition at 321.67 nm. Enhancement of the population of the metastable 3D2 level was achieved by optically pumping the ground state population via the 5s2 1S0 → 4d5p 1P1 transition at 363.31 nm while the ions were stored in a linear Paul trap. These data, when combined with previous spectroscopic results, give sufficient information for the nuclear spin o…

Laser spectroscopy of niobium fission fragments: first use of optical pumping in an ion beam cooler buncher.

A new method of optical pumping in an ion beam cooler buncher has been developed to selectively enhance ionic metastable state populations. The technique permits the study of elements previously inaccessible to laser spectroscopy and has been applied here to the study of Nb. Model independent mean-square charge radii and nuclear moments have been studied for $^{90,90\text{ }\mathrm{m},91,91\text{ }\mathrm{m},92,93,99,101,103}\mathrm{Nb}$ to cover the region of the $N=50$ shell closure and $N\ensuremath{\approx}60$ sudden onset of deformation. The increase in mean-square charge radius is observed to be less than that for Y, with a substantial degree of $\ensuremath{\beta}$ softness observed …

Isotope shifts from collinear laser spectroscopy of doubly charged yttrium isotopes

Collinear laser spectroscopy has been performed on doubly charged ions of radioactive yttrium in order to study the isotope shifts of the 294.6-nm $5s\phantom{\rule{0.16em}{0ex}}^{2}S_{1/2}\ensuremath{\rightarrow}5p\phantom{\rule{0.16em}{0ex}}^{2}P_{1/2}$ line. The potential of such an alkali-metal-like transition to improve the reliability of atomic-field-shift and mass-shift factor calculations, and hence the extraction of nuclear mean-square radii, is discussed. Production of yttrium ion beams for such studies is available at the IGISOL IV Accelerator Laboratory, Jyv\"askyl\"a, Finland. This newly recommissioned facility is described here in relation to the on-line study of accelerator-p…

High-resolution laser spectroscopy of Al27-32

Hyperfine spectra of Al27-32 (Z=13) have been measured at the ISOLDE-CERN facility via collinear laser spectroscopy using the 3s23p2P3/2o→3s24s2S1/2 atomic transition. For the first time, mean-square charge radii of radioactive aluminum isotopes have been determined alongside the previously unknown magnetic dipole moment of Al29 and electric quadrupole moments of Al29,30. A potentially reduced charge radius at N=19 may suggest an effect of the N=20 shell closure, which is visible in the Al chain, contrary to other isotopic chains in the sd shell. The experimental results are compared with theoretical calculations in the framework of the valence-space in-medium similarity renormalization gro…

Atom-at-a-time laser resonance ionization spectroscopy of nobelium

Resonance ionization spectroscopy of nobelium (atomic number 102) reveals its ground-state transition and an upper limit for its ionization potential, paving the way to characterizing even heavier elements via optical spectroscopy. Characterizing the heaviest elements in the periodic table is a gruelling task because they are radioactive, exist only for split seconds at a time and need to be artificially produced in sufficient quantities by complicated procedures. The heaviest element that has been characterized by optical spectroscopy is fermium, which has an atomic number of 100. Mustapha Laatiaoui et al. extend the methods used for fermium to perform optical spectroscopy on nobelium (ato…

Precision Measurement of the First Ionization Potential of Nobelium

One of the most important atomic properties governing an element's chemical behavior is the energy required to remove its least-bound electron, referred to as the first ionization potential. For the heaviest elements, this fundamental quantity is strongly influenced by relativistic effects which lead to unique chemical properties. Laser spectroscopy on an atom-at-a-time scale was developed and applied to probe the optical spectrum of neutral nobelium near the ionization threshold. The first ionization potential of nobelium is determined here with a very high precision from the convergence of measured Rydberg series to be 6.626 21±0.000 05  eV. This work provides a stringent benchmark for st…

Quadrupole moments of odd-A 53−63Mn: Onset of collectivity towards N=40

Physics letters / B 760, 387 - 392 (2016). doi:10.1016/j.physletb.2016.07.016

A new off-line ion source facility at IGISOL

An off-line ion source station has been commissioned at the IGISOL (Ion Guide Isotope Separator On-Line) facility. It offers the infrastructure needed to produce stable ion beams from three off-line ion sources in parallel with the radioactive ion beams produced from the IGISOL target chamber. This has resulted in improved feasibility for new experiments by offering reference ions for Penning-trap mass measurements, laser spectroscopy and atom trap experiments.

