Search results for "MACROMOLECULAR"

showing 10 items of 944 documents

Polylactic is a Sustainable, Low Absorption, Low Autofluorescence Alternative to Other Plastics for Microfluidic and Organ-on-Chip Applications

2020

Organ-on-chip (OOC) devices are miniaturized devices replacing animal models in drug discovery and toxicology studies. The majority of OOC devices are made from polydimethylsiloxane (PDMS), an elastomer widely used in microfluidic prototyping, but posing a number of challenges to experimentalists, including leaching of uncured oligomers and uncontrolled absorption of small compounds. Here we assess the suitability of polylactic acid (PLA) as a replacement material to PDMS for microfluidic cell culture and OOC applications. We changed the wettability of PLA substrates and demonstrated the functionalization method to be stable over a time period of at least 9 months. We successfully cultured …

BiocompatibilityPolydimethylsiloxane010401 analytical chemistryMicrofluidicstechnology industry and agricultureSettore ING-IND/34 - Bioingegneria IndustrialeNanotechnologymacromolecular substancesengineering.material010402 general chemistryElastomerSettore ING-INF/0701 natural sciences0104 chemical sciencesAnalytical Chemistrychemistry.chemical_compoundAutofluorescenceCoatingPolylactic acidchemistryBiocompatibility Cell culture Diseases Elastomers Microchannels Microfluidics Polydimethylsiloxane Silicones TransparencyengineeringSurface modificationAnalytical Chemistry
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Characterization and biodistribution of Au nanoparticles loaded in PLGA nanocarriers using an original encapsulation process

2021

Due to their imaging and radiosensitizing properties, ultrasmall gadolinium chelate-coated gold nanoparticles (AuNP) represent a promising approach in the diagnosis and the treatment of tumors. However, their poor pharmacokinetic profile, especially their rapid renal clearance prevents from an efficient exploitation of their potential for medical applications. The present study focuses on a strategy which resides in the encapsulation of AuNP in large polymeric NP to avoid the glomerular filtration and then to prolong the vascular residence time. An original encapsulation procedure using the polyethyleneimine (PEI) was set up to electrostatically entrap AuNP in biodegradable poly(lactic-co-g…

BiodistributionGadoliniumMetal NanoparticlesNanoparticlechemistry.chemical_elementmacromolecular substances02 engineering and technologyPolyethylene glycol01 natural sciencesPolyethylene Glycolschemistry.chemical_compoundColloid and Surface ChemistryPolylactic Acid-Polyglycolic Acid Copolymer0103 physical sciencesAnimalsTissue DistributionParticle SizePhysical and Theoretical ChemistryDrug Carriers010304 chemical physicstechnology industry and agricultureSurfaces and InterfacesGeneral Medicine021001 nanoscience & nanotechnologyRatsEncapsulation (networking)PLGAchemistryColloidal goldBiophysicsNanoparticlesGoldNanocarriers0210 nano-technologyBiotechnologyColloids and Surfaces B: Biointerfaces
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1H-NMR studies on poly(oxyethylene)-bound oligopeptides

1983

Conformational studies on poly(oxyethylene)-bound homo-, oligo-, guest-host, and sequential peptides synthesized according to the liquid-phase method were carried out by means of 1H-nmr spectroscopy. The solubilizing effect of the C-terminal polymeric support allowed a thorough investigation of the secondary structure in solution.

BiomaterialsOligopeptideChemistryOrganic ChemistryBiophysicsProton NMROrganic chemistrymacromolecular substancesGeneral MedicineSpectroscopyBiochemistryProtein secondary structureBiopolymers
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Performance of polyester-based electrospun scaffolds under in vitro hydrolytic conditions: From short-term to long-term applications

2019

The evaluation of the performance of polyesters under in vitro physiologic conditions is essential to design scaffolds with an adequate lifespan for a given application. In this line, the degradation-durability patterns of poly(lactide-co-glycolide) (PLGA), polydioxanone (PDO), polycaprolactone (PCL) and polyhydroxybutyrate (PHB) scaffolds were monitored and compared giving, as a result, a basis for the specific design of scaffolds from short-term to long-term applications. For this purpose, they were immersed in ultra-pure water and phosphate buffer solution (PBS) at 37 &deg

