0000000000118863
AUTHOR
Dmitry Gorelov
showing 62 related works from this author
Total absorption γ -ray spectroscopy of niobium isomers
2019
15 pags. 17 figs., 5 tabs.
First isomeric yield ratio measurements by direct ion counting and implications for the angular momentum of the primary fission fragments
2018
We report the first experimental determination of independent isomeric yield ratios using direct ion counting with a Penning trap, which offered such a high resolution in mass that isomeric states could be separated. The measurements were performed at the Ion Guide Isotope Separator On-Line (IGISOL) facility at the University of Jyvaskyla. The isomer production ratios of Ge-81, Y-96,Y-97 Sn-128(,1)30, and Sb-129 in the 25-MeV proton-induced fission of U-na(t) and Th-232 were studied. Three isomeric pairs (Ge-81, Y-96, and Sb-129) were measured for the first time for the U-na(t)(p, f) reaction, while all the reported yield ratios for the Th-232(p, f) reaction were determined for the first ti…
First determination of β-delayed multiple neutron emission beyond A = 100 through direct neutron measurement : The P2n value of 136Sb
2018
Background: β-delayed multiple neutron emission has been observed for some nuclei with A≤100, being the Rb100 the heaviest β2n emitter measured to date. So far, only 25P2n values have been determined for the ≈300 nuclei that may decay in this way. Accordingly, it is of interest to measure P2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A>100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of a…
Experimental study of 100Tc β decay with total absorption γ -ray spectroscopy
2017
The β decay of 100Tc has been studied by using the total absorption γ -ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. In this work the new Decay Total Absorption γ -ray Spectrometer in coincidence with a cylindrical plastic β detector has been employed. The β intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also r…
Total absorption studies of high priority decays for reactor applications: 86Br and 91Rb
2017
Preliminary results from beta decay studies of nuclei that are important for reactor applications are presented. The beta decays have been studied using the total absorption technique (TAS) and the pure beams provided by the JYFLTRAP system at the IGISOL facility of the University of Jyväskylä. peerReviewed
New accurate measurements of neutron emission probabilities for relevant fission products
2017
We have performed new accurate measurements of the beta-delayed neutron emission probability for ten isotopes of the elements Y, Sb, Te and I. These are fission products that either have a significant contribution to the fraction of delayed neutrons in reactors or are relatively close to the path of the astrophysical r process. The measurements were performed with isotopically pure radioactive beams using a constant and high efficiency neutron counter and a low noise beta detector. Preliminary results are presented for six of the isotopes and compared with previous measurements and theoretical calculations. peerReviewed
High-precision mass measurement ofS31with the double Penning trap JYFLTRAP improves the mass value forCl32
2010
Characterization of a Be(p,xn) Neutron Source for Fission Yields Measurements
2013
We report on measurements performed at The Svedberg Laboratory (TSL) to characterize a proton-neutron converter for independent fission yield studies at the IGISOL-JYFLTRAP facility (Jyv\"askyl\"a, Finland). A 30 MeV proton beam impinged on a 5 mm water-cooled Beryllium target. Two independent experimental techniques have been used to measure the neutron spectrum: a Time of Flight (TOF) system used to estimate the high-energy contribution, and a Bonner Sphere Spectrometer able to provide precise results from thermal energies up to 20 MeV. An overlap between the energy regions covered by the two systems will permit a cross-check of the results from the different techniques. In this paper, th…
Study of the β decay of fission products with the DTAS detector
2017
Total Absorption Spectroscopy measurements of the β decay of 103Mo and 103Tc, important contributors to the decay heat summation calculation in reactors, are reported in this work. The analysis of the experiment, performed at IGISOL with the new DTAS detector, show new β intensity that was not detected in previous measurements with Ge detectors. peerReviewed
