6533b822fe1ef96bd127cc67

RESEARCH PRODUCT

Evaluating plasmonic transport in current-carrying silver nanowires

Laurent MarkeyArnaud StolzErik DujardinMingxia SongAlexandre BouhelierDouguo ZhangJuan ArocasGérard Colas Des Francs

subject

Optics and PhotonicsSilverMaterials scienceGeneral Chemical EngineeringNanowireMetal Nanoparticles02 engineering and technology010402 general chemistry[ CHIM ] Chemical Sciences01 natural sciencesGeneral Biochemistry Genetics and Molecular Biology[CHIM]Chemical SciencesSurface plasmon resonancePlasmonGeneral Immunology and MicrobiologyNanowiresbusiness.industryPhysicsGeneral NeuroscienceSurface plasmonElectric ConductivityPlasmonic CircuitrySurface Plasmon Resonance021001 nanoscience & nanotechnology0104 chemical sciencesNanolithographyResistOptoelectronics0210 nano-technologybusinessLocalized surface plasmon

description

cited By 1; International audience; Plasmonics is an emerging technology capable of simultaneously transporting a plasmonic signal and an electronic signal on the same information support1,2,3. In this context, metal nanowires are especially desirable for realizing dense routing networks4. A prerequisite to operate such shared nanowire-based platform relies on our ability to electrically contact individual metal nanowires and efficiently excite surface plasmon polaritons5 in this information support. In this article, we describe a protocol to bring electrical terminals to chemically-synthesized silver nanowires6 randomly distributed on a glass substrate7. The positions of the nanowire ends with respect to predefined landmarks are precisely located using standard optical transmission microscopy before encapsulation in an electron-sensitive resist. Trenches representing the electrode layout are subsequently designed by electron-beam lithography. Metal electrodes are then fabricated by thermally evaporating a Cr/Au layer followed by a chemical lift-off. The contacted silver nanowires are finally transferred to a leakage radiation microscope for surface plasmon excitation and characterization8,9. Surface plasmons are launched in the nanowires by focusing a near infrared laser beam on a diffraction-limited spot overlapping one nanowire extremity5,9. For sufficiently large nanowires, the surface plasmon mode leaks into the glass substrate9,10. This leakage radiation is readily detected, imaged, and analyzed in the different conjugate planes in leakage radiation microscopy9,11. The electrical terminals do not affect the plasmon propagation. However, a current-induced morphological deterioration of the nanowire drastically degrades the flow of surface plasmons. The combination of surface plasmon leakage radiation microscopy with a simultaneous analysis of the nanowire electrical transport characteristics reveals the intrinsic limitations of such plasmonic circuitry.

https://hal.archives-ouvertes.fr/hal-01798018