0000000001309953

AUTHOR

Nayana Joseph

showing 8 related works from this author

An exclusive approach to 3,4-disubstituted cyclopentenes and alkylidene cyclopentenes via the palladium catalyzed ring opening of azabicyclic olefins…

2013

A simple and efficient method for the stereoselective ring opening of bicyclic hydrazines with various aryl halides under palladium catalysis has been elaborated. The reactions afforded trans-3,4-disubstituted cyclopentenes or alkylidene cyclopentenes in good to excellent yields. By taking advantage of multiple points of functionalization in the synthesized trans-3-phenyl-4-hydrazino-cyclopentene, we have synthesized the antidepressant Cypenamine (trans-2-phenylcyclopentylamine).

Bicyclic moleculeChemistryGeneral Chemical EngineeringArylchemistry.chemical_elementHalideGeneral ChemistryRing (chemistry)Medicinal chemistryCatalysischemistry.chemical_compoundReagentOrganic chemistryStereoselectivityta116PalladiumRSC Advances
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An easy access to fused chromanones via rhodium catalyzed oxidative coupling of salicylaldehydes with heterobicyclic olefins

2016

Abstract Herein we describe a detailed study on the rhodium catalyzed oxidative coupling of salicylaldehydes with heterobicyclic olefins such as diazabicyclic olefins and urea-derived bicyclic olefins. The developed method provides an ideal route to fused chromanone systems in a single synthetic step. Moreover, the scope of this methodology was extended to different oxa/aza-bridged bicyclic urea derivatives.

diazabicyclic olefinsBicyclic moleculechromanone010405 organic chemistryOrganic Chemistrychemistry.chemical_elementrhodium catalyzedsalicylaldehyde010402 general chemistry01 natural sciencesBiochemistry0104 chemical sciencesRhodiumCatalysischemistry.chemical_compoundchemistrySalicylaldehydeDrug DiscoveryOrganic chemistryOxidative coupling of methaneUrea derivativesta116urea derived bicyclic olefinsTetrahedron
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Rhodium catalyzed oxidative coupling of salicylaldehydes with diazabicyclic olefins: a one pot strategy involving aldehyde C–H cleavage and π-allyl c…

2013

An efficient one pot strategy for the synthesis of cyclopentene fused chromanone derivatives through the direct oxidative coupling of salicylaldehydes with bicyclic olefins in the presence of a rhodium-copper catalyst system is described. This is the first report on the ring opening-ring closing of bicyclic hydrazines via metal catalyzed oxidative coupling reaction.

chemistry.chemical_elementAlkenesRing (chemistry)Medicinal chemistryAldehydeCatalysisCatalysisRhodiumchemistry.chemical_compoundMaterials ChemistryOrganic chemistryMoleculeCyclopenteneRhodiumta116chemistry.chemical_classificationAldehydesAza CompoundsMolecular StructureOxidative CouplingBicyclic moleculeMetals and AlloysGeneral ChemistrySurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialschemistryChromonesCyclizationCeramics and CompositesOxidative coupling of methaneChemical Communications
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ChemInform Abstract: Rhodium Catalyzed Oxidative Coupling of Salicylaldehydes with Diazabicyclic Olefins: A One-Pot Strategy Involving Aldehyde C-H C…

2013

The title reaction involves the first example of ring opening and ring closing of bicyclic hydrazines (I) via metal catalyzed oxidative coupling reaction.

chemistry.chemical_classificationBicyclic moleculechemistry.chemical_elementGeneral MedicineRing (chemistry)Cleavage (embryo)Medicinal chemistryAldehydeRhodiumCatalysisMetalchemistryvisual_artvisual_art.visual_art_mediumOxidative coupling of methaneChemInform
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ChemInform Abstract: An Easy Access to Fused Chromanones via Rhodium Catalyzed Oxidative Coupling of Salicylaldehydes with Heterobicyclic Olefins.

2016

Diazabicyclic and urea-derived bicyclic olefins react with salicylaldehydes to produce various types of fused chromanone systems of biological interest in a single step (mechanism).

Bicyclic moleculeChemistrychemistry.chemical_elementOxidative coupling of methaneSingle stepGeneral MedicineCombinatorial chemistryCatalysisRhodiumChemInform
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An easy access to fused chromanones via rhodium catalyzed oxidative coupling of salicylaldehydes with heterobicyclic olefins

2016

Herein we describe a detailed study on the rhodium catalyzed oxidative coupling of salicylaldehydes with heterobicyclic olefins such as diazabicyclic olefins and urea-derived bicyclic olefins. The developed method provides an ideal route to fused chromanone systems in a single synthetic step. Moreover, the scope of this methodology was extended to different oxa/aza-bridged bicyclic urea derivatives. peerReviewed

diazabicyclic olefinschromanonerhodium catalyzedsalicylaldehydeurea derived bicyclic olefins
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CCDC 1449575: Experimental Crystal Structure Determination

2016

Related Article: Ajesh Vijayan, T.V. Baiju, E. Jijy, Praveen Prakash, M. Shimi, Nayana Joseph, Petri M. Pihko, Sunil Varughese, K.V. Radhakrishnan|2016|Tetrahedron|72|4007|doi:10.1016/j.tet.2016.05.031

Space GroupCrystallographyCrystal SystemCrystal StructureCell Parameterst-butyl 1315-bis(benzyloxy)-1014-dioxo-3-oxa-131516-triazatetracyclo[10.3.1.0211.049]hexadeca-468-triene-16-carboxylateExperimental 3D Coordinates
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CCDC 782677: Experimental Crystal Structure Determination

2013

Related Article: Nayana Joseph,Rani Rajan,Jubi John,N. V. Devika,S. Sarath Chand,E. Suresh,Petri M. Pihko,K. V. Radhakrishnan|2013|RSC Advances|3|7751|doi:10.1039/c3ra41504j

Space GroupCrystallographyCrystal SystemCrystal StructureCell ParametersDi-isopropyl 1-(2-(2-aminophenyl)cyclopent-3-en-1-yl)hydrazine-12-dicarboxylateExperimental 3D Coordinates
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