Characterization of a neutron–beta counting system with beta-delayed neutron emitters
2016
A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known β-delayed neutron emission properties. The setup consists of BELEN-20, a 4π neutron counter with twenty 3He proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for β counting and a selftriggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, β and β-neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on the accura…
Towards commissioning the new IGISOL-4 facility
2013
Abstract The Ion Guide Isotope Separator On-Line facility at the Accelerator Laboratory of the University of Jyvaskyla is currently being re-commissioned as IGISOL-4 in a new experimental hall. Access to intense beams of protons and deuterons from a new MCC30/15 cyclotron, with continued possibility to deliver heavy-ion beams from the K = 130 MeV cyclotron, offers extensive opportunities for long periods of fundamental experimental research, developments and applications. A new layout of beam lines with a considerable increase in floor space offers new modes of operation at the facility, as well as a possibility to incorporate more complex detector setups. We present a general overview of I…
High-Precision Proton-Capture Q Values for 25Al(p,γ)26Si and 30P(p,γ)31Si
2017
The masses of astrophysically relevant nuclei, 25Al and 30P, have recently been measured with the JYFLTRAP double Penning trap at the new IGISOL-4 facility at the University of Jyväskylä. Unparalleled precisions of 63 and 64 eV were achieved for the 25Al and 30P masses, respectively. The proton-capture Q values for 25Al(p, γ)26Si and 30P(p, γ)31S were also determined, and their precisions improved by a factor of 4 and 2, respectively, in comparison with AME12. The impact of the more precise values on the resonant proton-capture rate has also been studied. peerReviewed
Developments for neutron-induced fission at IGISOL-4
2016
At the IGISOL-4 facility, neutron-rich, medium mass nuclei have usually been produced via charged particle-induced fission of natural uranium and thorium. Neutron-induced fission is expected to have a higher production cross section of the most neutron-rich species. Development of a neutron source along with a new ion guide continues to be one of the major goals since the commissioning of IGISOL-4. Neutron intensities at di↵erent angles from a beryllium neutron source have been measured in an on-line experiment with a 30 MeV proton beam. Recently, the new ion guide coupled to the neutron source has been tested as well. Details of the neutron source and ion guide design together with prelimi…
Super-Allowed β Decay of23Mg Studied with a High-Precision Germanium Detector
2015
Large Impact of the Decay of Niobium Isomers on the Reactor ¯νe Summation Calculations
2019
Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The β-intensity distributions of 100gs;100mNb and 102gs;102mNb β decays have been determined using the total absorption γ-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyväskylä. Here, the double Penning trap system JYFLTRAP was employed to disentangle the β decay of the isomeric states. The new data obtained in this …
Total absorption γ -ray spectroscopy of the β -delayed neutron emitters I137 and Rb95
2019
The decays of the β-delayed neutron emitters I137 and Rb95 have been studied with the total absorption γ-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption γ-ray spectrometer, a segmented detector composed of 18 NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt γ rays and delayed neutron interactions to eliminate this source of contamination. Due to the s…
Measurement of the heaviest Beta-delayed 2-neutron emitter: 136Sb
2017
The Beta-delayed neutron emission probability, Pn , of very exotic nuclei is crucial for the understanding of nuclear structure properties of many isotopes and astrophysical processes such as the rapid neutron capture process (r-process). In addition Beta-delayed neutrons are important in a nuclear power reactor operated in a prompt sub-critical, delayed critical condition, as they contribute to the decay heat inducing fission reactions after a shut down. The study of neutron-rich isotopes and the measurement of Beta-delayed one-neutron emitters (Beta1n) is possible thanks to the Rare Isotope Beam (RIB) facilities, where radioactive beams allow the production of exotic nuclei of interest, w…