BiopolimersMaterials scienceBiopolymerGeneral Chemical EngineeringPolyestersPHBPolyestermacromolecular substancesMembranes (Biology)engineering.materialArticlelcsh:ChemistryPolyhydroxybutyratePolydioxanonechemistry.chemical_compoundCrystallinity:Enginyeria química [Àrees temàtiques de la UPC]BiopolymersMembranes (Biologia)biopolymerPolièstersPDOGeneral Materials SciencepolyesterTissue engineeringScaffoldsMolar massNanotecnologiaTermoplàsticstechnology industry and agriculturePLGAPolyesterPLGAIn vitro hydrolytic degradationlcsh:QD1-999chemistryChemical engineeringEnginyeria de teixitsPCLscaffoldstissue engineeringPolycaprolactoneengineeringin vitro hydrolytic degradationBiopolymer
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CaCl2, Bisoxazoline, and Malonate: A Protocol for an Asymmetric Michael Reaction

2015

A mild protocol for the asymmetric Michael addition of dimethyl malonate to various α,β-unsaturated carbonyl compounds was developed. The salient feature of this methodology is that a cheap and environmentally friendly Lewis acid, CaCl2, was used as a catalyst. An aminoindanol- and pyridine-derived ligand provided in the presence of CaCl2 Michael adducts in moderate to high enantioselectivities. The scope of the reaction was demonstrated.

Bisoxazolineinorganic chemicalsAminoindanol010405 organic chemistryChemistryLigandOrganic ChemistryMalonateCaCl2macromolecular substances010402 general chemistrybehavioral disciplines and activities01 natural sciencesDimethyl malonatehumanities0104 chemical sciencesCatalysisAdductchemistry.chemical_compoundMalonateMichael reactionOrganic chemistryLewis acids and basesta116The Journal of Organic Chemistry
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Evaluation of Ligno Boost™ softwood kraft lignin epoxidation as an approach for its application in cured epoxy resins

2018

Abstract In this study, modification of LignoBoost™ softwood kraft lignin with epichlorhydrin in water-organic solvents media was realized. Lignin-based epoxy resins were obtained by two ways: acetone extraction of glycidylated lignin or glycidylation of the acetone soluble lignin fraction. The effect of glycidylation regimes on the yields of acetone soluble fractions, their functional composition and physical-chemical characteristics was investigated using wet chemistry methods, FTIR spectroscopy, size exclusion chromatography (SEC) and differential scanning calorimetry (DSC). The positive effect of the biphasic phase transfer catalytic system – KOH/quaternary ammonium salt – on glycidylat…

Bisphenol ASoftwood010405 organic chemistrytechnology industry and agriculturefood and beveragesmacromolecular substances02 engineering and technologyEpoxy021001 nanoscience & nanotechnologycomplex mixtures01 natural sciences0104 chemical scienceschemistry.chemical_compoundVanillyl alcoholDifferential scanning calorimetrychemistryChemical engineeringvisual_artAcetonevisual_art.visual_art_mediumLigninAdhesive0210 nano-technologyAgronomy and Crop ScienceIndustrial Crops and Products
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A biostable, anti-fouling zwitterionic polyurethane-urea based on PDMS for use in blood-contacting medical devices.

2020

Polydimethylsiloxane (PDMS) is commonly used in medical devices because it is non-toxic and stable against oxidative stress. Relatively high blood platelet adhesion and the need for chemical crosslinking through curing, however, limit its utility. In this research, a biostable PDMS-based polyurethane-urea bearing zwitterion sulfobetaine (PDMS-SB-UU) was synthesized for potential use in the fabrication or coating of blood-contacting devices, such as a conduits, artificial lungs, and microfluidic devices. The chemical structure and physical properties of synthesized PDMS-SB-UU were confirmed by (1)H-nuclear magnetic resonance ((1)H-NMR), X-ray diffraction (XRD), and uniaxial stress-strain cur…

