Search results for "Roca"

showing 10 items of 1893 documents

Highly enantioselective synthesis of fluorinated gamma-amino alcohols through proline-catalyzed cross-Mannich reaction.

2005

A new, simple route for the synthesis of fluorinated beta-alkyl gamma-amino alcohols in optically pure form in only two steps and featuring proline catalysis from inexpensive and readily available starting materials is described. The applied strategy allows for the introduction of diversity into both the beta-fluoroalkyl and alpha-alkyl groups of these compounds. [reaction: see text]

Hydrocarbons FluorinatedProlineStereochemistryChemistryOrganic ChemistryEnantioselective synthesisStereoisomerismGeneral MedicineBiochemistryCombinatorial chemistryAmino AlcoholsCatalysisCatalysisMannich BasesOrganic chemistryProlinePhysical and Theoretical ChemistryMannich reactionOrganic letters
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New Cathepsin Inhibitors to Explore the Fluorophilic Properties of the S 2 Pocket of Cathepsin B: Design, Synthesis, and Biological Evaluation

2011

5 páginas, 1 figura, 2 tablas -- PAGS nros. 5256-5260

Hydrocarbons FluorinatedStereochemistryStereoisomerismhydrolasesstereoselectivityCatalysisCathepsin BCathepsin BNitrilesinhibitorsCombinatorial Chemistry TechniquesHumansMoleculefluorinated ligandsBiological evaluationCathepsinMolecular StructureCombinatorial Chemistry TechniquesligandsChemistryOrganic ChemistryStereoisomerismDipeptidesGeneral Chemistryfluorinated fluorinatedDesign synthesisDrug DesignpeptidesStereoselectivityChemistry – A European Journal
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An efficient synthesis of new fluorinated uracil derivatives.

2003

A series of potentially biologically active fluorinated uracil derivatives has been prepared in three steps from oxazolines and fluorinated nitriles with good chemical yields. Fustero Lardies, Santos, Santos.Fustero@uv.es ; Sanz Cervera, Juan Francisco, Juan.F.Sanz@uv.es ; Asensio Martinez, Amparo, Amparo.Asensio@uv.es

Hydrocarbons FluorinatedSynthesis ; Fluorinated uracil derivatives ; Oxazolines ; Biologically activeAntimetabolitesUNESCO::QUÍMICABiologically active:QUÍMICA::Química orgánica [UNESCO]UracilGeneral MedicineOxazolines:QUÍMICA [UNESCO]Combinatorial chemistryFluorinated uracil derivativesSynthesischemistry.chemical_compoundchemistryNitrilesUNESCO::QUÍMICA::Química orgánicaUracilOxazolesChemical communications (Cambridge, England)
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Measured and Modeled Residue Dynamics of Famoxadone and Oxathiapiprolin in Tomato Fields

2018

A reliable analytical method for the simultaneous determination of famoxadone and oxathiapiprolin dissipation kinetics as well as the metabolites of oxathiapiprolin (IN-E8S72 and IN-WR791) in tomato and soil was developed. We studied the dissipation of famoxadone and oxathiapiprolin in tomatoes grown using different kinetic curves in the area of Beijing in 2015 and 2016. Our results show that the most suitable model for two fungicides in 2015 and 2016 was first-order kinetic and second-order kinetic with the half-lives of 3.4 to 5.2 and 2.4 to 3.0 days, respectively. In addition, we applied the dynamic plant uptake model dynamiCROP and combined it with results from the field experiments to …

Hydrocarbons Fluorinatedhalf-lifeFood Contamination010501 environmental sciences01 natural scienceschemistry.chemical_compoundSolanum lycopersicumplant uptake modeldynamiCROPHumansSoil Pollutants0105 earth and related environmental sciencesGram010401 analytical chemistryOxathiapiprolinPesticide ResiduesFamoxadonefood and beveragesGeneral ChemistrydissipationpesticidesPesticideStrobilurinsFungicides Industrial0104 chemical sciencesFungicideKineticsHorticulturechemistryPyrazolesGeneral Agricultural and Biological SciencesHalf-Life
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Hydrogen-ion driven molecular motions in Cu2+-complexes of a ditopic phenanthrolinophane ligand