Theoretical and experimental studies of the neutron rich fission product yields at intermediate energies
2012
A new method to measure the fission product independent yields employing the ion guide technique and a Penning trap as a precision mass filter, which allows an unambiguous identification of the nuclides is presented. The method was used to determine the independent yields in the proton-induced fission of 232 Th and 238 U at 25 MeV. The data were analyzed with the consistent model for description of the fission product formation cross section at the projectile energies up to 100 MeV. Pre-compound nucleon emission is described with the two-component exciton model using Monte Carlo method. Decay of excited compound nuclei is treated within time-dependent statistical model with inclusion of the…
On the resonant neutrinoless double-electron-capture decay of ^{136}Ce
2011
Abstract The double-electron-capture Q value for the 136Ce decay to 136Ba has been determined at JYFLTRAP. The measured value 2378.53(27) keV excludes the energy degeneracy with the 0 + excited state of the decay daughter 136Ba at 2315.32(7) keV in a resonant 0 ν ECEC decay by 11.67 keV. The new Q value differs from the old adopted value 2419(13) keV (Atomic Mass Evaluation 2003) by 40 keV and is 50 times more precise. Our calculations show that the precise Q value renders the resonant 0 ν ECEC decay of 136Ce undetectable by the future underground detectors. We measured also the double-β decay Q value of 136Xe to be 2457.86(48) keV which agrees well with the value 2457.83(37) keV measured a…
Characterization of a cylindrical plastic β-detector with Monte Carlo simulations of optical photons
2017
In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic β-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extens…
Determination of β -decay ground state feeding of nuclei of importance for reactor applications
2020
12 pags., 6 figs., 3 tabs.
Independent Isotopic Product Yields in 25 MeV and 50 MeV Charged Particle Induced Fission of 238U and 232Th
2014
Abstract Independent isotopic yields for most elements from Zn to La in 25-MeV proton-induced fission of 238U and 232Th have been determined at the IGISOL facility in the University of Jyvaskyla. In addition, isotopic yields for Zn, Ga, Rb, Sr, Zr, Pd and Xe in 50-MeV proton-induced fission of 238U and for Zn, Ga, Rb, Sr, Cd and In in 25-MeV deuterium-induced fission of 238U have been measured. The utilised technique recently developed at the University of Jyvaskyla, is based on a combination of the ion guide technique and the ability of a Penning trap to unambiguously identify the isotopes by their atomic mass. Since the yields are determined by ion counting, no prior knowledge beyond the …
Precise measurements of half-lives and branching ratios for the ββ mirror transitions in the decay of 23Mg and 27Si
2017
Half-lives and branching ratios for the two mirror ββ decays of 23Mg and 27Si have been measured at the University of Jyväskylä with the IGISOL facility. The results obtained, T1/2=11.303(3)T1/2=11.303(3) s and T1/2=4.112(2)T1/2=4.112(2) s for the half-lives of 23Mg and 27Si , respectively, are 7 and 8 times more precise than the averages of previous measurements. The values obtained for the super-allowed branching ratios of 23Mg and 27Si are B.R.=92.18(8)%B.R.=92.18(8)% and B.R.=99.74(2)%B.R.=99.74(2)% , respectively. The result for 23Mg is three times more precise than the average of the previous measurements, while for 27Si the precision has not been improved, the average of the previous…
Mass measurements in the vicinity of the doubly magic waiting pointNi56
2010
Masses of $^{56,57}\mathrm{Fe}$, $^{53}\mathrm{Co}$${}^{m}$, $^{53,56}\mathrm{Co}$, $^{55,56,57}\mathrm{Ni}$, $^{57,58}\mathrm{Cu}$, and $^{59,60}\mathrm{Zn}$ have been determined with the JYFLTRAP Penning trap mass spectrometer at the Ion-Guide Isotope Separator On-Line facility with a precision of $\ensuremath{\delta}m/m\ensuremath{\leqslant}3\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}$. The ${Q}_{\mathrm{EC}}$ values for $^{53}\mathrm{Co}$, $^{55}\mathrm{Ni}$, $^{56}\mathrm{Ni}$, $^{57}\mathrm{Cu}$, $^{58}\mathrm{Cu}$, and $^{59}\mathrm{Zn}$ have been measured directly with a typical precision of better than $0.7 \mathrm{keV}$ and Coulomb displacement energies have been dete…