On the decrease in charge radii of multi-quasi particle isomers

Abstract We report changes in mean-square charge radii, δ 〈 r 2 〉 , magnetic moments and quadrupole moments for three multi-quasi particle isomers; 97m2Y, 176mYb and 178m1Hf. All the isomers are observed to display a decrease in 〈 r 2 〉 compared to the lower-lying nuclear state on which the isomer is built. The decreases in 〈 r 2 〉 occur despite the isomers showing increases in quadrupole moment. Possible mechanisms for the effect, which is now seen for six multi-quasi particle isomers, are discussed.

Magnetic and quadrupole moments of neutron deficient 58-62Cu isotopes

Abstract This paper reports on the ground state nuclear moments measured in 58–62Cu using collinear laser spectroscopy at the ISOLDE facility. The quadrupole moments for 58–60Cu have been measured for the first time as Q ( Cu 58 ) = − 15 ( 3 ) efm 2 , Q ( Cu 59 ) = − 19.3 ( 19 ) efm 2 , Q ( Cu 60 ) = + 11.6 ( 12 ) efm 2 and with higher precision for 61,62Cu as Q ( Cu 61 ) = − 21.1 ( 10 ) efm 2 , Q ( Cu 62 ) = − 2.2 ( 4 ) efm 2 . The magnetic moments of 58,59Cu are measured with a higher precision as μ ( Cu 58 ) = + 0.570 ( 2 ) μ N and μ ( Cu 59 ) = + 1.8910 ( 9 ) μ N . The experimental nuclear moments are compared to large-scale shell-model calculations with the GXPF1 and GXPF1A effective i…

High-resolution laser spectroscopy of long-lived plutonium isotopes

Long-lived isotopes of plutonium were studied using two complementary techniques, high-resolution resonance ionisation spectroscopy (HR-RIS) and collinear laser spectroscopy (CLS). Isotope shifts have been measured on the $5f^67s^2\ ^7F_0 \rightarrow 5f^56d^27s\ (J=1)$ and $5f^67s^2\ ^7F_1 \rightarrow 5f^67s7p\ (J=2)$ atomic transitions using the HR-RIS method and the hyperfine factors have been extracted for the odd mass nuclei $^{239,241}$Pu. Collinear laser spectroscopy was performed on the $5f^67s\ ^8F_{1/2} \rightarrow J=1/2\; (27523.61\text{cm}^{-1})$ ionic transition with the hyperfine $A$ factors measured for $^{239}$Pu. Changes in mean-squared charge radii have been extracted and s…

Changes in nuclear structure along the Mn isotopic chain studied via charge radii

The hyperfine spectra of $^{51,53-64}$Mn were measured in two experimental runs using collinear laser spectroscopy at ISOLDE, CERN. Laser spectroscopy was performed on the atomic $3d^5\ 4s^2\ ^{6}\text{S}_{5/2}\rightarrow 3d^5\ 4s4p\ ^{6}\text{P}_{3/2}$ and ionic $3d^5\ 4s\ ^{5}\text{S}_2 \rightarrow 3d^5\ 4p\ ^{5}\text{P}_3$ transitions, yielding two sets of isotope shifts. The mass and field shift factors for both transitions have been calculated in the multiconfiguration Dirac-Fock framework and were combined with a King plot analysis in order to obtain a consistent set of mean-square charge radii which, together with earlier work on neutron-deficient Mn, allow the study of nuclear struc…

Probing the single-particle behavior above Sn132 via electromagnetic moments of Sb133,134 and N=82 isotones

