Long-range magnetic order in the porous metal–organic framework Ni(pyrazine)[Pt(CN)4]

6533b82ffe1ef96bd1295377

RESEARCH PRODUCT

Long-range magnetic order in the porous metal–organic framework Ni(pyrazine)[Pt(CN)4]

J. Alberto Rodríguez-velamazán José Antonio Real Miguel A. Gonzalez Roberta Poloni E. Lhotel Olivier Roubeau Elias Palacios

subject

Range (particle radiation)Pyrazine Chemistry Magnetic order Inorganic chemistry General Physics and Astronomy 02 engineering and technology Neutron scattering 010402 general chemistry 021001 nanoscience & nanotechnology 01 natural sciences Heat capacity 0104 chemical sciences chemistry.chemical_compound Crystallography Antiferromagnetism Condensed Matter::Strongly Correlated Electrons [PHYS.COND.CM-SCE]Physics [physics]/Condensed Matter [cond-mat]/Strongly Correlated Electrons [cond-mat.str-el]Physical and Theoretical Chemistry 0210 nano-technology Spin (physics)Porosity ComputingMilieux_MISCELLANEOUS

description

A combined study involving DFT calculations, neutron scattering, heat capacity and magnetic measurements at very low temperatures demonstrates the long-range magnetic ordering of Ni(pyrazine)[Pt(CN)4] below 1.9 K, describing its antiferromagnetic spin arrangement. This compound belongs to the family of porous coordination polymers M(pyrazine)[Pt(CN)4] (M = divalent metal), renowned for showing interesting combinations of porosity and magnetic properties. The possibility of including long-range magnetic ordering, one of the most pursued functional properties, opens new perspectives for the multifunctionality of this class of compounds.

year	journal	country	edition	language
2017-01-01	Physical Chemistry Chemical Physics

https://doi.org/10.1039/c7cp06310e

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