Strong γ-ray emission from neutron unbound states populated in β-decay: Impact on (n,γ) cross-section estimates
2017
J. L. Taín et al. -- 6 pags., 7 figs., 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0
Nuclear fission studies with the IGISOL method and JYFLTRAP
2015
there is no unique model or theory which describes all aspects of this phenomenon. Experimental measurements of nuclear fission product distributions still remains quite a challenging task for modern technologies. In the present work nuclear fission is studied from the radioactive ion beam production point of view. Some models suggest that the neutron-induced fission can be more favorable for production of neutron-rich nuclides than the proton-induced fission. The general idea of this thesis is to compare all aspects of both approaches in connection with the IGISOL method. A new technique to determine independent fission product yields was suggested for the comparison. This technique has be…
Precision Mass Measurements beyond $^{132}$Sn: Anomalous behaviour of odd-even staggering of binding energies
2012
Atomic masses of the neutron-rich isotopes $^{121-128}$Cd, $^{129,131}$In, $^{130-135}$Sn, $^{131-136}$Sb, and $^{132-140}$Te have been measured with high precision (10 ppb) using the Penning trap mass spectrometer JYFLTRAP. Among these, the masses of four r-process nuclei $^{135}$Sn, $^{136}$Sb, and $^{139,140}$Te were measured for the first time. The data reveals a strong $N$=82 shell gap at $Z$=50 but indicates the importance of correlations for $Z>50$. An empirical neutron pairing gap expressed as the odd-even staggering of isotopic masses shows a strong quenching across $N$=82 for Sn, with the $Z$-dependence that is unexplainable by the current theoretical models.
Production of pure samples of 131mXe and 135Xe
2011
Pure samples of (131m)Xe, (133m)Xe, (133)Xe and (135)Xe facilitate the calibration and testing of noble gas sampler stations and related laboratory instrumentation. We have earlier reported a Penning trap-based production method for pure (133m)Xe and (133)Xe samples. Here we complete the work by reporting the successful production of pure (131m)Xe and (135)Xe samples using the same technique. In addition, we present data on xenon release from graphite.
Simulations of the stopping efficiencies of fission ion guides
2017
With the Ion Guide Isotope Separator On-Line (IGISOL) facility, located at the University of Jyväskylä, products of nuclear reactions are separated by mass. The high resolving power of the JYFLTRAP Penning trap, with full separation of individual nuclides, capacitates the study of nuclides far from the line of stability. For the production of neutron-rich medium-heavy nuclides, fissioning of actinides is a feasible reaction. This can be achieved with protons from an in-house accelerator or, alternatively, with neutrons through the addition of a newly developed Be(p,xn)-converter. The hereby-obtained fission products are used in nuclear data measurements, for example fission yields, nuclear …
Total absorption spectroscopy of fission fragments relevant for reactor antineutrino spectra
2016
International audience; The accurate determination of reactor antineutrino spectra remains a very active research topic for which new methods of study have emerged in recent years. Indeed, following the long-recognized reactor anomaly (measured antineutrino deficit in short baseline reactor experiments when compared with spectral predictions), the three international reactor neutrino experiments Double Chooz, Daya Bay and Reno have recently demonstrated the existence of spectral distortions in their measurements with respect to the same predictions. These spectral predictions were obtained through the conversion of integral beta-energy spectra obtained at the ILL research reactor. Several s…
Characterization of a neutron-beta counting system with beta-delayed neutron emitters
2016
Abstract A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known β-delayed neutron emission properties. The setup consists of BELEN-20, a 4π neutron counter with twenty 3He proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for β counting and a self-triggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, β and β–neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on …