2004

One of the first kinetic evaluations of a metal ion interchange between the two coordination sites of a ditopic macrocycle is presented. Garcia-España Monsonis, Enrique, Enrique.Garcia-Es@uv.es ; Soriano Soto, Concepción, Concepcion.Soriano@uv.es ; Verdejo Viu, Begoña, Begona.Verdejo@uv.es

Hydrogen ionHydrogenStereochemistryUNESCO::QUÍMICAKineticschemistry.chemical_elementHydrocarbons CyclicHydrogen ; Cu2 ; Phenanthrolinophane ; Ditopic macrocycleDitopic macrocycleLigands:QUÍMICA [UNESCO]CatalysisIonPhenanthrolinophaneCu2Materials ChemistryMolecular motionOrganometallic CompoundsLigandChemistryUNESCO::QUÍMICA::Química inorgánicaMetals and AlloysGeneral ChemistryHydrogen-Ion Concentration:QUÍMICA::Química inorgánica [UNESCO]Surfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsCrystallographyKineticsCeramics and CompositesProtonsCopperHydrogen
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Modelling electrocatalysis of hydroquinone oxidation by nicotinamide adenine dinucleaotide coenzyme encapsulated within SBA-15 and MCM-41 mesoporous …

2006

The electrochemical response of NADH associated to two mesoporous aluminosilicates, MCM-41 and SBA-15, is described upon attachment of such materials into polymer-film electrodes. The studied materials display a significant electrocatalytic activity towards the oxidation of 1,4-dihydrobenzoquinone, H2Q. Two models for describing the electrocatalytic process, based on the general theory of mediated electrocatalysis and the Lovric and Scholz formulation of the voltammetry of microparticles are discussed. Voltammetric and chronoamperometric data indicate that the electrocatalytic process involves the formation of a surface-confined NADH–H2Q adduct in the case of SBA-15, while a surface reactio…

HydroquinoneGeneral Chemical EngineeringElectrochemistryElectrocatalystMolecular sievechemistry.chemical_compoundMCM-41Chemical engineeringchemistryElectrochemistryOrganic chemistryCyclic voltammetryMesoporous materialVoltammetryElectrochimica Acta
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AICA-ribosiduria due to ATIC deficiency: Delineation of the phenotype with three novel cases, and long-term update on the first case.

2020

5-Amino-4-imidazolecarboxamide-ribosiduria (AICA)-ribosiduria is an exceedingly rare autosomal recessive condition resulting from the disruption of the bifunctional purine biosynthesis protein PURH (ATIC), which catalyzes the last two steps of de novo purine synthesis. It is characterized biochemically by the accumulation of AICA-riboside in urine. AICA-ribosiduria had been reported in only one individual, 15 years ago. In this article, we report three novel cases of AICA-ribosiduria from two independent families, with two novel pathogenic variants in ATIC. We also provide a clinical update on the first patient. Based on the phenotypic features shared by these four patients, we define AICA-…

Hydroxymethyl and Formyl TransferasesMalemedicine.medical_specialtyCyclohydrolase activityBioinformaticsCongenital AbnormalitiesEpilepsyMultienzyme ComplexesIntellectual DisabilityGeneticsmedicineHumansBifunctional Purine Biosynthesis Protein PURHChildGenetics (clinical)ATIC DEFICIENCYEpilepsybusiness.industryInfant NewbornInfantmedicine.diseaseAminoimidazole CarboxamidePhenotypePhenotypeNucleotide DeaminasesChild PreschoolMutationMedical geneticsFemaleRibonucleosidesNephrocalcinosisbusinessRare diseaseJournal of inherited metabolic diseaseREFERENCES
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Update I. A systematic review on the efficacy and safety of chloroquine/hydroxychloroquine for COVID-19

2020

Purpose To assess efficacy and safety of chloroquine (CQ)/hydroxychloroquine (HCQ) for treatment or prophylaxis of COVID-19 in adult humans. Materials and methods MEDLINE, PubMed, EMBASE and two pre-print repositories (bioRxiv, medRxiv) were searched from inception to 8th June 2020 for RCTs and nonrandomized studies (retrospective and prospective, including single-arm, studies) addressing the use of CQ/HCQ in any dose or combination for COVID-19. Results Thirty-two studies were included (6 RCTs, 26 nonrandomized, 29,192 participants). Two RCTs had high risk, two ‘some concerns’ and two low risk of bias (Rob2). Among nonrandomized studies with comparators, nine had high risk and five moderat…

