Search results for " Silicate"

showing 10 items of 126 documents

Neptunium(V) Sorption and Diffusion in Opalinus Clay

2009

The sorption and diffusion behavior of 8 x 10(-6) M Np(V) in Opalinus Clay (OPA) with synthetic pore water (pH 7.6) as mobile phase was studied under ambient conditions by batch and diffusion experiments, respectively. The Kd value determined by batch experiments with OPA suspensions is equal to 0.025 +/- 0.005 m3/kg. The diffusion-accessible porosity epsilon of intact OPA as determined by through- and out-diffusion experiments with tritiated water (HTO) is equal to 0.15 +/- 0.01. The diffusion coefficient De and the rock capacity factor alpha of 22Na+ in OPA were measured by through-, out-, and in-diffusion experiments and asserted the reliability of these diffusion techniques. For the dif…

Tritiated waterNeptuniumDiffusionchemistry.chemical_elementSorptionGeneral ChemistryModels TheoreticalThermal diffusivityCapacity factorDiffusionNeptuniumchemistry.chemical_compoundWaste ManagementchemistryRadioactive WastePhase (matter)ClayEnvironmental ChemistryAluminum SilicatesPorosityPorositySwitzerlandNuclear chemistryEnvironmental Science & Technology
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Fabrication and characterization of barium silicate ultrathin films as an alternative gate oxide

2008

Down-scaling of elementary CMOS elements requires the replacement of SiO2 as a gate oxide. By the identification of the formation conditions of barium silicate in direct contact of a silicon substrate, this study revealed a potential candidate. First of all, a reaction between Ba and SiO2 leading to the formation of barium silicate as been evidenced by in-situ XPS and SR-PES analyses. Then, barium silicate films have been elaborated by oxygen and barium co-deposition at 580 °C. Thermal treatments under vacuum showed that barium silicate was thermally stable up to 900 °C. TEM and SIMS ex-situ analyses revealed a sharp interface with the substrate. Finally, an experimental setup dedicated to …

[CHIM.MATE] Chemical Sciences/Material chemistrysilicate de baryuminterfacial reactivity[ CHIM.MATE ] Chemical Sciences/Material chemistrybarium silicateXPS[CHIM.MATE]Chemical Sciences/Material chemistry[PHYS.COND]Physics [physics]/Condensed Matter [cond-mat]SR-PESréactivité interfaciale[PHYS.COND] Physics [physics]/Condensed Matter [cond-mat]high-k[ PHYS.COND ] Physics [physics]/Condensed Matter [cond-mat]
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Study of parameters endogeneous and exogeneous to ordinary Portland ciment influencing hydration of its main phase : tricalcium silicate

2012

This work devoted to study various parameters influencing hydration of silicate phase main Ordinary Portland Cement (OPC) was performed at the Laboratoire Interdisciplinaire Carnot de Bourgogne (ICB). This study is part of the project "Crystal Growth Control" initiated by BASF in order to monitor and provide the best as possible the hydration of Ordinary Portland Cement. The dissolution of alite, like the pure C3S one, is fast in pure water. Speed decreases with deviation from equilibrium and the concentration of aluminates ions in solution. There is also an adsorption on the surface of the aluminum which is into the alite and released by dissolution. Germination and growth of C-S-H has bee…

[SPI.OTHER]Engineering Sciences [physics]/OtherInorganic saltsOrdinary Portland cement[ SPI.OTHER ] Engineering Sciences [physics]/OtherSilicate tricalcique[SPI.OTHER] Engineering Sciences [physics]/OtherHydratationTricalcium silicateHydrationCiment Portland OrdinaireCinétiqueKineticsSels inorganiquesAlite[CHIM.OTHE] Chemical Sciences/Other[ CHIM.OTHE ] Chemical Sciences/OtherCroissance C-S-HC-S-H GrowthAluminium[CHIM.OTHE]Chemical Sciences/OtherDissolution
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Uptake of actinides by calcium silicate hydrate (C-S-H) phases