Isomeric states close to doubly magic $^{132}$Sn studied with JYFLTRAP
2012
The double Penning trap mass spectrometer JYFLTRAP has been employed to measure masses and excitation energies for $11/2^-$ isomers in $^{121}$Cd, $^{123}$Cd, $^{125}$Cd and $^{133}$Te, for $1/2^-$ isomers in $^{129}$In and $^{131}$In, and for $7^-$ isomers in $^{130}$Sn and $^{134}$Sb. These first direct mass measurements of the Cd and In isomers reveal deviations to the excitation energies based on results from beta-decay experiments and yield new information on neutron- and proton-hole states close to $^{132}$Sn. A new excitation energy of 144(4) keV has been determined for $^{123}$Cd$^m$. A good agreement with the precisely known excitation energies of $^{121}$Cd$^m$, $^{130}$Sn$^m$, an…
High-precision mass measurements of 25Al and 30P at JYFLTRAP
2016
The masses of the astrophysically relevant nuclei 25Al and 30P have been measured with a Penning trap for the first time. The mass-excess values for 25Al ( $\Delta = -8915.962(63)$ keV) and 30P ( $\Delta = -20200.854(64)$ keV) obtained with the JYFLTRAP double Penning trap mass spectrometer are in good agreement with the Atomic Mass Evaluation 2012 values but $ \approx$ 5-10 times more precise. A high precision is required for calculating resonant proton-capture rates of astrophysically important reactions 25Al (p, $ \gamma$ )26Si and 30P(p, $ \gamma$ )31S . In this work, $ Q_{(p,\gamma)} = 5513.99(13)$ keV and $ Q_{(p,\gamma)} = 6130.64(24)$ keV were obtained for 25Al and 30P , respectivel…
Independent isotopic yields in 25 MeV and 50 MeV proton-induced fission of natU
2016
Independent isotopic yields for elements from Zn to La in the 25 MeV proton-induced fission of natUnatU were determined with the JYFLTRAP facility. In addition, isotopic yields for Zn, Ga, Rb, Sr, Zr, Pd and Xe in the 50 MeV proton-induced fission of natUnatU were measured. The deduced isotopic yield distributions are compared with a Rubchenya model, the GEF model with universal parameters and the semi-empirical Wahl model. Of these, the Rubchenya model gives the best overall agreement with the obtained data. Combining the isotopic yield data with mass yield data to obtain the absolute independent yields was attempted. The result depends on the mass yield distribution. peerReviewed
MONSTER: a time of flight spectrometer for β-delayed neutron emission measurements
2012
The knowledge of the β-decay properties of nuclei contributes decisively to our understanding of nuclear phenomena: the β-delayed neutron emission of neutron rich nuclei plays an important role in the nucleosynthesis r-process and constitutes a probe for nuclear structure of very neutron rich nuclei providing information about the high energy part of the full beta strength (Sβ) function. In addition, β-delayed neutrons are essential for the control and safety of nuclear reactors. In order to determine the neutron energy spectra and emission probabilities from neutron precursors a MOdular Neutron time-of-flight SpectromeTER (MONSTER) has been proposed for the DESPEC experiment at the future …
Measurements of isomeric yield ratios of fission products from proton-induced fission on natU and 232Th via direct ion counting
2017
Independent isomeric yield ratios (IYR) of 81Ge, 96Y, 97Y, 97Nb, 128Sn and 130Sn have been determined in the 25 MeV proton-induced fission of natU and 232Th. The measurements were performed at the Ion Guide Isotope Separator On-Line (IGISOL) facility at the University of Jyväskylä. A direct ion counting measurement of the isomeric fission yield ratios was accomplished for the first time, registering the fission products in less than a second after their production. In addition, the IYRs of natU were measured by means of γ-spectroscopy in order to verify the consistency of the recently upgraded experimental setup. From the obtained results, indications of a dependence of the production rate …
Mass Measurements for the rp Process
2017