Magnetic and quadrupole moments of the $7/{2}^{+}$ ground state in $^{133}\mathrm{Sb}$ and the $({7}^{\ensuremath{-}})$ isomer in $^{134}\mathrm{Sb}$ have been measured by collinear laser spectroscopy to investigate the single-particle behavior above the doubly magic nucleus $^{132}\mathrm{Sn}$. The comparison of experimental data of the $7/{2}^{+}$ states in $^{133}\mathrm{Sb}$ and neighboring $N=82$ isotones to shell-model calculations reveals the sensitivity of magnetic moments to the splitting of the spin-orbit partners $\ensuremath{\pi}0{g}_{9/2}$ and $\ensuremath{\pi}0{g}_{7/2}$ across the proton shell closure at $Z=50$. In contrast, quadrupole moments of the $N=82$ isotones are insen…

Development of the CRIS (Collinear Resonant Ionisation Spectroscopy) beam line

The CRIS (Collinear Resonant Ionisation Spectroscopy) beam line is a new experimental set up at the ISOLDE facility at CERN. CRIS is being constructed for highresolution laser spectroscopy measurements on radioactive isotopes. These measurements can be used to extract nuclear properties of isotopes far from stability. The CRIS beam line has been under construction since 2009 and testing of its constituent parts have been performed using stable and radioactive ion beams, in preparation for its first on-line run. This paper will present the current status of the CRIS experiment and highlight results from the recent tests. ispartof: pages:012070-6 ispartof: Journal of Physics: Conference Serie…

Nuclear charge radii of 62−80Zn and their dependence on cross-shell proton excitations

Nuclear charge radii of 62−80Zn have been determined using collinear laser spectroscopy of bunched ion beams at CERN-ISOLDE. The subtle variations of observed charge radii, both within one isotope and along the full range of neutron numbers, are found to be well described in terms of the proton excitations across the Z=28 shell gap, as predicted by large-scale shell model calculations. It comprehensively explains the changes in isomer-to-ground state mean square charge radii of 69−79Zn, the inversion of the odd-even staggering around N=40 and the odd-even staggering systematics of the Zn charge radii. With two protons above Z=28, the observed charge radii of the Zn isotopic chain show a cum…

Experimental determination of anIπ=2−ground state inCu72,74

This article reports on the ground-state spin and moments measured in $^{72,74}\mathrm{Cu}$ using collinear laser spectroscopy at the CERN On-Line Isotope Mass Separator (ISOLDE) facility. From the measured hyperfine coefficients, the nuclear observables $\ensuremath{\mu}$(${}^{72}\mathrm{Cu})=\ensuremath{-}1.3472(10){\ensuremath{\mu}}_{N}$, $\ensuremath{\mu}({}^{74}\mathrm{Cu})=\ensuremath{-}1.068(3){\ensuremath{\mu}}_{N}$, $Q({}^{72}\mathrm{Cu})=+8(2) {\mathrm{efm}}^{2}$, $Q({}^{74}\mathrm{Cu})=+26(3) {\mathrm{efm}}^{2}$, $I({}^{72}\mathrm{Cu})=2$, and $I({}^{74}\mathrm{Cu})=2$ have been determined. Through a comparison of the measured magnetic moments with different models, the negative …

Evidence of a sudden increase in the nuclear size of proton-rich silver-96

Understanding the evolution of the nuclear charge radius is one of the long-standing challenges for nuclear theory. Recently, density functional theory calculations utilizing Fayans functionals have successfully reproduced the charge radii of a variety of exotic isotopes. However, difficulties in the isotope production have hindered testing these models in the immediate region of the nuclear chart below the heaviest self-conjugate doubly-magic nucleus 100Sn, where the near-equal number of protons (Z) and neutrons (N) lead to enhanced neutron-proton pairing. Here, we present an optical excursion into this region by crossing the N = 50 magic neutron number in the silver isotopic chain with th…

Discovery of a long-lived low-lying isomeric state in Ga-80

Collinear laser spectroscopy was performed on the $^{80}\mathrm{Ga}$ isotope at ISOLDE, CERN. A low-lying isomeric state with a half-life much greater than $200$ ms was discovered. The nuclear spins and moments of the ground and isomeric states and the isomer shift are discussed. Probable spins and parities are assigned to both long-lived states (${3}^{\ensuremath{-}}$ and ${6}^{\ensuremath{-}}$) deduced from a comparison of the measured moments to shell-model calculations.