ICU Intensive care unit;medicine.medical_treatmentCritical Care and Intensive Care MedicineRR Risk Ratio0302 clinical medicineChloroquineRCT Randomized clinical trialMedicineHCQ Hydroxychloroquine;Prospective StudiesProspective cohort studyChloroquine COVID-19 Hydroxychloroquine Mortality SARS-CoV-2ChloroquineECG Electrocardiogram;Rob2 Revised tool for Risk of Bias in randomized trials;CI Confidence interval;Coronavirus InfectionsPost-Exposure ProphylaxisHydroxychloroquinemedicine.drugmedicine.medical_specialtyCoronavirus disease 2019 (COVID-19)Pneumonia ViralMEDLINEContext (language use)Antiviral AgentsArticleWHO World Health OrganizationBetacoronavirus03 medical and health sciencesInternal medicineHumansMortalityCOVID-19 Coronavirus disease 2019;Post-exposure prophylaxisPandemicsRetrospective StudiesCQ Chloroquine;SARS-CoV-2ROBINS-I Risk of Bias in Non-randomized Studies of Interventions;business.industryCOVID-19030208 emergency & critical care medicineHydroxychloroquineRetrospective cohort studyHCWs Healthcare workers;NOS Newcastle Ottawa Scale;COVID-19 Drug Treatment030228 respiratory systembusinessHR Hazard Ratio;Journal of Critical Care
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Isomer effects in fragmentation of Polycyclic Aromatic Hydrocarbons

2015

We have observed significant differences in the fragmentation patterns of isomeric Polycyclic Aromatic Hydrocarbon (PAH) cations following collisions with helium atoms at center-of-mass energies around 100 eV. This is in contrast to the situation at other collision energies or in photo-absorption experiments where isomeric effects are very weak and where the lowest-energy dissociation channels (H- and C2H2-loss) domihate in statistical fragmentation processes. In the 100 eV range, non-statistical fragmentation also competes and is uniquely linked to losses of single carbon atoms (CHx-losses). We find that such CHx-losses are correlated with the ionic ground state energy within a given group…

IONSCollision-induced dissociationIonic bondingPolycyclic aromatic hydrocarbonPhotochemistryANTHRACENE01 natural sciencesDissociation (chemistry)IsomersMOLECULESchemistry.chemical_compoundFragmentation (mass spectrometry)Fragmentation0103 physical sciencesMoleculeCollisionsTANDEM MASS-SPECTROMETRYPolycyclic Aromatic HydrocarbonsPhysical and Theoretical ChemistryCOLLISION-INDUCED DISSOCIATION010303 astronomy & astrophysicsInstrumentationSpectroscopyNon-statistical fragmentationchemistry.chemical_classificationAnthracenePolycyclic Aromatic Hydrocarbons PAHs[PHYS.PHYS.PHYS-ATM-PH]Physics [physics]/Physics [physics]/Atomic and Molecular Clusters [physics.atm-clus]010401 analytical chemistryCondensed Matter Physics0104 chemical sciencesDIFFERENTIATIONchemistryIONIZATIONCATIONSGROWTH[PHYS.PHYS.PHYS-CHEM-PH]Physics [physics]/Physics [physics]/Chemical Physics [physics.chem-ph]Ground stateC14H10International Journal of Mass Spectrometry
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ISOLATED SHORT PR IN CHILDREN WITH PALPITATION: AN ELECTROCARDIOGRAPHIC FINDING OF FAST-SLOW NODAL TACHYCARDIA?

2007

ISOLATED SHORT PR IN CHILDREN WITH PALPITATION: AN ELECTROCARDIOGRAPHIC FINDING OF FAST-SLOW NODAL TACHYCARDIA?

ISOLATED SHORT PR IN CHILDREN WITH PALPITATION: AN ELECTROCARDIOGRAPHIC FINDING OF FAST-SLOW NODAL TACHYCARDIA?
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