One of the key parameters for the reaction network calculations for the rapid proton capture (rp) process, occurring e.g., in type I X-ray bursts, are the masses of the involved nuclei. Nowadays, masses of even rather exotic nuclei can be measured very precisely employing Penning-trap mass spectrometry. With the JYFLTRAP Penning trap at the IGISOL facility, masses of around 100 neutron-deficient nuclei have been determined with a typical precision of a few keV. Most recently, 25Al, 30P, 31Cl, and 52Co have been measured. Of these, the precision of the mass-excess value of 31Cl was improved from 50 to 3.4 keV, and the mass of 52Co was experimentally determined for the first time. The mass of…
Fission studies at IGISOL/JYFLTRAP: Simulations of the ion guide for neutron-induced fission and comparison with experimental data
2020
For the production of exotic nuclei at the IGISOL facility, an ion guide for neutron-induced fission has been developed and tested in experiments. Fission fragments are produced inside the ion guide and collected using a helium buffer gas. Meanwhile, a GEANT4 model has been developed to simulate the transportation and stopping of the charged fission products. In a recent measurement of neutron-induced fission yields, implantation foils were located at different positions in the ion guide. The gamma spectra from these foils and the fission targets are compared to the results from the GEANT4 simulation. In order to allow fission yield measurements in the low yield regions, towards the tails a…
First evidence of multiple β-delayed neutron emission for isotopes with a > 100
2017
The β-delayed neutron emission probability, Pn, of very neutron-rich nuclei allows us to achieve a better understanding of the nuclear structure above the neutron separation energy, Sn. The emission of neutrons can become the dominant decay process in neutron-rich astrophysical phenomena such as the rapid neutron capture process (r-process). There are around 600 accessible isotopes for which β-delayed one-neutron emission (β1n) is energetically allowed, but the branching ratio has only been determined for about one third of them. β1n decays have been experimentally measured up to the mass A ∼ 150, plus a single measurement of 210Tl. Concerning two-neutron emitters (β2n), ∼ 300 isotopes are …
Precision Mass Measurements beyondSn132: Anomalous Behavior of Odd-Even Staggering of Binding Energies
2012
Atomic masses of the neutron-rich isotopes $^{121--128}\mathrm{Cd}$, $^{129,131}\mathrm{In}$, $^{130--135}\mathrm{Sn}$, $^{131--136}\mathrm{Sb}$, and $^{132--140}\mathrm{Te}$ have been measured with high precision (10 ppb) using the Penning-trap mass spectrometer JYFLTRAP. Among these, the masses of four $r$-process nuclei $^{135}\mathrm{Sn}$, $^{136}\mathrm{Sb}$, and $^{139,140}\mathrm{Te}$ were measured for the first time. An empirical neutron pairing gap expressed as the odd-even staggering of isotopic masses shows a strong quenching across $N=82$ for Sn, with a $Z$ dependence that is unexplainable by the current theoretical models.
r Process (n, γ) Rate Constraints from the γ Emission of Neutron Unbound States in β decay
2017
Total absorption gamma-ray spectroscopy is used to measure accurately the intensity of γγ emission from neutron-unbound states populated in the ββ-decay of delayed-neutron emitters. From the comparison of this intensity with the intensity of neutron emission a constraint on the (n, γγ) cross section for highly unstable neutron-rich nuclei can be deduced. A surprisingly large γγ branching was observed for a number of isotopes which might indicate the need to increase by a large factor the Hauser-Feshbach (n, γγ) cross-section estimates that impact on r process abundance calculations. peerReviewed
Recent mass measurements for the r process at JYFLTRAP
2013
Mass Measurements for the rp Process
2017
Summation Calculations for Reactor Antineutrino Spectra, Decay Heat and Delayed Neutron Fractions Involving New TAGS Data and Evaluated Databases
2018
9 pags., 3 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Design of a neutron converter for fission studies at the IGISOL facility
2012
The upgraded IGISOL facility with JYFLTRAP, at the accelerator laboratory of the University of Jyvaskyla, has been supplied with a new cyclotron which will provide proton or deuteron beams of the order of 100 μA with up to 30 MeV energy. This makes it an ideal place for measurements of neutron-induced fission fragments from various actinides, in view of proposed future nuclear fuel cycles. In the present paper, some considerations for the design of a neutron converter, based on simulations with the Monte Carlo codes MCNPX and FLUKA, are described.
