Search results for "PSU"

showing 10 items of 678 documents

Inside a Shell—Organometallic Catalysis Inside Encapsulin Nanoreactors

2021

Abstract Compartmentalization of chemical reactions inside cells are a fundamental requirement for life. Encapsulins are self‐assembling protein‐based nanocompartments from the prokaryotic repertoire that present a highly attractive platform for intracellular compartmentalization of chemical reactions by design. Using single‐molecule Förster resonance energy transfer and 3D‐MINFLUX analysis, we analyze fluorescently labeled encapsulins on a single‐molecule basis. Furthermore, by equipping these capsules with a synthetic ruthenium catalyst via covalent attachment to a non‐native host protein, we are able to perform in vitro catalysis and go on to show that engineered encapsulins can be used …

Mycobacterium smegmatisHomogeneous catalysisNanotechnologyNanoreactor010402 general chemistrysingle-molecule FRET01 natural sciences7. Clean energyCatalysisCatalysis03 medical and health sciencesBacterial ProteinsFluorescence Resonance Energy TransferOrganometallic CompoundsParticle SizeResearch Articles030304 developmental biology0303 health sciencesChemistryencapsulinsGeneral Medicineself-assemblyGeneral ChemistrySingle-molecule FRETCompartmentalization (psychology)Bioorthogonal Chemistryhomogeneous catalysisNanostructures0104 chemical sciencesFörster resonance energy transferMicroscopy FluorescenceCovalent bondSelf-assemblyMINFLUXResearch ArticleAngewandte Chemie International Edition
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Acetylcholinesterase-Capped Mesoporous Silica Nanoparticles That Open in the Presence of Diisopropylfluorophosphate (a Sarin or Soman Simulant)

2016

Mesoporous silica nanoparticles loaded with rhodamine B and capped with acetylcholinesterase are able to be selectively opened and deliver their cargo in the presence of nerve agent simulant diisopropyl fluorophosphate (DFP).

NANOCAPSULESRESPONSIVE CONTROLLED-RELEASESarinGATED MATERIALSNanoparticle02 engineering and technologyCHEMICAL WARFARE AGENTS010402 general chemistry01 natural sciencesBiochemistryNanocapsuleschemistry.chemical_compoundQUIMICA ORGANICADESIGNSomanmedicineRhodamine BOrganic chemistryDRUG-DELIVERYPhysical and Theoretical ChemistryNerve agentNANOCONTAINERSChemistryQUIMICA INORGANICAOrganic ChemistryDNAMesoporous silica021001 nanoscience & nanotechnologyGUEST MOLECULES0104 chemical sciencesDiisopropyl fluorophosphateDCNP0210 nano-technologymedicine.drugNuclear chemistryOrganic Letters
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Mechanism of nanocapsules formation by the emulsion-diffusion process.

2007

International audience; A detailed investigation into the mechanisms of nanocapsule formation by means of the two stages “emulsion–diffusion” process is reported. Such widely used process is still poorly understood. An emulsion of oil, polymer and ethyl acetate is fabricated as a first step; dilution with pure water allows ethyl acetate to diffuse out from the droplets, leaving a suspension of nanocapsules at the end. It has been shown that the size of nanocapsules was related to the chemical composition of the organic phase and the size of primary emulsion through a simple geometrical relationship. As a consequence, most of the properties of the nanocapsules were decided at the emulsificat…

NanocapsuleDiffusionEthyl acetate02 engineering and technologyEmulsion–diffusion010402 general chemistry01 natural sciencesNanocapsulesSuspension (chemistry)Biomaterialschemistry.chemical_compoundColloid and Surface ChemistryPhase (matter)Polymer chemistry[SPI.GPROC]Engineering Sciences [physics]/Chemical and Process Engineeringchemistry.chemical_classificationEmulsionAqueous two-phase systemPolymer021001 nanoscience & nanotechnology0104 chemical sciencesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsPolycaprolactoneProcesschemistryChemical engineeringEmulsion0210 nano-technologyJournal of colloid and interface science
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Biomolecular conjugation inside synthetic polymer nanopores via glycoprotein-lectin interactions

2011

We demonstrate the supramolecular bioconjugation of concanavalin A (Con A) protein with glycoenzyme horseradish peroxidase (HRP) inside single nanopores, fabricated in heavy ion tracked polymer membranes. Firstly, the HRP-enzyme was covalently immobilized on the inner wall of the pores using carbodiimide coupling chemistry. The immobilized HRP-enzyme molecules bear sugar (mannose) groups available for the binding of Con A protein. Secondly, the bioconjugation of Con A on the pore wall was achieved through its biospecific interactions with the mannose residues of the HRP enzyme. The immobilization of biomolecules inside the nanopore leads to the reduction of the available area for ionic tran…

