0000000000204442
AUTHOR
Burkhard Fricke
Hydrogen-like bismuth
Atomic physics at heavy ion storage rings allows to study matter in an extreme ionization state and at very high velocity. The concept of electron cooling yields an ion beam with epithermal temperatures, which is suited for many precision experiments. At the ESR even the heaviest elements can be stored up to the fully stripped charge state. The H-like ions with nuclear spin exhibit a groundstate hfs-splitting in the optical region. This can be used as a probe for QED at high Z and magnetization inside the nucleus. The topics related to cooling of ions and laser spectroscopy in a storage ring are reported and a first result of the 1s hfs in 209Bi82+ is discussed for the relevance in testing …
New access to the magnetic moment distribution in the nucleus by laser spectroscopy of highly charged ions
Abstract The availability of high intensity, high quality beams of highly charged ions has started a new application for laser spectroscopy. High resolution spectroscopy can now be applied to a study of hydrogen-like atomic states in heavy elements. In principal, this will allow a determination of the hyperfine splitting with an accuracy in the 10 −6 -range or better. Presently this exceeds the limits given by the uncertainties of the nuclear quantities, especially the distribution of the nuclear magnetization in the nucleus. Since the new approach can be applied to a family of test cases, it can provide a wide experimental basis for the separation of nuclear and QED effects. This is especi…
Isotope Shift Measurements for Superdeformed Fission Isomeric States
Optical isotope shift measurements have been performed for the ${}^{240,242}{\mathrm{Am}}^{f}$ fission isomers with low target production rates of $10{\mathrm{s}}^{\ensuremath{-}1}$ employing resonance ionization spectroscopy in a buffer gas cell. Isotope shift ratios ${\mathrm{IS}}^{240f,241}/{\mathrm{IS}}^{243,241}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}39.2(8)$ and ${\mathrm{IS}}^{242f,241}/{\mathrm{IS}}^{243,241}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}41.4(8)$ have been measured at the 500.02 nm transition. A difference in the nuclear mean charge radii $\ensuremath{\delta}〈{r}^{2}{〉}_{\mathrm{opt}}^{242f,241}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}5.34(2…
Precision Laser Spectroscopy of the Ground State Hyperfine Splitting of HydrogenlikeBi82+209
The first direct observation of a hyperfine splitting in the optical regime is reported. The wavelength of the $M1$ transition between the $F=4$ and $F=5$ hyperfine levels of the ground state of hydrogenlike $^{209}\mathrm{Bi}^{82+}$ was measured to be ${\ensuremath{\lambda}}_{0}=243.87(4)$ nm by detection of laser induced fluorescence at the heavy-ion storage ring ESR at GSI. In addition, the lifetime of the laser excited $F=5$ sublevel was determined to be ${\ensuremath{\tau}}_{0}=0.351(16)$ ms. The method can be applied to a number of other nuclei and should allow a novel test of QED corrections in the previously unexplored combination of strong magnetic and electric fields in highly cha…
Hyperfine measurements in a storage ring
Starting with a look at the outstanding role of the hydrogen atom in modern physics, this work reviews aspects of an extension of precision spectroscopy to the ground-state hyperfine structure of highly charged hydrogenic ions. In this connection, the preferences of heavy-ion storage rings are outlined and illuminated by the laser-spectroscopic measurement (the first of that kind) of the 1s hyperfine splitting of 209Bi82+, stored in the heavy-ion storage ring at GSI. The experimental results, including the mean lifetime of the upper 1s substate, are compared with the presently available theoretical calculations. The relevance of studying further hydrogenicc ions in the vicinity of the doubl…
Isotope shift and hyperfine structure measurements at the242f Am fission isomer
Istope shift and hyperfine structure measurements have been performed for the242fAm fission isomer with target production rates of only a few per second. The method is based on resonance ionization spectroscopy (RIS) in a buffer gas cell with radioactive decay detection of the ionization process (RADRIS). A relative isotope shift ratioX exp=IS242f,241/ IS243,241=41.7±0.9 has been measured for the 500.02 nm transition corresponding to a nuclear parameter Λ242f,241=5.4±0.3 fm2. The analysis of the quadrupole moment based on the deformed Fermi-model of the nuclear charge distribution including second order corrections results inQ 20=38.2 ±1.4( −0.8 +0.4 )model eb. The measurement of the hyperf…
Intermetallic compounds of the heaviest elements: the electronic structure and bonding of dimers of element 112 and its homolog Hg
Abstract Fully relativistic (four-component) density-functional calculations were performed for the element 112 dimers (112)X (X = Pd, Cu, Ag and Au) and those of its lighter homolog, Hg. A relatively small decrease of about 15–20 kJ/mol in bonding was found from the HgX to (112)X compounds. Respectively, the bond lengths were increased by 0.06 A on the average. The Mulliken population analysis has shown this effect to be a result of a decreasing contribution of the relativistically stabilized 7s-AO of element 112 to bonding. The following trend in the binding energies was predicted for (112)X as a function of X: Pd >Cu>Au>Ag, exactly as the trend obtained experimentally for adsorption of H…