Production of Sn and Sb isotopes in high-energy neutron induced fission of natU
2018
The first systematic measurement of neutron-induced fission yields has been performed at the upgraded IGISOL-4 facility at the University of Jyväskylä, Finland. The fission products from high-energy neutron-induced fission of nat U were stopped in a gas cell filled with helium buffer gas, and were online separated with a dipole magnet. The isobars, with masses in the range A = 128-133 , were transported to a tape-implantation station and identified using γ -spectroscopy. We report here the relative cumulative isotopic yields of tin (Z = 50) and the relative independent isotopic yields of antimony (Z = 51). Isomeric yield ratios were also obtained for five nuclides. The yields of tin show a …
Coulomb displacement energies as a probe for nucleon pairing in the $f_{7/2}$ shell
2014
Coulomb displacement energies of $T=1/2$ mirror nuclei have been studied via a series of high-precision $Q_\mathrm{EC}$-value measurements with the double Penning trap mass spectrometer JYFLTRAP. Most recently, the $Q_\mathrm{EC}$ values of the $f_{7/2}$-shell mirror nuclei $^{45}$V ($Q_\mathrm{EC}=7123.82(22)$ keV) and $^{49}$Mn ($Q_\mathrm{EC}=7712.42(24)$ keV) have been measured with an unprecedented precision. The data reveal a 16-keV ($1.6\sigma$) offset in the adopted Atomic Mass Evaluation 2012 value of $^{49}$Mn suggesting the need for further measurements to verify the breakdown of the quadratic form of the isobaric multiplet mass equation. Precisely measured $Q_\mathrm{EC}$ values…
A ROOT-based analysis tool for measurements of neutron-induced fission products at the IGISOL facility
2012
For the sustainable development of nuclear energy, the handling of used nuclear fuel is a key issue. Innovative fuel cycles are being developed for the transmutation of minor actinides and long-lived fission products. In view of these developments, accurate knowledge of the fuel inventory is necessary. The IGISOL facility with JYFLTRAP, at the accelerator laboratory of the University of Jyvaskyla, will be used to measure independent fission yield distributions from neutron-induced fission on different actinides. In this paper, an analysis tool is developed, using the CERN-based ROOT Data Analysis Framework, with the objective of performing full data analysis within the same code. The analys…
Advanced model for the prediction of the neutron-rich fission product yields
2013
The consistent models for the description of the independent fission product formation cross sections in the spontaneous fission and in the neutron and proton induced fission at the energies up to 100 MeV is developed. This model is a combination of new version of the two-component exciton model and a time-dependent statistical model for fusion-fission process with inclusion of dynamical effects for accurate calculations of nucleon composition and excitation energy of the fissioning nucleus at the scission point. For each member of the compound nucleus ensemble at the scission point, the primary fission fragment characteristics: kinetic and excitation energies and their yields are calculate…
Characterization and performance of the DTAS detector
2018
11 pags., 16 figs., 3 tabs.
A neutron source for IGISOL-JYFLTRAP : Design and characterisation
2017
A white neutron source based on the Be(p, nx) reaction for fission studies at the IGISOL-JYFLTRAP facility has been designed and tested. 30MeV protons impinge on a 5mm thick water-cooled beryllium disc. The source was designed to produce at least 1012 fast neutrons/s on a secondary fission target, in order to reach competitive production rates of fission products far from the valley of stability. The Monte Carlo codes MCNPX and FLUKA were used in the design phase to simulate the neutron energy spectra. Two experiments to characterise the neutron field were performed: the first was carried out at The Svedberg Laboratory in Uppsala (SE), using an Extended-Range Bonner Sphere Spectrometer and …
QECvalues of the superallowedβemittersC10,Ar34,Ca38, andV46
2011
The ${Q}_{\mathrm{EC}}$ values of the superallowed ${\ensuremath{\beta}}^{+}$ emitters $^{10}\mathrm{C}$, $^{34}\mathrm{Ar}$, $^{38}\mathrm{Ca}$, and $^{46}\mathrm{V}$ have been measured with the JYFLTRAP Penning-trap mass spectrometer to be 3648.12(8), 6061.83(8), 6612.12(7), and 7052.44(10) keV, respectively. All four values are substantially improved in precision over previous results. Of the well-known superallowed emitters, only $^{14}\mathrm{O}$ has yet to have had its ${Q}_{\mathrm{EC}}$ value measured with a Penning trap.
