6533b85afe1ef96bd12b9634

RESEARCH PRODUCT

Removing krypton from xenon by cryogenic distillation to the ppq level

E. AprileJ. AalbersF. AgostiniM. AlfonsiF. D. AmaroM. AnthonyF. ArneodoP. BarrowL. BaudisB. BauermeisterM. L. BenabderrahmaneT. BergerP. A. BreurA. BrownE. BrownS. BruennerG. BrunoR BudnikL. BütikoferJ. CalvénJ. M. R. CardosoM. CervantesD. CichonD. CoderreA. P. ColijnJ. ConradJ. P. CussonneauM. P. DecowskiP. PerioP. Di GangiA. Di GiovanniS. DiglioE. DuchovniG. EurinJ. FeiA. D. FerellaA. FieguthD. FrancoW. FulgioneAndrea Gallo RossoM. GallowayF. GaoM. GarbiniC. GeisL. W. GoetzkeL. GrandiZ. GreeneC. GrignonC. HasterokE. HogenbirkC. HuhmannR. ItayB. KaminskyG. KesslerA. KishH. LandsmanR. F. LangD. LellouchL. LevinsonM. Le CallochQ. LinS. LindemannM. LindnerJ. A. M. LopesA. ManfrediniI. MarisT. Marrodán UndagoitiaJ. MasbouF. V. MassoliD. MassonD. MayaniY. MengM. MessinaK. MicheneauB. MiguezA. MolinarioM. MurraJ. NaganomaK. NiU. OberlackS. E. A. OrrigoP. PakarhaB. PelssersR. PersianiF. PiastraJ. PienaarM. -C PiroV. PizzellaG. PlanteN. PrielL. RauchS. ReichardC. ReuterA. RizzoS. RosendahlN. RuppR. SaldanhaJ. M. F. Dos SantosG. SartorelliM. ScheibelhutS. SchindlerJ. SchreinerM. SchumannL. Scotto LavinaM. SelviP. ShaginE. ShockleyM. SilvaH. SimgenM. V. SiversA. SteinD. ThersA. TiseniG. TrincheroC. TunnellN. UpoleH. WangY. WeiC. WeinheimerJ. WulfJ. YeY. ZhangI. CristescuCollaboration Xenon

subject

CryostatPhysics - Instrumentation and DetectorsXenonPhysics and Astronomy (miscellaneous)WIMPDark matterAnalytical chemistryFOS: Physical scienceschemistry.chemical_elementlcsh:AstrophysicsWeakly Interact Massive ParticleSciences de l'ingénieur01 natural sciences7. Clean energyXenonlcsh:QB460-4660103 physical sciencesDark Matterlcsh:Nuclear and particle physics. Atomic energy. RadioactivitySensitivity (control systems)[PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det]010306 general physicsComputer science information & general worksEngineering (miscellaneous)Liquid XenonComputingMilieux_MISCELLANEOUSPhysicsAir separationPhysique010308 nuclear & particles physicsDistillation ColumnKryptonKryptonOrder (ring theory)Instrumentation and Detectors (physics.ins-det)AstronomiechemistryDirect Searchddc:000lcsh:QC770-798TPCOrder of magnitude

description

The XENON1T experiment aims for the direct detection of dark matter in a detector filled with 3.3 tons of liquid xenon. In order to achieve the desired sensitivity, the background induced by radioactive decays inside the detector has to be sufficiently low. One major contributor is the β-emitter 85Kr which is present in the xenon. For XENON1T a concentration of natural krypton in xenon natKr/Xe<200ppq (parts per quadrillion, 1ppq=10-15mol/mol) is required. In this work, the design, construction and test of a novel cryogenic distillation column using the common McCabe–Thiele approach is described. The system demonstrated a krypton reduction factor of 6.4 · 10 5 with thermodynamic stability at process speeds above 3 kg/h. The resulting concentration of natKr/Xe<26ppq is the lowest ever achieved, almost one order of magnitude below the requirements for XENON1T and even sufficient for future dark matter experiments using liquid xenon, such as XENONnT and DARWIN.

10.1140/epjc/s10052-017-4757-1http://hal.in2p3.fr/in2p3-01439234