NanometresSynthetic membraneTransport equationNanoporesInformation processingRectification propertiesCylinders (shapes)Materials TestingConcanavalin AGeneral Materials ScienceFunctional polymersConical nanoporeschemistry.chemical_classificationChemistryBlocking effectElectric rectifiersComputer simulationEnzymesData processingNanoporeEnzyme moleculesFunctional polymersMolecular imprintingPorosityBio-molecularInner wallsMolecular imprintingSupramolecular chemistryNanotechnologyHorseradish peroxidaseIonic transportsNanocapsulesBio-conjugationMoleculeParticle SizeAqueous solutionsGlycoproteinsBiomoleculesBioconjugationBiomoleculeNanostructuresModel simulationChemical engineeringModels ChemicalPolymer membraneConductance stateFISICA APLICADABiospecific interactionSynthetic polymersSugarsSupramolecular chemistryPore wallCarbodiimide-coupling chemistry
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Microencapsulation of antioxidant compounds through innovative technologies and its specific application in meat processing

2018

Background Meat has a complex physical structure and chemical composition that is very prone to oxidation. Plants are sources of biologically active compounds (antioxidants) of interest as potential raw materials for meat processing, primary as replacements for synthetic additives. Some examples are essential oils from aromatic plants that are usually unstable under common processing and storage conditions and exhibit strong smell and off flavour. Hence, stable delivery systems like encapsulation are required. Scope and approach Encapsulation, and particularly spray-drying, offers protection of active compounds, their controlled and targeted release in food products and ability to mask unac…

Natural antioxidants ; Meat processing ; Encapsulation ; Wall materials ; Spray-drying ; NanotechnologyMeat packing industryOff-flavourComputer sciencebusiness.industrySpray-dryingAromatic plants04 agricultural and veterinary sciencesNatural antioxidantsRaw materialMeat processing040401 food scienceWall material0404 agricultural biotechnologyPhysical structureWall materialsFood productsNanotechnologyEncapsulationBiochemical engineeringbusinessTargeted releaseFood ScienceBiotechnology
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Xenotransplantation of parathyroids in rats using barium-alginate and polyacrylic acid multilayer microcapsules

2001

The integrity and function of encapsulated parathyroid tissue following xenotransplantation is limited by oxygen and nutrition supply and capsule fibrosis. Since some of these factors depend on stability and biocompatibility of the coating material, multilayer microcapsules have been developed. Parathyroid tissue pieces and digested single cells from pigs were encapsulated in barium-alginate and in polyacrylic acid (PAA) multilayer capsules. After 7 days of culture the function of the encapsulated cells were assessed. Subsequently, in a part of the cultured microcapsules the viability was directly assessed whereas the other part was transplanted in dark animal [DA] rats for 30 days. After e…

NecrosisBiocompatibilityAlginatesCell SurvivalSwineBarium CompoundsTransplantation HeterologousAcrylic ResinsConnective tissueParathyroid hormoneToxicologyPathology and Forensic MedicineParathyroid Glandschemistry.chemical_compoundDrug Delivery SystemsCoated Materials BiocompatibleGlucuronic AcidIn vivoFibrosismedicineAnimalsCells CulturedChemistryHexuronic AcidsGraft SurvivalCapsuleCell BiologyGeneral MedicineAnatomymedicine.diseaseGlucuronic acidMolecular biologyRatsmedicine.anatomical_structureParathyroid Hormonemedicine.symptomExperimental and Toxicologic Pathology
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Evaluation of the healing of precoated vascular dacron prostheses.

1991

Knitted and woven Dacron grafts commercially coated with bovine collagen, gelatin and human albumin were implanted end-to-side between the infrarenal aorta and the bifurcation in 35 growing pigs. Grafts were explanted after 4, 8 and 12 weeks and compared to 6 uncoated knitted prostheses preclotted with blood that served as a control. Uncoated grafts rapidly developed a firmly attached neointima lined with endothelium. Compared with coated grafts the thrombus-free area of uncoated grafts was significantly larger (P less than 0.05). The slow resorption of albumin resulted in a delayed and incomplete neointimal healing and failing graft incorporation. Although the bovine collagen was only mini…