COLLINEAR LASER SPECTROSCOPY ON NEUTRON-RICH Mn ISOTOPES APPROACHING N = 40

We have studied 51,53−64Mn (Z=25) via bunched-beam collinear laser spectroscopy at ISOLDE, CERN. Model-independent information on the ground- and isomeric state spins, as well as their g-factors is obtained from the measured hyperfine spectra. The spins are essential for further establishing the level schemes in the mass region, while the g-factors reveal the changing ground state wave functions in the Mn chain approaching N=40. ispartof: pages:699-702 ispartof: Acta Physica Polonica B vol:46 issue:3 pages:699-702 ispartof: location:Zakopane, Poland status: published

Cu charge radii reveal a weak sub-shell effect at N=40

Collinear laser spectroscopy on Cu58-75 isotopes was performed at the CERN-ISOLDE radioactive ion beam facility. In this paper we report on the isotope shifts obtained from these measurements. State-of-the-art atomic physics calculations have been undertaken in order to determine the changes in mean-square charge radii δ(r2)A,A′ from the observed isotope shifts. A local minimum is observed in these radii differences at N=40, providing evidence for a weak N=40 sub-shell effect. However, comparison of δ(r2)A,A′ with a droplet model prediction including static deformation deduced from the spectroscopic quadrupole moments, points to the persistence of correlations at N=40.

Nuclear charge radii and electromagnetic moments of radioactive scandium isotopes and isomers

International audience; Collinear laser spectroscopy experiments with the Sc + transition 3d4s 3 D 2 → 3d4p 3 F 3 at λ = 363.1 nm were performed on the 42−46 Sc isotopic chain using an ion guide isotope separator with a cooler-buncher. Nuclear magnetic dipole and electric quadrupole moments as well as isotope shifts were determined from the hyperfine structure for five ground states and two isomers. Extensive multi-configurational Dirac-Fock calculations were performed in order to evaluate the specific mass-shift, M SMS, and field-shift, F, parameters which allowed evaluation of the charge radii trend of the Sc isotopic sequence. The charge radii obtained show systematics more like the Ti r…

Recent Advances in On-Line Laser Spectroscopy

At radioactive ion beam facilities, particle accelerators are employed to induce nuclear reactions in order to provide short-lived nuclei for immediate study using a variety of spectroscopic techniques. These exotic isotopes/isomers are formed into a beam of fast ions, which are mass analyzed in-flight during transport to a chosen experimental set-up. As an additional filter, the atomic level structure provides a selective fingerprint, which distinguishes one element from another due to the varying numbers of protons and electrons. This property is exploited in laser ion sources whereby high power, pulsed tuneable laser radiation is used to excite and ionize the atom in order to enhance the…

Nuclear moments and charge radii of neutron-deficient francium isotopes and isomers

Collinear laser fluorescence spectroscopy has been performed on the ground and isomeric states of $^{204,206}\mathrm{Fr}$ in order to determine their spins, nuclear moments, and changes in mean-squared charge radii. A new experimental technique has been developed as part of this work which much enhances the data collection rate while maintaining the high resolution. This has permitted the extension of this study to the two isomeric states in each nucleus. The investigation of nuclear $g$ factors and mean-squared charge radii indicates that the neutron-deficient Fr isotopes lie in a transitional region from spherical towards more collective structures.

