Search results for "quantum dot"
showing 10 items of 418 documents
Struktūra un fotofizikālie procesi 0D un 1D InGaN kompozītu materiālos
2014
Šajā disertācijā tiek aprakstīti strukturālās un fotofizikālās MOCVD izaudzēto GaN nanovadu (NV) un InGaN kvantu punktu (KP) īpašības. Abos gadījumos ir parādīts, ka ex-situ RHEED mērījumi ir iespējami un sniedz kvalitatīvu informāciju par struktūru. Kombinācijā ar citām metodēm, pirmkārt, ir parādīts, ka nemetāliskā katalizatora veicinātā GaN NV īpašības, kad sintezēts uz GaN (0001) virsmas, atšķiras no tradicionāli iegūtajiem. Šinī gadījumā katalizators lokalizējas pie nanovadu pamatnes nevis tā galā un augšanas virziens ir atšķirīgs no kristalogrāfiskās c-ass, rezultātā iegūstot semipolārās NV struktūras. Otrkārt, InGaN kvantu punktos ir konstatēt saspiesta kristāliskā režģa struktūra au…
Sensing Chiral Drugs by Using CdSe/ZnS Nanoparticles Capped withN-Acetyl-L-Cysteine Methyl Ester
2013
Chiral quantum dots (QDs), differing in their core or shell size and, consequently, in their optical properties, were synthesized by the treatment of commercially available amine-capped quantum dots with methyl ester N-acetyl-L-cysteine (CysP). Interestingly, their colloidal methanol solutions remain stable for several months. Their NMR and IR spectra were in accordance with CysP binding to the QD surface through two anchoring groups; its thiolate (strongly bound) and the carbonyl group of its ester (weaker bound) group, whereas their circular dichroism (CD) spectra showed a new broad redshifted band, suggesting that the attachment to the QD surface modified the conformational equilibrium t…
A random-walk benchmark for single-electron circuits
2021
Mesoscopic integrated circuits aim for precise control over elementary quantum systems. However, as fidelities improve, the increasingly rare errors and component crosstalk pose a challenge for validating error models and quantifying accuracy of circuit performance. Here we propose and implement a circuit-level benchmark that models fidelity as a random walk of an error syndrome, detected by an accumulating probe. Additionally, contributions of correlated noise, induced environmentally or by memory, are revealed as limits of achievable fidelity by statistical consistency analysis of the full distribution of error counts. Applying this methodology to a high-fidelity implementation of on-dema…
Quantum Well States in Two-Dimensional Gold Clusters on MgO Thin Films
2008
The electronic structure of ultra-small Au clusters on thin MgO/Ag(001) films has been analyzed by scanning tunneling spectroscopy and density functional theory. The clusters exhibit two-dimensional (2D) quantum well states, whose shapes resemble the eigen-states of a 2D electron gas confined in a parabolic potential. From the symmetries of the HOMO and LUMO of a particular cluster, its electron filling and charge state is determined. In accordance to a DFT Bader-charge analysis, aggregates containing up to twenty atoms accumulate one to four extra electrons due to a charge transfer from the MgO/Ag interface. The HOMO - LUMO gap is found to close for clusters containing between 70 and 100 a…
Anisotropic polarization of non‐polar GaN quantum dot emission
2009
We report on experimental and theoretical studies of the polarization selection rules of the emission of non-polar GaN/AlN self-assembled quantum dots. Time-integrated and time-resolved photoluminescence measurements have been performed to determine the degree of polarization. It is found that the emission of some samples can be predominantly polarized parallel to the wurtzite c axis, in striking difference with the previously reported results for bulk GaN and its heterostructures, in which the emission was preferentially polarized perpendicular to the c axis. Theoretical calculations based on an 8-band k·p model are used to analyze the relative importance of strain, confinement and quantum…
Vortices in rotating two-component boson and fermion traps
2010
Quantum liquids may carry angular momentum by the formation of vortex states. This is well known for Bose-Einstein condensates in rotating traps, and was even found to occur in quantum dots at strong magnetic fields. Here we consider a two-component quantum liquid, where coreless vortices and interlaced lattices of coreless vortices appear in a very similar way for fermions and bosons with repulsive two-body interactions. The ground states at given angular momentum, as well as the pair correlations for equal and different numbers of atoms in the two components, are studied. (C) 2009 Elsevier B.V. All rights reserved.
Random population model to explain the recombination dynamics in single InAs/GaAs quantum dots under selective optical pumping
2011
18 páginas, 3 tablas, 9 figuras.-- et al.
Decoherence of the Exciton and Decay of the Excitonic Polaron in Quantum Dots
2005
Bulk-phonon mechanisms of decoherence of an exciton confined in a quantum dot (QD) are considered in order to establish time limitations for the coherent control of the exciton with relevance to its application in quantum information processing. These are the formation and decay of the excitonic polaron. The estimations of characteristic dephasing times for the InAs/GaAs QD are discussed.
Influence of strain in the reduction of the internal electric field in GaN/AlN quantum dots grown ona-plane 6H-SiC
2006
The strain state of stacks of GaN/AIN quantum dots (QDs) grown on (0001) and (1120) 6H-SiC has been investigated by means of Raman spectroscopy. Depending on the orientation of the wurtzite axis with respect to the growth direction it is found that the piezoelectric contribution to the electrostatic potential may either reinforce that arising from the spontaneous polarization or oppose it. The experimental results are compared with a theoretical model for the strain and polarization field in QDs of both orientations that allows the calculation of the electrostatic potential in the QDs. Both the experimental results and the theoretical model indicate that the internal electric field and elec…
Characterization of quantum dot/conducting polymer hybrid films and their application to light-emitting diodes.
2009
Quantum dot/conducting polymer hybrid films are used to prepare light-emitting diodes (LEDs). The hybrid films (CdSe@ZnS quantum dots excellently dispersed in a conducting polymer matrix, see figure) are readily prepared by various solution-based processes and are also easily micropatterned. The LEDs exhibit a turn-on voltage of 4 V, an external quantum efficiency greater than 1.5%, and almost pure-green quantum-dot electroluminescence.