Neointimamedicine.medical_specialtyBovine collagenfood.ingredientEndotheliumSurface PropertiesSwineProsthesis DesignGelatinfoodmedicineAnimalsSerum AlbuminWound Healingbusiness.industryPolyethylene TerephthalatesAlbuminGraft Occlusion VascularCapsuleHyperplasiamedicine.diseaseSurgeryResorptionBlood Vessel ProsthesisProsthesis Failuremedicine.anatomical_structureMicroscopy Electron ScanningGelatinSurgeryFemaleCollagenEndothelium VascularbusinessBiomedical engineeringLangenbecks Archiv fur Chirurgie
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Sur les Terminaisons Nerveuses Sensitives du Clitoris chez la Truie (Sus scrofa domesticus)

1991

Summary On the Sensory Nerve-Endings in the Porcine Clitoris Neural receptors of the porcine clitoris were examined using light and electron microscopy. Perfusion with ink allowed study of the unique vascular arrangement associated with the genital corpuscles. Sensory nerve-endings were generally rounded and formed a morphologically and structurally characteristic unit. They were composed of a network of primarily non-myelinated nerve fibers and flat cells. Between these structures, isolated small blood vessels were embedded amongst collagen fibers and amorphous material. An external capsule of variable thickness always surrounded the structures. A complex arrangement of vessels in the cent…

Neural receptorsExternal capsuleGeneral VeterinaryVariable thicknessCapsuleClitorisGeneral MedicineAnatomyBiologylaw.inventionmedicine.anatomical_structurelawGlomerulusmedicineElectron microscopeAnatomia, Histologia, Embryologia: Journal of Veterinary Medicine Series C
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Electrical properties of Au/CdZnTe/Au detectors grown by the boron oxide encapsulated Vertical Bridgman technique

2016

Abstract In this work we report on the results of electrical characterization of new CdZnTe detectors grown by the Boron oxide encapsulated Vertical Bridgman technique (B-VB), currently produced at IMEM-CNR (Parma, Italy). The detectors, with gold electroless contacts, have different thicknesses (1 and 2.5 mm) and the same electrode layout, characterized by a central anode surrounded by a guard-ring electrode. Investigations on the charge transport mechanisms and the electrical contact properties, through the modeling of the measured current–voltage ( I – V ) curves, were performed. Generally, the detectors are characterized by low leakage currents at high bias voltages even at room tempera…

Nuclear and High Energy PhysicsTraveling heater method electrical propertie02 engineering and technology01 natural sciencesBoron oxide encapsulated Vertical Bridgman techniqueTraveling heater methodElectrical resistivity and conductivity0103 physical sciencesInstrumentationDeposition (law)010302 applied physicsPhysicsInterfacial layer-thermionic-diffusionbusiness.industryCdZnTe detectorsCdZnTe detectorSettore FIS/01 - Fisica SperimentaleBiasing021001 nanoscience & nanotechnologySettore FIS/07 - Fisica Applicata(Beni Culturali Ambientali Biol.e Medicin)Electrical contactsAnodeBoron oxideelectrical propertiesElectrodeOptoelectronics0210 nano-technologybusinessVoltageNuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment
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Extranodal extension of nodal metastases is a poor prognostic moderator in non-small cell lung cancer: a meta-analysis

2018

Extranodal extension (ENE) of nodal metastasis is defined as the extension of metastatic cells through the nodal capsule into the perinodal tissue. This morphological parameter, recently proposed as an important prognostic factor in different types of malignancy, has not been included in the TNM staging system for non-small cell lung cancer (NSCLC). In this systematic review with meta-analysis, we weighted the prognostic role of ENE in patients with lymph node-positive NSCLC. Two independent authors searched SCOPUS and PubMed through 28 February 2017. Prospective and retrospective studies on NSCLC, comparing patients with presence of ENE (ENE+) ENE+) vs. only intranodal extension (ENE–) and…

Oncologymedicine.medical_specialtyLung NeoplasmsExtracapsular; Extranodal; Lung cancer; Metastasis; NSCLC; PrognosisTNM staging systemNSCLCMalignancyMetastasisPathology and Forensic MedicineMetastasis03 medical and health sciences0302 clinical medicineCarcinoma Non-Small-Cell LungInternal medicinemedicine030212 general & internal medicineLung cancerMolecular BiologyEne reactionLung cancer . NSCLC . Prognosis . Extranodal . Extracapsular . MetastasisExtracapsularbusiness.industryHazard ratioRetrospective cohort studyCell BiologyGeneral MedicinePrognosismedicine.diseaseLymphatic Metastasis030220 oncology & carcinogenesisRelative riskExtranodalLymph NodesLung cancerNeoplasm Recurrence Localbusiness
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