Blood PlateletsBiofoulingChemical structurePolyurethanesBiomedical Engineering02 engineering and technologymacromolecular substancesengineering.material010402 general chemistry01 natural sciencesHemolysisArticlechemistry.chemical_compoundPlatelet AdhesivenessCoatingCoated Materials BiocompatiblemedicineAnimalsGeneral Materials ScienceDimethylpolysiloxanesCuring (chemistry)PolyurethaneSheepPolydimethylsiloxaneChemistrytechnology industry and agricultureFibrinogenGeneral ChemistryGeneral Medicine021001 nanoscience & nanotechnologymedicine.diseaseHemolysisElectrospinning0104 chemical sciencesRatsQuaternary Ammonium CompoundsChemical engineeringengineeringUreaAdsorptionSulfonic Acids0210 nano-technologyJournal of materials chemistry. B
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Development and validation of a novel risk score for asthma exacerbations: The risk score for exacerbations.

2015

BACKGROUND: Identifying patients at risk of future severe asthma exacerbations, those whose asthma might be less treatment responsive, or both might guide treatment selection. OBJECTIVE: We sought to investigate predictors for failure to achieve Global Initiative for Asthma (GINA)-defined good current asthma control and severe exacerbations on treatment and to develop a simple risk score for exacerbations (RSE) for clinical use. METHODS: A large data set from 3 studies comparing budesonide/formoterol maintenance and reliever therapy with fixed-dose inhaled corticosteroid/long-acting ?2-agonist therapy was analyzed. Baseline patient characteristics were investigated to determine dominant pre…

BudesonidePediatricsmedicine.medical_specialtyFramingham Risk ScoreMultivariate analysisbusiness.industryRespiratory Medicine and AllergyImmunologymacromolecular substancesmedicine.diseaserespiratory tract diseasesBudesonide/formoterolAsthma Control Questionnaireimmune system diseasesmedicineImmunology and AllergyFormoterolbusinessBody mass indexmedicine.drugAsthma
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Cigarette smoke alters the EZH2/DAB2IP expression in bronchial epithelial cells. A risk factor for lung cancer in COPD patients

2016

Cigarette smoke is an environmental risk factor for COPD and Lung cancer, leading causes of morbidity and mortality worldwide. In cancer, enhancer of zeste homolog 2 (EZH2) silenced disabled homolog 2 interacting protein gene (DAB2IP) (tumor-suppressor gene) bytri-methylation of lysine 27 on histone H3 (H3K27me3). We studied EZH2 and DAB2IP expression in airway epithelial cells from COPD patients and their potential involvement in the progression of COPD toward lung cancer. We assessed EZH2 and DAB2IPimmunoreactivity in bronchial epithelial cells from surgical specimens of COPD patients and healthy control subjects (HC) by immunohistochemistry. Bronchial epithelial cell line (16HBE), primar…

COPDLungbusiness.industryEZH2Cancermacromolecular substancesrespiratory systemmedicine.diseaserespiratory tract diseasesHistone H3medicine.anatomical_structureApoptosisImmunologymedicineCancer researchImmunohistochemistrybusinessLung cancer3.2 Airway Cell Biology and Immunopathology
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A urochordate putative homolog of human EB1, the protein which binds APC1

1996

Abstract The human EB1 protein has been cloned by virtue of its interaction with the C-terminus of the APC (adenomatous polyposis coli) protein, whose C-terminal truncated forms have been shown to accompany sporadic and familial forms of colorectal cancer. We have cloned a putative EB1 homolog from Botryllus schlosseri (Urochordata, Ascidiacea). The deduced protein is 287 amino acids long, and is identical with 48% of the residues in human EB1 and 24–25% in two yeast hypothetical proteins. We propose that such a high degree of conservation among EB1 homologs is indicative of an essential regulatory mechanism in eukaryotic cells.

Cancer ResearchAdenomatous polyposis coliMolecular Sequence Datamacromolecular substancesBotryllus schlosseriPolymerase Chain ReactionHomology (biology)Conserved sequenceBacterial ProteinsComplementary DNAAnimalsHumansAmino Acid SequenceUrochordataGeneticschemistry.chemical_classificationBase SequencebiologyfungiNucleic acid sequenceProteinsSequence Analysis DNAbiology.organism_classificationYeastAmino acidOncologychemistrybiology.proteinSequence AlignmentCancer Letters
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