First experiment with the NUSTAR/FAIR Decay Total Absorption γ-Ray Spectrometer (DTAS) at the IGISOL IV facility
2015
V. Guadilla et al. ; 4 págs.; 4 figs.; 1 tab.
JYFLTRAP: a Penning trap for precision mass spectroscopy and isobaric purification
2012
In this article a comprehensive description and performance of the double Penning-trap setup JYFLTRAP will be detailed. The setup is designed for atomic mass measurements of both radioactive and stable ions and additionally serves as a very high-resolution mass separator. The setup is coupled to the IGISOL facility at the accelerator laboratory of the University of Jyväskylä. The trap has been online since 2003 and it was shut down in the summer of 2010 for relocation to the upgraded IGISOL facility. Numerous atomic mass and decay energy measurements have been performed using the time-of-flight ion-cyclotron resonance technique. The trap has also been used in several decay spectroscopy expe…
Accurate Fission Data for Nuclear Safety
2013
The Accurate fission data for nuclear safety (AlFONS) project aims at high precision measurements of fission yields, using the renewed IGISOL mass separator facility in combination with a new high current light ion cyclotron at the University of Jyvaskyla. The 30 MeV proton beam will be used to create fast and thermal neutron spectra for the study of neutron induced fission yields. Thanks to a series of mass separating elements, culminating with the JYFLTRAP Penning trap, it is possible to achieve a mass resolving power in the order of a few hundred thousands. In this paper we present the experimental setup and the design of a neutron converter target for IGISOL. The goal is to have a flexi…
Characterization of a cylindrical plastic {\beta}-detector with Monte Carlo simulations of optical photons
2017
V. Guadilla et al. -- 5 pags., 8 figs., tab.
Fission yield measurements at IGISOL
2016
The fission product yields are an important characteristic of the fission process. In fundamental physics, knowledge of the yield distributions is needed to better understand the fission process. For nuclear energy applications good knowledge of neutroninduced fission-product yields is important for the safe and efficient operation of nuclear power plants. With the Ion Guide Isotope Separator On-Line (IGISOL) technique, products of nuclear reactions are stopped in a buffer gas and then extracted and separated by mass. Thanks to the high resolving power of the JYFLTRAP Penning trap, at University of Jyväskylä, fission products can be isobarically separated, making it possible to measure rela…
Trap-assisted separation of nuclear states for gamma-ray spectroscopy: the example of100Nb
2011
Low-lying levels in 100Mo are known to be populated by beta decay from both the ground and isomeric states in 100Nb. The small energy difference (~3 ppm) between the two parent states and the similarity of their half-lives make it difficult to distinguish experimentally between the two decay paths. A new technique for separating different states of nuclei has recently been developed in a series of experiments at the IGISOL facility, using the JYFLTRAP installation, at the University of Jyvaskyla where mass resolution ~2 ppm was achieved in mass measurements and in the production of 133mXe. This paper reports on the extension of this technique to allow the separate study of the gamma-ray dec…
Large Impact of the Decay of Niobium Isomers on the Reactor ν¯e Summation Calculations
2019
Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data ob…
TAGS measurements of $^{100}$Nb ground and isomeric states and $^{140}$Cs for neutrino physics with the new DTAS detector
2016
V. Guadilla et al. -- 4 pags., 6 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Disentangling decaying isomers and searching for signatures of collective excitations in β decay
2019
6 pags., 3 figs., 1 tab. -- 27th International Nuclear Physics Conference (INPC2019) 29 July - 2 August 2019, Glasgow, UK