2018

Abstract The sorption of actinides (Th, U – Am) was studied in dependence of the solid-to-liquid (S/L) ratio (0.5–20.0 g/L) and the calcium-to-silicon (C:S) ratio. The C:S ratio was varied between 1.80 and 0.70 to simulate the changing composition of the C-S-H phases during cement degradation from high to low C:S ratios. The decrease of the calcium content in the C-S-H phases by time is accompanied by a decrease in pH in the corresponding suspensions from 12.6 to 10.2. X-ray photoelectron spectroscopy (XPS) of the C-S-H phases showed an increasing depletion of Ca on the surface with increasing C:S ratio in comparison to the composition of the solid phase as a whole. The sorption experiments…

cementTechnology02 engineering and technology010501 environmental sciences01 natural sciencesRedoxAmchemistry.chemical_compoundX-ray photoelectron spectroscopyGeochemistry and PetrologyOxidation statePhase (matter)Environmental ChemistryThCalcium silicate hydrateSpectroscopy0105 earth and related environmental sciencesUactinideshigh-energy resolution X-ray absorption near-edge structure (HR-XANES)SorptionX-ray photoelectron spectroscopy (XPS)Pu021001 nanoscience & nanotechnologyPollutionNpC-S-Hchemistryradioactive wasteSorptionAbsorption (chemistry)0210 nano-technologyddc:600Nuclear chemistry
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Biogeochemical Cycle of Silica in an Apolyhaline Interdunal Holocene Lake (Chad, N'Guigmi Region, Niger)

1999

During the Holocene, the apolyhaline conditions in interdunal ephemeral lakes in the Lake Chad region led to various diagenetic processes, which resulted in: (a) clay authigenesis, (b) organic matter lithification (plants and cyanobacterial mats), (c) precipitation of sodium silicate (magadiite, kenyaite, zeolite), and (d) chert neoformation. Each step in this diagenetic process involves silica, which can be highly mobile under such conditions. Therefore, the paleoenvironmental variations can be investigated using the Si cycle.http://link.springer. de/link/service/journals/00114/bibs/9086010/90860475.htm</HEA

chemistry.chemical_classificationBiogeochemical cycleEcologyEphemeral keyGeochemistrySodium silicateGeneral MedicineDiagenesischemistry.chemical_compoundchemistryOrganic matterPrecipitationLithificationEcology Evolution Behavior and SystematicsHoloceneGeologyNaturwissenschaften
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Different kinds of solid solutions in the V2O5-ZrSiO4-NaF system by sol-gel processes and their characterization

1993

Abstract In the V2O5-ZrSiO4-NaF system, three kinds of substances have been identified by sol-gel methods depending on the V2O5 amounts in the composition. Their characterization by X-ray diffraction, measurements of unit cell parameters, UV-visible (UV-V) spectroscopy, differential thermal analysis and lab colour parameter determination allow the consideration of three kinds of solid solution in the zircon lattice: (a) V+5,V+4-ZrSiO4, thermally stable and with a deep green colour; (b) V+4-ZrSiO4, thermally stable and blue coloured, made by the sol-gel method and with V2O5 amounts lower than 0·03 mol per formula weight; and (c) Na+,F−,V+4-ZrSiO4, a solid solution with a deep blue-turquoise …

chemistry.chemical_classificationMaterials scienceMolar massInorganic chemistryAnalytical chemistrychemistry.chemical_compoundchemistryDifferential thermal analysisZirconium(IV) silicateX-ray crystallographyMaterials ChemistryCeramics and CompositesQualitative inorganic analysisChemical compositionInorganic compoundSolid solutionJournal of the European Ceramic Society
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Computer simulations of undercooled fluids and the glass transition