Laser assisted decay spectroscopy at the CRIS beam line at ISOLDE

A new collinear resonant ionization spectroscopy (Cris)beam line has recently been installed at Isolde, Cern utilising lasers to combine collinear laser spectroscopy and resonant ionization spectroscopy. The combined technique offers the ability to purify an ion beam that is heavily contaminated with radioactive isobars, including the ground state of an isotope from its isomer, allowing sensitive secondary experiments to be performed. A new programme aiming to use the Cris technique for the separation of nuclear isomeric states for decay spectroscopy will commence in 2011. A decay spectroscopy station, consisting of a rotating wheel implantation system for alpha decay spectroscopy, and thre…

Nuclear spins, magnetic moments, and quadrupole moments of Cu isotopes fromN=28toN=46: Probes for core polarization effects

Measurements of the ground-state nuclear spins and magnetic and quadrupole moments of the copper isotopes from $^{61}\mathrm{Cu}$ up to $^{75}\mathrm{Cu}$ are reported. The experiments were performed at the CERN online isotope mass separator (ISOLDE) facility, using the technique of collinear laser spectroscopy. The trend in the magnetic moments between the $N=28$ and $N=50$ shell closures is reasonably reproduced by large-scale shell-model calculations starting from a $^{56}\mathrm{Ni}$ core. The quadrupole moments reveal a strong polarization of the underlying Ni core when the neutron shell is opened, which is, however, strongly reduced at $N=40$ due to the parity change between the $\mat…

Impact of buffer gas quenching on the $^1S_0$ $\to$ $^1P_1$ ground-state atomic transition in nobelium

International audience; Using the sensitive Radiation Detected Resonance Ionization Spectroscopy (RADRIS) techniquean optical transition in neutral nobelium (No, Z = 102) was identified. A remnant signal when delaying the ionizing laser indicated the influence of a strong buffer gas induced de-excitation of the optically populated level. A subsequent investigation of the chemical homologue, ytterbium (Yb, Z = 70), enabled a detailed study of the atomic levels involved in this process, leading to the development of a rate equation model. This paves the way for characterizing resonance ionization spectroscopy (RIS) schemes used in the studyof nobelium and beyond, where atomic properties are c…

Laser spectroscopy of gallium isotopes beyond N = 50

The installation of an ion-beam cooler-buncher at the ISOLDE, CERN facility has provided increased sensitivity for collinear laser spectroscopy experiments. A migration of single-particle states in gallium and in copper isotopes has been investigated through extensive measurements of ground state and isomeric state hyperfine structures. Lying beyond the N = 50 shell closure, 82Ga is the most exotic nucleus in the region to have been studied by optical methods, and is reported here for the first time. ispartof: pages:012071-6 ispartof: Journal of Physics: Conference Series vol:381 issue:1 pages:012071-6 ispartof: Rutherford Centennial Conference on Nuclear Physics location:Manchester, UK dat…

Charge Radius of the Short-Lived Ni68 and Correlation with the Dipole Polarizability

We present the first laser spectroscopic measurement of the neutron-rich nucleus ^{68}Ni at the N=40 subshell closure and extract its nuclear charge radius. Since this is the only short-lived isotope for which the dipole polarizability α_{D} has been measured, the combination of these observables provides a benchmark for nuclear structure theory. We compare them to novel coupled-cluster calculations based on different chiral two- and three-nucleon interactions, for which a strong correlation between the charge radius and dipole polarizability is observed, similar to the stable nucleus ^{48}Ca. Three-particle-three-hole correlations in coupled-cluster theory substantially improve the descrip…

Collinear laser spectroscopy at ISOLDE: new methods and highlights

Over three and a half decades of collinear laser spectroscopy and the COLLAPS setup have played a major role in the ISOLDE physics programme. Based on a general experimental principle and diverse approaches towards higher sensitivity, it has provided unique access to basic nuclear properties such as spins, magnetic moments and electric quadrupole moments as well as isotopic variations of nuclear mean square charge radii. While previous methods of outstanding sensitivity were restricted to selected chemical elements with special atomic properties or nuclear decay modes, recent developments have yielded a breakthrough in sensitivity for nuclides in wide mass ranges. These developments include…