2000

Abstract Two model studies are presented that attempt to describe the static and dynamic properties of glass-forming fluids via molecular dynamics simulations: The first model is an atomistically realistic model of SiO 2 , the second model provides a coarse-grained description of polymer liquids, i.e., typical `fragile' glassformers, while SiO 2 is the prototype of a `strong glassformer'. For both models, attention is given to the questions as to which range of temperatures are properties in equilibrium, and whether such simulations can help to interpret experiments and/or check theoretical predictions. While in the simulation of SiO 2 using the potential of van Beest, Kramer and van Santen…

chemistry.chemical_classificationThermodynamicsSodium silicatePolymerAtmospheric temperature rangeCondensed Matter PhysicsElectronic Optical and Magnetic Materialschemistry.chemical_compoundMolecular dynamicsMonomerchemistryMaterials ChemistryCeramics and CompositesGlass transitionPolymer meltMacromoleculeJournal of Non-Crystalline Solids
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PLASMOGENY, A NEW SCIENCE OF THE ORIGIN OF LIFE

2014

The Church has always hampered the progress of Mankind so as to retain its hold over awareness, which is the basis of secular exploitation of the people.

chemistry.chemical_compoundchemistryAbiogenesisColloidal silicaInorganic chemistrySodium silicatePotassium silicatePotassium chromate
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Comparative Surface Morphology, Chemical Composition, and Cytocompatibility of Bio-C Repair, Biodentine, and ProRoot MTA on hDPCs

2020

Biocompatibility is an essential property for any vital pulp material that may interact with the dental pulp tissues. Accordingly, this study aimed to compare the chemical composition and ultrastructural morphology of Biodentine (Septodont, Saint Maur-des-Fosses, France), ProRoot MTA (Dentsply Tulsa Dental Specialties, Johnson City, TN, USA), and Bio-C Repair (Angelus, Londrina, PR, Brazil), as well as their biological effects on human dental pulp cells. Chemical element characterization of the materials was undertaken using scanning electron microscopy and energy dispersive X-ray analysis (SEM-EDX). The cytotoxicity was assessed by analyzing the cell viability (MTT assay), cell morphology …

cytocompatibilityBiocompatibilityvital pulp materialschemistry.chemical_element02 engineering and technologyCalciumCell morphologylcsh:TechnologyArticleFlow cytometry03 medical and health sciences0302 clinical medicinestomatognathic systemdental pulp cellsmedicineGeneral Materials ScienceMTT assayViability assaycalcium silicate materialsCytotoxicitylcsh:Microscopylcsh:QC120-168.85calcium silicate materialmedicine.diagnostic_testlcsh:QH201-278.5Chemistrylcsh:Tdental pulp cell030206 dentistry021001 nanoscience & nanotechnologystomatognathic diseasesendodonticlcsh:TA1-2040Pulp (tooth)lcsh:Descriptive and experimental mechanicslcsh:Electrical engineering. Electronics. Nuclear engineering0210 nano-technologylcsh:Engineering (General). Civil engineering (General)lcsh:TK1-9971Nuclear chemistryMaterials
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Successful treatment of paraquat poisoning: activated charcoal per os and "continuous hemoperfusion".

1982

AbstractIngestion of paraquat results in an extremely dangerous poisoning. The first aim is to clear the gastrointestinal tract by inducing emesis and performing gastric/gut lavage; as much activated charcoal as possible should be administered per os and as quickly as possible. The best measure to eliminate paraquat from blood and tissue is hemoperfusion with coated activated charcoal; it has to be performed in the sense of “continuous hemoperfusion” about 8 h/d over a period of 2–3 weeks. These measures give a chance to lower the lethality of paraquat poisoning.

inorganic chemicalsMaleParaquatTime FactorsAdolescentHealth Toxicology and Mutagenesismedicine.medical_treatmentMagnesium CompoundsToxicologychemistry.chemical_compoundParaquatMedicineAnimalsHumansAluminum CompoundsKaolinTherapeutic IrrigationGastrointestinal tractbusiness.industrySilicatesRats Inbred StrainsHemoperfusionPARAQUAT POISONINGRatsHemoperfusionchemistryActivated charcoalAnesthesiaCharcoalBentoniteAluminum SilicatesFemaleAdsorptionbusinessJournal of toxicology. Clinical toxicology
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